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RESEARCH PAPER · Reaction Chemistry & Engineering · 2022

Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes

Linxiao Chen, Yifeng Zhu, Laura C. Meyer, Lillian Hale, Thuy Thanh Le, Abhijeet Karkamkar, Johannes A. Lercher, Oliver Y. Gutiérrez, János Szanyi

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Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanesOriginalHydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Current Prospects for Plastic Waste Treatment163Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Catalytic conversion of polyethylene into aromatics with Pt/ZSM-5: insights into reaction pathways and rate-controlling step regulation53Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Transport limitations in polyolefin cracking at the single catalyst particle level66Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways31Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals61Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Synergistic Effect of Activated Carbon, NiO and Al2O3 on Improving the Thermal Stability and Flame Retardancy of Polypropylene Composites9A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113A two-stage strategy for upcycling chlorine-contaminated plastic waste141Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Upcycling of polyvinyl chloride to hydrocarbon waxes via dechlorination and catalytic hydrogenation50Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Ni-catalyzed carbon–carbon bonds cleavage of mixed polyolefin plastics waste42Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26Thermodynamic and Kinetic Insights into Hydrogen Adsorption and Dissociation on the Ru (0001) Surface under STM and Catalytic Conditions11Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture17Precise activation of C–C bonds for recycling and upcycling of plastics81Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins39Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Fundamental, technical and environmental overviews of plastic chemical recycling88Synthesis of α-methylene-δ-valerolactone and its selective polymerization from a product mixture for concurrent separation and polymer production6Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Population Balance Equations for Reactive Separation in Polymer Upcycling20Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45Interfacial Reactions in Chemical Recycling and Upcycling of Plastics18Polyolefin melt-phase effects on alkane hydrogenolysis over Pt catalysts5Catalytic recycling of plastics into value-added products28Effect of CeO2 morphology and Ru impregnation method on CH4 selectivity reduction in polyethylene waste conversion to liquid fuels and lubricants15Applications of nickel-containing structured microfibrous catalysts for the process of propane hydrogenolysis0Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes12Computational insights into hydrogen interaction with the Ru (1011) and Ru (1010) surfaces: implications for alkane and polyolefin hydrogenolysis1Hydrogenolysis and hydrocracking of biomass and plastic wastes to produce high-value products1Revolutionizing Solid Hydrocarbon Sourcing: Plastic’s Journey from Waste to Upcycled Treasure50Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Upgrading of waste polyolefins with non-noble metal catalysts21Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Using Nickel-Containing Structured Microfiber Catalysts in the Hydrogenolysis of Propane0Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Upcycling of Waste Plastics into Value-Added Chemicals6Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Optimized pyrolysis of household plastic waste in Indonesia for oil production: Hydrocarbon profiling, fuel alternative, and potential biomedical application9Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Co-recycling of plastics and other waste materials70Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Catalytic Upcycling of Polyethylene into Naphtha Using Commercial Heterogeneous Catalysts3Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Tuning Catalytic Reactivity via Wetting Control through Oxygen Vacancies: Ru Clusters on Anatase TiO2 and CeO2 Supports22Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Advancing chemical recycling for waste plastic conversion1Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking11Research progress of high value utilization of waste polyethylene plastics6Benchmarking electro-Fenton-driven decomposition of synthetic polymers0Carbon–carbon bond cleavage for lignin and plastics deconstruction0Case Studies on the Polymer-Water Nexus: Microplastic Degradation Using Catalyzed Wet Oxidation0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Steering C–C bond cleavage and hydrogenation in polystyrene hydrocracking through external Brønsted acid sites over Ni/zeolites1Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis6Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Advancing Waste Plastic Valorization: Catalytic Production of Aviation Fuel over Zeolite and Ru/CNT-Based Catalysts4Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3One-pot co-upcycling of mixed polyolefin waste6Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Synergistic Mechanisms and Product Regulation in the Co-Pyrolysis of Biomass and Food Packaging Waste: A Study Based on Reaction Kinetics and GHG Calculation1Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling0Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Hydrotreatment of Nylon 66 and Amide Model Compounds Over Sulfided NiMo Catalysts0Sustainable Aviation Fuel (SAF): A Mini-Review of Advances in Catalytic Pathways Using Lipid-Based Feedstocks and Plastic Waste3Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Acyclic Hydrocarbon α , ω ‐Dienes: From Biomass and Plastic Upcycling to Carbocycles, Precision Polymers, and Cross‐Linked Elastomers0Catalytic Hydrothermal Liquefaction of Polyethylene With Pt/C to Tune Product Selectivity0Internal transport modulates catalytic hydrogenolysis of polyolefins0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0Molecular Insights into Competitive Adsorption in the Deconstruction of Mixed Polyolefin Waste0

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