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RESEARCH PAPER · JACS Au · 2023

Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins

Manav Chauhan, Neha Antil, Bharti Rana, Naved Akhtar, Chhaya Thadhani, Wahida Begum, Kuntal Manna

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Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of PolyolefinsOriginalVariation in Catalytic Efficacies of a 2D pH‐Stable MOF by Altering Activation Methods26Mechanochemical Encapsulation of Enzymes into MOFs for Photoenzymatic Enantioselective Catalysis32Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Metal–Organic Framework-Supported Mono Bipyridyl–Iron Hydroxyl Catalyst for Selective Benzene Hydroxylation into Phenol13Catalytic chemical recycling and upcycling of polyolefin plastics27Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks38Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks10Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23N -Alkylation of aniline derivatives by a bipyridyl metal–organic framework supported cobalt catalyst2Advancements in Cancer Treatment: Harnessing the Synergistic Potential of Graphene-Based Nanomaterials in Combination Therapy25Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Architecting molecularly dispersed Cu(I)-active sites at UiO-MOF nodes for thermocatalytic oxidation of methane to ethanol using O210Defective Metal–Organic Frameworks Confined PdO with High Resistance to Reduction: An Efficient Photocatalyst for Hydrodeoxygenation of Lignin Derivatives24Engineering Mono- vs Dinuclear Iron(II)-Active Sites to Steer Liquid Oxygenate Selectivity in Methane Oxidation Pathways Using O217Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Cobalt Catalyzed Selective Monoborylation of Methane8CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20Metal–organic frameworks: frontier of surface organometallic chemistry3Catalytic Depolymerization of Plastics to Valuable Products7Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Synthesis of 1,4‐DHP‐Based Bio‐Active Molecules by a pH‐Stable Lewis Acidic Ni‐MOF Catalyst2Architecting Metal–Organic Framework-Based/Derived Catalysts for Methane Functionalization7Regioselective hydroboration of alkenes by metal-organic framework confined mononuclear bipyridyl–iron hydride catalyst3Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Controlled Pyrolysis of Polystyrene Using Metal–Organic Frameworks4Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Liquid-Dependent Structural Responses of a Metal–Organic Framework Revealed by Liquid-Phase Three-Dimensional Electron Diffraction0Emerging Catalytic Platforms for Plastic Waste Recycling and Upcycling Over MOFs and COFs: Catalyst Engineering and Reaction Mechanisms0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0

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  2. Mechanochemical Encapsulation of Enzymes into MOFs for Photoenzymatic Enantioselective Catalysis

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  3. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

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  4. Metal–Organic Framework-Supported Mono Bipyridyl–Iron Hydroxyl Catalyst for Selective Benzene Hydroxylation into Phenol

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  5. Catalytic chemical recycling and upcycling of polyolefin plastics

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  7. Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks

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  8. Catalytic Upcycling of Polyolefins

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  9. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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  10. Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts

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  11. Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development

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  12. N -Alkylation of aniline derivatives by a bipyridyl metal–organic framework supported cobalt catalyst

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  13. Advancements in Cancer Treatment: Harnessing the Synergistic Potential of Graphene-Based Nanomaterials in Combination Therapy

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  14. Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions

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  15. MOF Catalysts for Plastic Depolymerization

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  16. MOF Catalysts for Plastic Depolymerization

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  17. Architecting molecularly dispersed Cu(I)-active sites at UiO-MOF nodes for thermocatalytic oxidation of methane to ethanol using O2

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  18. Defective Metal–Organic Frameworks Confined PdO with High Resistance to Reduction: An Efficient Photocatalyst for Hydrodeoxygenation of Lignin Derivatives

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  19. Engineering Mono- vs Dinuclear Iron(II)-Active Sites to Steer Liquid Oxygenate Selectivity in Methane Oxidation Pathways Using O2

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  20. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

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  21. Cobalt Catalyzed Selective Monoborylation of Methane

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  22. CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor

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  24. Catalytic Depolymerization of Plastics to Valuable Products

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  25. Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst

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  34. Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst

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  35. A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis

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