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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins

Akalanka Tennakoon, Xun Wei Wu, Max Meirow, Daniel Howell, Jarod Willmon, Jiaqi Yu, Jessica V. Lamb, Massimiliano Delferro, Erik Luijten, Wenyu Huang, Aaron David Sadow

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Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of PolyolefinsOriginalPerspectives from the 2022 Cohort of the American Chemical Society Summer School on Green Chemistry & Sustainable Energy13Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8A multiscale investigation of polypropylene glycol polymer upcycling to propionaldehyde via catalytic cracking on acid sites of mesoporous Y zeolites2Advances in catalytic chemical recycling of synthetic textiles43Characterization of polymer properties and identification of additives in commercially available research plastics112Opportunities and challenges for plastic depolymerization by biomimetic catalysis36Removal of phenoxy acid herbicide from water by magnetic mesoporous silicate1Artificial Processive Catalytic Systems3Population Balance Equations for Reactive Separation in Polymer Upcycling20Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex12Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex3Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59The Overlooked Potential of Sulfated Zirconia: Reexamining Solid Superacidity Toward the Controlled Depolymerization of Polyolefins11Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Chemical upcycling of high-density polyethylene into upcycled waxes as rheology modifiers and paper coating materials12Recycling polyolefin plastic waste at short contact times via rapid joule heating93Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Nanoengineering Multilength-Scale Porous Hierarchy in Mesoporous Metal–Organic Framework Single Crystals73Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Accurately tuning the pore size and acidity of mesoporous zeolites for enhancing the catalytic hydrocracking of polypropylene24Photothermal Catalytic Recycling of Polyester Over Magnetic Ni−MnO x Nanocatalyst16Mo-modified MCM-48 encapsulated ZSM-5 core–shell catalyst for methane dehydro-aromatization with enhanced activity and stability0Upgrading of waste polyolefins with non-noble metal catalysts21Ligand-Shell Cooperativity in a Bilayer Silica-Sandwiched Mixed-Metals Nanocatalyst Design for Absolute Selectivity Switch3Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Upcycling of Waste Plastics into Value-Added Chemicals6Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Synergistic Catalysis for Recycling and Upcycling of Plastics35Coordinating cracking and hydrogenation of polyethylene waste via acid-metal site isolation for selective hydrocarbon production10Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Methods for Carbon Mass Closure in Polyolefin Hydrocracking6CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Self-supporting characteristics in hierarchical monolith catalyst with highly accessible active sites for boosting lean methane catalytic oxidation8Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Ligand–Substrate Self-Sorting in Silica-Encased Rh-Nanopetals as Model Catalyst for Hydroformylation of Arylalkenes0Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11On the Influence of Catalyst Mesopore Structure in the Catalytic Cracking of Polypropylene1Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants2Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Research progress of high value utilization of waste polyethylene plastics6Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe12A semi-flow reactor design diverts catalytic hydrogenolysis of polyolefins to metastable kinetic products1Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Polymer Deconstruction and Redesign Strategies for Plastics Recycling0Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Upcycling plastic waste into high‑performance lubricants: Enabled by robust and synergistic tribofilm formation with MoDTC and ZDDP0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Short-Range Order Stabilized Ultrafine Pd on Carbon-Supported Medium-Entropy Mesoporous Interfaces for Plastic Upcycling0

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  2. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

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