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RESEARCH PAPER · ACS Catalysis · 2024

Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation

Yi‐Yu Wang, Akalanka Tennakoon, Xun Wei Wu, Chinmay Sahasrabudhe, Long Hao Qi, Baron Peters, Aaron David Sadow, Wenyu Huang

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Catalytic Hydrogenolysis of Polyethylene Under Reactive SeparationOriginalThermal oxo-degradation of plastic wastes to valuable compounds0Population Balance Equations for Reactive Separation in Polymer Upcycling20Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316Influence of Trace Metal in Plastics on Catalyst Activity and Reusability during Polyolefins Upcycling with Polyoxometalates2Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Photothermal Catalytic Recycling of Polyester Over Magnetic Ni−MnO x Nanocatalyst16Upcycling of waste plastics: strategies, status-quo, and prospects3Recent developments in recycling of post-consumer polyethylene waste33Polymer Molecular Weight Distributions: A Tutorial on Transformations between Number Density, Mass Density, and Linear/Logarithmic Axes4Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Optimization of low-temperature catalytic cracking of polyolefin waste in open-batch reactors using zeolite beta with controlled intrinsic properties20Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions17Primary products from kinetic-limited high-density polyethylene pyrolysis at near vacuum7Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors8Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Thermal Oxo-degradation and Catalytic Upgrading of Plastic Waste to Light Olefins for a Circular Economy7Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Advancing chemical recycling for waste plastic conversion1Valorization of plastic waste into drop-in fuels: Economic and environmental perspectives16Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants2Breaking the yield–selectivity trade-off in polystyrene waste valorization via tandem depolymerization and hydrogenolysis18Thermochemical upcycling of plastic waste: A comprehensive view from technology to commercialization2Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling4An integrated techno-economic analysis and life cycle assessment of lube oil production from post-use polypropylene and comparison with conventional base oils0Plastic Waste Conversion into Monomers Using Microwaves0A semi-flow reactor design diverts catalytic hydrogenolysis of polyolefins to metastable kinetic products1Material Engineering of Cu 0 /Cu + Sites and Oxygen Vacancies for Efficient In Situ Hydrodeoxygenation of Lignin‐Based Compounds4Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene0Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Polystyrene waste valorization via selective C–C bond cleavage: the second life of polymers0The Influence of Incorporating Alkaline Metals on Alumina for Xylitol Hydrogenolysis over Ni Catalysts1Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Upcycling plastic waste into high‑performance lubricants: Enabled by robust and synergistic tribofilm formation with MoDTC and ZDDP0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0In-situ hydrogen generation via water-gas shift reaction over Ni-Fe3O4/USY: A sustainable pathway for efficient polypropylene hydrogenolysis0

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  1. Thermal oxo-degradation of plastic wastes to valuable compounds

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  2. Population Balance Equations for Reactive Separation in Polymer Upcycling

    Langmuir · 2024-02-13

    Changhae Andrew Kim, Chinmay Sahasrabudhe, Yiyu Wang, Ryan D. Yappert, Andreas Heyden, Wenyu Huang, Aaron David Sadow, Baron Peters

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  3. Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts

    Materials · 2024-04-18

    Hyungjin Cho, Ahyeon Jin, Sun‐Ju Kim, Young-Min Kwon, Eunseo Lee, Jae Man Shin, Byung Hyo Kim

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  4. Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity

    ACS Sustainable Resource Management · 2024-06-10

    Makenna L. Pennel, Yile Jiang, Matteo Cargnello

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  5. Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering

    Macromolecules · 2024-08-13

    Xuchun Wang, Xingyi Lyu, Xun Wei Wu, Lilin He, Jessica V. Lamb, Alexander S. Filatov, Massimiliano Delferro, Wenyu Huang, Byeongdu Lee

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  6. Catalytic Upcycling of Polyolefins

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    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  7. Influence of Trace Metal in Plastics on Catalyst Activity and Reusability during Polyolefins Upcycling with Polyoxometalates

    ACS Catalysis · 2024-10-07

    Hongda Zhu, Justin T. Douglas, Bala Subramaniam

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  8. Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling

    Nature Communications · 2024-11-29

    Taeeun Kwon, Byeongchan Ahn, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  9. Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies

    Industrial & Engineering Chemistry Research · 2024-12-06

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  10. Photothermal Catalytic Recycling of Polyester Over Magnetic Ni−MnO x Nanocatalyst

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    Xiaofei Lai, Shiyun Xiong, Biao Jiang, Yong Xu

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  11. Upcycling of waste plastics: strategies, status-quo, and prospects

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  12. Recent developments in recycling of post-consumer polyethylene waste

    Green Chemistry · 2025-01-01

    Yang Ma, Xinyao Jiang, Xinyue Xiang, Ping Qu, Maiyong Zhu

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  13. Polymer Molecular Weight Distributions: A Tutorial on Transformations between Number Density, Mass Density, and Linear/Logarithmic Axes

    Industrial & Engineering Chemistry Research · 2025-02-06

    Ziqiu Chen, Changhae Andrew Kim, Yiyu Wang, Aaron David Sadow, Anne M. LaPointe, Baron Peters

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  14. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  15. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

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  16. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  17. Optimization of low-temperature catalytic cracking of polyolefin waste in open-batch reactors using zeolite beta with controlled intrinsic properties

    Communications Engineering · 2025-03-24

    Hankyeul Kang, Junghwa Yoon, Dongwoo Jun, Ki Hyuk Kang, Insoo Ro, Soo-Hwa Jeong, Jong Hun Kang

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  18. Polyethylene Upcycling to Liquid Alkanes in Molten Salts under Neat and External Hydrogen Source-Free Conditions

    Journal of the American Chemical Society · 2025-04-07

    Liqi Qiu, Felipe Polo‐Garzon, Luke L. Daemen, Min-Jae Kim, Jinghua Guo, Bobby G. Sumpter, Michael Köehler, Carlos Alberto Steren, Tao Wang, Logan T. Kearney, Tomonori Saito, Zhenzhen Yang, Sheng Dai

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  19. Primary products from kinetic-limited high-density polyethylene pyrolysis at near vacuum

    Chemical Engineering Journal · 2025-05-03

    M. Doga Tekbas, Matthew R. Wright, Hsi‐Wu Wong

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  20. Population Balance Models for Catalytic Depolymerization: From Elementary Steps to Multiphase Reactors

    Accounts of Chemical Research · 2025-05-16

    Lela K. Manis, Jiankai Ge, Changhae Andrew Kim, Emmanuel Ejiogu, Ziqiu Chen, Ryan D. Yappert, Baron Peters

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  21. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

    JACS Au · 2025-07-24

    Anna E. Brenner, Griffin Drake, Gregg T. Beckham, Yuriy Román‐Leshkov

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  22. Thermal Oxo-degradation and Catalytic Upgrading of Plastic Waste to Light Olefins for a Circular Economy

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    Jessica L. Brown, Harish Radhakrishnan, Isabel Coffman, Khairun N. Tumu, Greg W. Curtzwiler, Keith L. Vorst, Ryan Smith, Robert C. Brown, Xianglan Bai, Tannon J. Daugaard

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  23. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

    ACS Catalysis · 2025-09-23

    Zachary M. Gdowski, Rishi Raj, Aditya Bhan, K. Andre Mkhoyan, Mahesh K. Mahanthappa, Frank S. Bates

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  24. Advancing chemical recycling for waste plastic conversion

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  25. Valorization of plastic waste into drop-in fuels: Economic and environmental perspectives

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  26. Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants

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  27. Breaking the yield–selectivity trade-off in polystyrene waste valorization via tandem depolymerization and hydrogenolysis

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  28. Thermochemical upcycling of plastic waste: A comprehensive view from technology to commercialization

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  30. An integrated techno-economic analysis and life cycle assessment of lube oil production from post-use polypropylene and comparison with conventional base oils

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  31. Plastic Waste Conversion into Monomers Using Microwaves

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  32. A semi-flow reactor design diverts catalytic hydrogenolysis of polyolefins to metastable kinetic products

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  33. Material Engineering of Cu 0 /Cu + Sites and Oxygen Vacancies for Efficient In Situ Hydrodeoxygenation of Lignin‐Based Compounds

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  35. Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling

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  36. Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene

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  37. Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene

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  38. Polystyrene waste valorization via selective C–C bond cleavage: the second life of polymers

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  39. The Influence of Incorporating Alkaline Metals on Alumina for Xylitol Hydrogenolysis over Ni Catalysts

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  42. Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons

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  44. Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management

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  45. In-situ hydrogen generation via water-gas shift reaction over Ni-Fe3O4/USY: A sustainable pathway for efficient polypropylene hydrogenolysis

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