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RESEARCH PAPER · Science Advances · 2023

A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins

Zetian Qiu, Siyu Lin, Zhuo Chen, Anqi Chen, Yitian Zhou, Xudong Cao, Yu Wang, Bo‐Lin Lin

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A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefinsOriginalEnd-of-Life Plastics Management: A Review7Medium entropy metal oxide induced *OH species targeted transfer strategy for efficient polyethylene terephthalate plastic recycling33Bridging the Gap Between Academia and Chemical Industry through Entrepreneurship: An Account on the Case of Hydrogen-assisted Catalytic Plastic Waste Valorisation0Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins17The catalytic performance of (ZrO) n ( n = 1–4, 12) clusters for Suzuki–Miyaura cross-coupling: a DFT study6Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Coupled conversion of polyethylene and carbon dioxide catalyzed by a zeolite–metal oxide system50Activation of periodate by iron-containing sludge from groundwater treatment plants for degradation of methylene blue in wastewater7Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Catalytic Deconstruction of Ethylene Vinyl Acetate Copolymer and Polyethylene Mixtures via Hydroconversion: Challenges and Solutions8Catalytic chemical recycling and upcycling of polyolefin plastics27Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking24Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316Unlocking the structure-activity relationship of hierarchical MFI zeolites towards the hydrocracking of HDPE14Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst27Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst6Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Induction Heating for the Electrification of Catalytic Processes51Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Can mixed plastics be recycled and upcycled without separation?11Circular plastic economy for sustainable development: current advances and future perspectives49Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Upgrading of waste polyolefins with non-noble metal catalysts21Catalytic and engineering strategies for enhanced hydrogenation reactions: A review of heterogeneous catalysts and process optimization15Biowastes as sustainable catalysts for water treatment: A comprehensive overview20Co-upcycling of polyethylene terephthalate and polyoxymethylene into valuable chemicals13Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Improving hydrogen production via ex-situ catalytic fast pyrolysis of non-thermal plasma pretreated HDPE with 1Fe1Ni/γ-Al2O3 catalyst22Investigating the Role of Acid Sites in the Hydrocracking of Polyethylene-EVOH Multilayer Film Waste over Pt/BEA Catalyst7Persulfate-Based Advanced Oxidation Reforming of Polyethylene Terephthalate Fiber into Formate via Singlet Oxygen Activation25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides26Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Upcycling of Waste Plastics into Value-Added Chemicals6Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Catalytic conversion of oxygen-containing aromatic plastic wastes into cycloalkanes aviation fuels1Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels4Synergistic Catalysis for Recycling and Upcycling of Plastics35Coordinating cracking and hydrogenation of polyethylene waste via acid-metal site isolation for selective hydrocarbon production10Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics7Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics0Overcoming limitations in polyolefins upcycling by codesigning endothermic-exothermic magnetocatalytic system8Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Ambient solar thermal catalysis for polyolefin upcycling using copper encapsulated in silicon nanosheets and chloroaluminate ionic liquid32A Minimalist Design for a Dual-Catalyst System for High-Efficiency Conversion of Waste Plastics into Liquid Fuel Products27Hydroprocessing of waste plastics to produce diesel under low processing temperatures using ionic liquid catalyst6A Multifunctional Photothermal Catalyst Enabling Full‐Day Sustainable Power and Indoor Air Quality Control3Selective electrified polyethylene upcycling by pore-modulated pyrolysis25Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics9Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts3Dual-catalyst system without supported metals toward polyethylene waste upcycling3A review of the pathways, limitations, and perspectives of plastic waste recycling46Thermal Oxo-degradation and Catalytic Upgrading of Plastic Waste to Light Olefins for a Circular Economy7Catalytic Depolymerization of Plastics to Valuable Products7Efficient electrooxidation of PET-derived ethylene glycol using a Fe3O4–NiCo2O4 heterostructure: Toward sustainable plastic upcycling3Bayesian Optimization of Hierarchical ZSM-5 for High-Efficiency Polyolefin Waste Recycling to Light Olefins7Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2Advances and Insights in Electrocatalytic Upcycling of Polyethylene Terephthalate Plastic Wastes23Selective hydrocracking of polystyrene waste over Pt- and Ru-supported zeolite catalysts into high yield LPG and ethylbenzene4Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Multiscale exploration of chemical looping steam gasification of waste plastics: Decomposition behavior, kinetics, mechanism, and polymer specific reactivity for polyethylene, polypropylene, and polystyrene0Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling4A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Direct upcycling of mixed plastic waste into liquid alkanes3Plastic Waste Conversion into Monomers Using Microwaves0Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites3Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites5Photothermal Oxidative Upcycling of Polyethylene to Aliphatic Dicarboxylic Acids over a Pt/TiO 2 Catalyst10Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Compressed CO 2 -Assisted Catalytic Hydrocracking of Polyethylene over Ru-Loaded Zeolites0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Toward a circular plastic economy: A review of life cycle assessment studies on chemical recycling processes for fossil-based plastics2Mechanochemically functionalized waste plastics for NO2 sensing0iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Hydrocracking of polypropylene over Ni-loaded two-dimensional zeolite catalysts for LPG-rich hydrocarbon production0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Catalyst‐Free Upcycling of Polyethylene Waste Into Oxidized Polyethylene Wax1Catalyst‐Free Upcycling of Polyethylene Waste Into Oxidized Polyethylene Wax1Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Collaborative Pt–Ni Sites Enable CO-Tolerant Hydrocracking for Upcycling Polyolefin Waste1Catalyst reusability in plastic-to-fuel conversion: Deactivation mechanisms, regeneration pathways, and scale-up implications3Bifunctional nanocatalyst design for polyolefin hydrocracking2Enabling Refinery Integration for Plastic Waste Recycling: A Probabilistic Techno-economic Analysis and Carbon Footprint Assessment of Poly-Crude Production0Confined Isomerization Enables Solar-Thermal Upcycling of Polyolefins into High-Octane Gasoline0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0Spatially orthogonal CeOx-Zn sites on diatomite-aerogel-derived hierarchical HZSM-5 enable gated dechlorination and BTX-selective upcycling of PVC/PET mixed plastics0Circular management of single-use polyolefins via hydrocracking over zeolite-based catalysts0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. End-of-Life Plastics Management: A Review

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  42. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

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  43. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

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  44. Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides

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  45. Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst

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  46. Upcycling of Waste Plastics into Value-Added Chemicals

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  47. Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling

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  48. Catalytic conversion of oxygen-containing aromatic plastic wastes into cycloalkanes aviation fuels

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  49. Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels

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    Xinlei Han, Yuchen Zhou, Shenglian Chen, Huanhao Chen, Jiuxuan Zhang, Zhengyan Qu, Feng Zeng, Tuo Ji, Hong Li Jiang, Wei Cao, Zhenchen Tang, Rizhi Chen

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  50. Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels

    Angewandte Chemie · 2025-04-29

    Xinlei Han, Yuchen Zhou, Shenglian Chen, Huanhao Chen, Jiuxuan Zhang, Zhengyan Qu, Feng Zeng, Tuo Ji, Hong Li Jiang, Wei Liang Cao, Zhenchen Tang, Rizhi Chen

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