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RESEARCH PAPER · Nature Sustainability · 2023

A two-stage strategy for upcycling chlorine-contaminated plastic waste

Pavel A. Kots, Brandon C. Vance, Caitlin M. Quinn, Cong Wang, Dionisios G. Vlachos

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A two-stage strategy for upcycling chlorine-contaminated plastic wasteOriginalInsights into the evolution of chemical structure and pyrolysis reactivity of PVC-derived hydrochar during hydrothermal carbonization17Upcycling contaminated plastics21Solar-driven photocatalysis for recycling and upcycling plastics122Precise activation of C–C bonds for recycling and upcycling of plastics81Conversion of diverse post-consumer PVC waste materials to PE via dual catalytic tandem dehydrochlorination–hydrogenation14Conversion of waste poly(vinyl chloride) to branched polyethylene mediated by silylium ions29Fundamental, technical and environmental overviews of plastic chemical recycling88Selective Recovery of Para-Xylene from Polyethylene Terephthalate Plastic26Superstructure optimization for management of low-density polyethylene plastic waste24Recent Advancements in Pyrolysis of Halogen-Containing Plastics for Resource Recovery and Halogen Upcycling: A State-of-the-Art Review74Hydrogenation of waste PET degraded bis(2-hydroxyethyl)cyclohexane- 1,4-dicarboxylate to 1,4-cyclohexanedimethanol over Cu-based catalysts15Kill two birds with one stone: To reduce toxicity and enhance photodegradation of antibiotics by lead cesium bromide via tin doping17Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Chlorinated plastics offer unique opportunities and challenges in upcycling25Tandem catalysis enables chlorine-containing waste as chlorination reagents48Rethinking Chlorinated Plastic: Can Direct Upcycling of Mixed Plastic Wastes Surpass Preseparation?2Complete hydrogenolysis of mixed plastic wastes101Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35More Than 30 Years of PVC Recycling—Need for Regulation9Oxygen-mediated acceleration of chloride capture and migration by copper oxide in PVC-based cable pyrolysis1Room-Temperature Upcycling of Mixed PVC and Polyolefin Waste1High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Low-temperature dechlorination of polyvinyl chloride (PVC) for production of H 2 and carbon materials using liquid metal catalysts35Upcycling of polyvinyl chloride to porous carbon for high-performance electromagnetic wave absorption materials40Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Catalytic Synergy between Lewis Acidic Alumina and Pt in Hydrodechlorination for Plastic Chemical Recycling38Catalytic Upcycling of Polyolefins316Unraveling the Impact of Oxygen Vacancy on Electrochemical Valorization of Polyester Over Spinel Oxides32Facile Conversion of Oil Shale Semicoke and Ferrous Sulfate Byproduct into Yellowish-Red α-Fe2O3 Composite Pigments via Twin Screw Extrusion Strategy2Synergistic technologies for a circular economy: upcycling waste plastics and biomass34PVC Dechlorination for Facilitating Plastic Chemical Recycling: A Systematic Literature Review of Technical Advances, Modeling and Assessment25Transformative and sustainable approach to waste plastic mixture valorization5Biotechnology for the degradation and upcycling of traditional plastics10Efficient polycarbonate plastic upcycling into jet fuel cycloalkanes over a bifunctional MoCo/NiC hetero-catalyst12Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Mechanochemical Treatment of Waste Poly (Vinyl Chloride) for Alcohol Halogenation by Ball Milling and Triboelectric Material1Plasmonic Copper‐Ruthenium Superstructure for Efficient Photothermal Conversion and Plastic Recycling39Progress toward sustainable polymer technologies with ball-mill grinding45Critical advances and assessment on chemo-biological conversions of waste polyvinyl chloride10Click dechlorination of halogen-containing hazardous plastics towards recyclable vitrimers25A better fate for PVC2Room-temperature co-upcycling of polyvinyl chloride and polypropylene50One-pot synthesis of waste poly (vinyl-chloride) derived carbon dots for antimicrobial applications6Photothermal Upcycling of Waste Polyvinyl Chloride Plastics27Two-step conversion of waste plastic into light olefins and aromatics on metal-free carbon felt catalyst under radiofrequency heating11Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Chemical transformation of polyurethane into valuable polymers26Microwave‐Powered Liquid Metal Degradation of Polyolefins30Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Hydrothermal dechlorination of polyvinyl chloride for solid fuel: A heterogeneous model based on in situ sampling and cross-section characterization6Hydroxyl Spillover in Fe–Se Dual-Site Catalysts for Mixed Plastics Assay28A hindered-urea vitrimer: recyclable for circular use and upcyclable for rechargeable batteries12Co-upcycling of mixed polypropylene and polyesters5Co-upcycling of polyvinyl chloride/cotton mixed waste into 5-isopropoxymethylfurfural3Dechlorination strategies for chemical recycling of polyvinyl chloride-containing plastic wastes0Highly adaptable oxidative upcycling of polyolefins to multifunctional chemicals containing oxygen and nitrogen9Tuning solvent strength can fractionate PVC into ultra-low molecular weight material with low dispersity6Understanding the competition between hydrodechlorination and Friedel–Crafts alkylation in PVC dechlorination with silylium ions7Upcycling for Sustainable Manufacturing: Insights and New Methods1Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Enzymatic degrading chlorophenol wastewater by mixed strains of immobilized white rot fungi8Boosting the optimization strategy for the waste plastics pyrolysis engineering application: A machine learning multi-dimensional evaluation framework9Recycling homocarbon backbone polymers toward a circular materials economy12Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides26Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Relay Catalysis Enabling the Value‐Added Upgrading of Plastic Wastes2Recyclability of Plastics from Waste Mobile Phones According to European Union Regulations REACH and RoHS4Co-recycling of plastics and other waste materials70Synthesis of New Functionalized Polymers Through the Post‐Modification of Polyvinyl Chloride1Facile visible-light upcycling of diverse waste plastics using a single organocatalyst with minimal loadings42Synergistic Catalysis for Recycling and Upcycling of Plastics35Atmospheric, continuous degradation of poly(ethylene terephthalate) waste by ZnO23Chemical Feedstock Recovery Through Plastic Pyrolysis: Challenges and Perspectives Toward a Circular Economy13In-line NMR guided orthogonal transformation of real-life plastics63Chemical recycling of polyvinyl chloride: Recent progress in pretreatment dechlorination and chlorine recycling19Advances in Chlorinated Polyethylene: Properties, Applications, and Future Directions10Influence of Metal Compounds on Structural and Electrochemical Characteristics of Chars from PVC Pyrolysis1Synthesis and Properties of Poly(vinyl chloride)-b-polyethylene Multiblock Copolymers through the Hydrodechlorination of PVC with Silylium Ions14Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts3The role of polyvinyl chloride in achieving circularity in the built environment: A comprehensive review9Integrated low-temperature PVC and polyolefin upgrading38Comprehensive overview of key principles, innovative techniques, and environmental implications of plastic chemical recycling6Catalytic Upcycling of PET: From Waste to Chemicals and Degradable Polymers48Dual interface strategies using carbon dots for fabricating thermally conductive polymers by pyrrhotite and waste plastics1Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Catalytic cascade depolymerization for sustainable recycling of waste polyvinyl chloride28Removal of impurities in the entrained flow gasification of plastic waste pyrolysis oil2Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Plastic waste recycling: an overview of the mechanical, chemical, and thermal technologies18Breaking the yield–selectivity trade-off in polystyrene waste valorization via tandem depolymerization and hydrogenolysis18Electrocatalytic dechlorination of polyvinylidene chloride for tandem dual radical-driven synthesis of β-chloroalcohols0Energy-efficient and sustainable bromine recovery from e-waste via microdroplet-enhanced spray pyrolysis0Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Pulse‐Constructed Cu δ+ /CuO x Reduces the C─Cl Dipole Moment to Enable Complete Deuterodechlorination of Trichloroacetic Acid0Pulse‐Constructed Cu δ+ /CuO x Reduces the C─Cl Dipole Moment to Enable Complete Deuterodechlorination of Trichloroacetic Acid2Bridging solar harvesting technologies using hydrogels towards sustainability2Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals0Dechlorination of poly(vinyl chloride): thermal benchmarks and complementary non-thermal pathways toward sustainable recycling1Electrochemical depolymerization of polycarbonates under catalyst-free conditions0Influence of chlorine impurities on chemical recycling of plastic waste and adsorptive dechlorination0Manipulating electronic and geometric effects of Pt nanoparticles exerted from Co single atoms in the selective hydrogenation of epichlorohydrin1Visible-light-induced upcycling of perchloroethylene into trichloroacetamides using chlorine dioxide1Mechanochemical upcycling of poly (vinyl chloride) for alcohol halogenation6Techno-Economic and Life Cycle Assessment of Chemical Recycling and Upcycling of Mixed Plastics Waste Containing Poly-vinyl-chloride7A sustainable cascade catalysis strategy for PVC recycling under mild conditions0Chemical Upcycling of Waste Chlorinated Plastics into α,ω-Dienes via Consecutive Dehydrochlorination-Hydrogenation with HCl Trapping and Metathesis1Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Study on phased strategies for sustainable aviation fuel (SAF) industrialization based on a tripartite evolutionary game3Boosting production of hydrogen from polyvinyl chloride degradation at room temperature1Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Dynamic Covalent Chemistry: A Boon for Closed-Loop Recycling of Polymer Networks5Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Influence of polyvinyl chloride contaminant on chemical recycling of polyethylene via thermal and catalytic pyrolysis0Dual engineering of thermodynamics and kinetics in covalent organic frameworks for separation9Electrochemically mediated disproportionation for selective formaldehyde upcycling in acid2Recent polymer modification strategies for reducing plastic waste and enhancing recyclability1Advances in photocatalytic plastics reforming for concurrent hydrogen evolution and selective upgrading0Electrification opportunities and challenges in solid waste utilization0Ozonolysis as a Pathway for the Depolymerization and Chemical Recycling of Polyvinyl Chloride0Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Reprogramming hydrogen-bonding networks at the solvent–polymer interface for mixed polyester waste depolymerization with high selectivity0Effect of chlorine impurities on chemical recycling of plastic waste and dechlorination kinetics1Bifunctional nanocatalyst design for polyolefin hydrocracking2Network analyses reveal geographically continuous elemental patterns in municipal solid waste incineration fly ash0Synergistic Co-Conversion of PVC/Cotton Textile to Phthalic Acid and Sorbitol over a Ru/TiO2 Catalyst0Upcycling of polyvinyl chloride into polyalphaolefin lubricants0Coke poisoning of Lewis acidic Al sites during hydrodechlorination of plastic pyrolysis oil and its mitigation by two-step hydrotreating0Hydrodeoxygenation of Mixed Plastic Wastes Towards Aviation Fuels over Ni−Re Alloy Catalyst0Lubricant Base Oils From Polyethylene via Pyrolysis and Catalytic Upgrading0Catalytic Upcycling of Waste Polyethylene Terephthalate: Recent Advances in Catalyst Design, Reaction Pathway Control, and High-Value Conversion0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Enhanced Catalytic Dechlorination of Polyvinyl Chloride (PVC) and H2 Production Enabled by Synergistic Gaδ+/Ga0 Active Sites in Liquid Metal Particles0Spatially orthogonal CeOx-Zn sites on diatomite-aerogel-derived hierarchical HZSM-5 enable gated dechlorination and BTX-selective upcycling of PVC/PET mixed plastics0Emerging Approaches for Dechlorination of Plastic Waste Prior to Thermochemical Recycling: A Comprehensive Review0Copolymer microstructure evolution in hydrodechlorination of PVC: A triad kinetics model for sequence modification0Detoxification of Chlorinated Dioxins and Furans in Soils via One-Step, Self-Sustaining Smoldering0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  49. Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation

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  50. Hydrothermal dechlorination of polyvinyl chloride for solid fuel: A heterogeneous model based on in situ sampling and cross-section characterization

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