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RESEARCH PAPER · Nature Communications · 2022

Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts

Pavel A. Kots, Tianjun Xie, Brandon C. Vance, Caitlin M. Quinn, Matheus Dorneles de Mello, J. Anibal Boscoboinik, Cong Wang, Pawan Kumar, Eric A. Stach, Nebojša Marinković, Lu Ma, Steven N. Ehrlich, Dionisios G. Vlachos

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Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalystsOriginalHydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Revealing opposite behaviors of catalyst for VOCs Oxidation: Modulating electronic structure of Pt nanoparticles by Mn doping50Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47A two-stage strategy for upcycling chlorine-contaminated plastic waste141Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Constructing ultrafine Pt nanoparticles anchored on N-doped porous carbon nanofibers for efficient and stable oxygen reduction reaction10SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Effect of Hydrogen Spillover on the Ru/TiO2-Catalyzed Guaiacol Hydrodeoxygenation: Rutile vs Anatase TiO2100Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Precise activation of C–C bonds for recycling and upcycling of plastics81Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters21Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Kinetics and reaction mechanism of Pd-Catalyzed chlorobenzene hydrogenolysis5Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Research Progress in Fuel Oil Production by Catalytic Pyrolysis Technologies of Waste Plastics29Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Boosting electrocatalytic activity of Ru for hydrogen evolution through engineering Ru on multiple interfaces of 1T-MoS2 and carbon29Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Effect of reaction media on hydrogenolysis of polyethylene plastic waste: Polymer-surface interactions in small alkane/polymer blends35Predicting hydrogenolysis reaction barriers of large hydrocarbons on metal surfaces using machine learning: Implications for polymer deconstruction15Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Catalytic chemical recycling and upcycling of polyolefin plastics27Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Modulating electronic structure and exposed surface area of Cu-based catalysts by Pd doping for enhanced CO2 hydrogenation to methanol13Copolymerization of Olefins and Conjugated Dienes: A Promising Approach to Produce Recyclable Polyolefins14Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Effect of CeO2 morphology and Ru impregnation method on CH4 selectivity reduction in polyethylene waste conversion to liquid fuels and lubricants15Engineering nanoparticle structure at synergistic Ru-Na interface for integrated CO2 capture and hydrogenation16Towards circularity of plastics: A materials informatics perspective15Ru/TiO2 Catalyzed High‐Yield Synthesis of Furanic Diols by 5‐Hydroxymethylfurfural Hydrogenation with Switchable Selectivity11Plasmonic Copper‐Ruthenium Superstructure for Efficient Photothermal Conversion and Plastic Recycling39Sulfate residuals on Ru catalysts switch CO2 reduction from methanation to reverse water-gas shift reaction46Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Intensification & Scale-up of Waste Plastic Upcycling to Lubricants Conversion0Low temperature polyolefin deconstruction via tandem cracking-hydrogenation2Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Local Electric Field Modulation of Surface Vacancies Enhances CO2 Methanation in Pure Water18La2O2CO3-Supported Ni Nanoparticles with Enhanced Metal–Support Interactions for Selective Hydrogenation9Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Boosting Metal‐Support Interactions Between Ni and MoOx for the Hydrodeoxygenation of Lipids to Alkanes3Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Strong Metal Support Interaction in Ru/V 2 O 3 Mitigates Reactant Induced Poisoning in Succinic Acid Hydrogenation7Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Catalytic Strategies for the Production of Alkane‐Based Lubricant Base Oils from Biomass and Plastic Wastes11Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Synergistic Catalysis for Recycling and Upcycling of Plastics35Construction of PtFe/FeOx-Al2O3 interface via regulating the metal – support interactions for selective hydrogenation of cinnamaldehyde14Coordinating cracking and hydrogenation of polyethylene waste via acid-metal site isolation for selective hydrocarbon production10Carbon quantum dots (CQDs)-supported CeO2/Al2O3 with tunable band gap for the efficient degradation of plastic waste into porous carbon materials under mild conditions: experiment and DFT3Oxidation of n-alkanes using TS-1 and H2O2: Effects of chain length and solvents2Selective Upcycling of Aromatic Polymer Waste into Light C6C9 Aromatics Over Ru‐Supported Catalysts6Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16In-line NMR guided orthogonal transformation of real-life plastics63Synergistic regulation of oxygen vacancy and Lewis acid sites by Ru loading in LaMnOx catalysts for boosting 2-butanol production from levulinic acid and levulinates4Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Tuning Catalytic Reactivity via Wetting Control through Oxygen Vacancies: Ru Clusters on Anatase TiO2 and CeO2 Supports22Integrated low-temperature PVC and polyolefin upgrading38The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Dual-control strategy for selective upgrading of polyethylene waste into jet fuel-range alkanes2Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17TiO 2 ‐Supported Ru–Fe Catalysts for the Hydrodeoxygenation of Bis(2‐hydroxyethyl) Terephthalate (BHET) Prepared by the Glycolysis of Polyethylene Terephthalate (PET)1Phase‐Guided Assembly of RuO 2 Epitaxial Films on TiO 2 Nanofibers: Interfacial Coherence Outperforming Defect‐Driven Mismatch for Active Site Generation in Li–O 2 Batteries6Selective hydrocracking of polystyrene waste over Pt- and Ru-supported zeolite catalysts into high yield LPG and ethylbenzene4Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Boosting activity of heterogeneous Ru catalysts via solid-phase infiltration and syngas-mediated redispersion2A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Carbon–carbon bond cleavage for lignin and plastics deconstruction0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Efficient depolymerization of polystyrene waste into styrene monomers over the microwave-assisted Zn/b-ZnO catalyst system1Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Electron Traps in Thermal Heterogeneous Catalysis: Fundamentals, Detection, and Applications of CO2 Hydrogenation1Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Mesoporous silica as a tunable support for dual-function Ba–Ru catalysts: impact on CO2 adsorption and methanation performance3Unveiling selectivity shift in CO2 methanation with TiO2 supported subnanometer Ru particles1Regulation Mechanism of Entropy–Enthalpy Compensation Effect on Charge Trap Energy Levels in Hydrogen-Bonded PP- g -MA/PVDF Composites2Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems0Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Synergy of Ru and NiAl-LDH for efficient selective hydrogenation of phenolic compounds under visible light0Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Protective Spillover-Hydrogenation Catalyst Based on Pd-Loaded Metal–Organic Frameworks4Photothermal Dehydrogenation of Waste Plastics Using Ni@p-SiO2/Au Catalyst for Hydrogen Production0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Ambient-pressure conversion of plastic waste to jet fuel cycloalkanes by tandem hydropyrolysis and vapour-phase hydrogenation2From waste to wealth: Advanced strategies and mechanisms for chemical recycling and upcycling of polymeric materials1Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Design and analysis of a new Ru-Cu/ZSM-5 bimetallic catalyst for hydrogenolysis of polyolefin waste0Confined Isomerization Enables Solar-Thermal Upcycling of Polyolefins into High-Octane Gasoline0Ambient Hydrogenolysis of α-O-4 Lignin Model Compounds over Perovskite-Supported Pd Catalysts0Low-loading Ru catalysts supported on N-doped TiO2 for efficient hydrogenation of phenolic feedstocks to cyclohexanol derivatives0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0Efficient and Selective Low-Temperature Polypropylene Hydrogenolysis Using Zr-Doped Mixed Metal Oxides Catalysts0

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  10. Effect of Hydrogen Spillover on the Ru/TiO2-Catalyzed Guaiacol Hydrodeoxygenation: Rutile vs Anatase TiO2

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  47. Engineering nanoparticle structure at synergistic Ru-Na interface for integrated CO2 capture and hydrogenation

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  48. Towards circularity of plastics: A materials informatics perspective

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