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RESEARCH PAPER · Applied Catalysis B: Environmental · 2023

SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

Weilin Tu, Mingyu Chu, Xianpeng Wang, Xuchun Wang, Yifan Li, Wenxiu Yang, Muhan Cao, Lu Wang, Youyong Li, Tsun‐Kong Sham, Yi Cui, Qiao Zhang, Jinxing Chen

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SMSI-induced charge transfer for selective hydrogenolysis of polyolefinsOriginalPrecise activation of C–C bonds for recycling and upcycling of plastics81Catalytic dehydrogenation for hydrogen production controlled by metal-supported heterogeneous catalysts20Construction of Highly Active Pd–Ti 3+ Sites in Defective Pd/TiO 2 Catalysts for Efficient Hydrogenation of Styrene–Butadiene–Styrene78Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Promoting Catalytic Performance Involving Hydrogen Spillover by Ion Exchange of Pt@A Catalysts to Regulate Reactant Adsorption3From Charge to Spin: An In‐Depth Exploration of Electron Transfer in Energy Electrocatalysis180Unique role of silica in MOF-Derived High-Loading Palladium-on-Ceria single atom catalysts with excellent efficiency and durability9Insights into support effects of Ag/SiO2 catalysts for dimethyl glycolate semi-hydrogenation to methyl glycolate8Silica-modified Pt/TiO2 catalysts with tunable suppression of strong metal–support interaction for cinnamaldehyde hydrogenation10Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Non-Photochemical Origin of Selectivity Difference between Light and Dark Catalytic Conditions2Modulation of metal–support interactions in Pt–TiOx synergistic catalysts for propane dehydrogenation16Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Hydroconversion of waste polyethylene plastics under mild conditions using mechanically mixed bifunctional catalysts: Impact of metal-acid balance and proximity9Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Overturning CO2 Hydrogenation Selectivity from CH4 to CO by Strong Ru–FeOx Interaction Arising from a Multilayer Epitaxial Structure9A fluorinated COF-encapsulated CeO 2 @Pt sandwich catalyst enables dual interfacial-electronic modulation for liquid-phase hydrogenation2Activity enhancement of Ru/TiO 2 catalysts for catalytic hydrogenation of amides to amines through controlling strong metal–support interactions6Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Hydrogen/solvent-free plastic valorization via loosely coordinated ruthenium sites steering selective aromatization7Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Optimizing the Electronic Structure of IrOx Sub-2 nm Clusters via Tunable Metal Support Interaction for Acidic Oxygen Evolution Reaction42Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Recent Progress in the Design and Application of Strong Metal–Support Interactions in Electrocatalysis37Promoted synergistic interactions between Ce and Ni in hierarchical porous Ce-UiO-66 supported Ni NPs for dicyclopentadiene hydrogenation to tetrahydrodicyclopentadiene6Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Synergistic Catalysis for Recycling and Upcycling of Plastics35Interfacial engineering electron-rich Cuδ−-Ov-Zn oxygen vacancy via Mn Cu alloy in LDH structure for selective CO2 conversion to methanol13Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Strong metal-support interaction effect enhances kinetic synergy factors between photocatalysis and peroxymonosulfate activation for ultrafast pollutant removal5Selective cleavage of C-H and C-C bonds of ethane by tuning the CoO -ZrO2 interaction: The surface construction of Co-O-Zr site and Co3O40Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Upcycling Polyethylene into Separable Aromatics Through Tandem Catalysis with CO2 at Atmospheric Pressure2Reducibility of Unsupported and Al 2 O 3 -Supported RuO 2 Catalysts: When Ru Oxide Challenges Ru Metal in Hydrogenation5Regulating the TiO x -Pt Interaction over Pt/TiN Catalyst for the Hydrodeoxygenation of m -cresol2Carbon–carbon bond cleavage for lignin and plastics deconstruction0Efficient photocatalytic conversion of air into nitrate over 2D ultrathin WO3 promoted by Ru nanoclusters and oxygen vacancies synergistically0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Theoretical insights into encapsulation-induced CO 2 reduction selectivity reversal on Ru supported on TiO x catalysts0Nanoconfined Photothermal Catalysis: Mechanisms, Engineering Strategies, and Solar Fuel Synthesis28Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Integration of plasmonic 2D Pt/TiO2 and spectrally-selective continuous gas-lift reactor for high-efficiency photothermal rWGS0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Laser-Engineered Defective Carbon-Supported Ni Catalyst Boosts Dry Reforming of Methane3Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling0Oligomerization and co-oligomerization of waste polypropylene cracking products to sustainable aviation fuel components0Enhanced hydrogen-rich syngas production from steam gasification of woody biomass using fly-ash supported Ni bifunctional catalysts6Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1Machine learning induced tandem catalysis for high-value recovery of polyolefins: pathways, mechanisms and products0Tuning the Metal/Oxide Ratio in Inverse Ni–Al 2 O 3 Catalysts for Selective Cleavage of β‐O‐4 Linkage in Lignin Model Compounds0Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Atomically dispersed cerium enabling mild polyolefin hydrocracking to simple gas streams0Unraveling the effects of pore structure on the performance of Ru/SiO2 catalysts for the selective hydrogenation of dimethyl terephthalate to dimethyl 1,4-cyclohexanedicarboxylate0Highly active and selective heterogeneous Ru/La2O3-CeO2 catalyst for hydrogenolysis of LDPE to valuable chemicals0

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