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RESEARCH PAPER · Angewandte Chemie International Edition · 2023

Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles

Shibashish D. Jaydev, Antonio José Martín, Marc‐Eduard Usteri, Katia Chikri, Henrik Eliasson, Rolf Erni, Javier Pérez‐Ramírez

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Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium NanoparticlesOriginalHierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst27Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst6Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Two-step conversion of waste plastic into light olefins and aromatics on metal-free carbon felt catalyst under radiofrequency heating11Induction Heating for the Electrification of Catalytic Processes51Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0From rags to riches: the role of the chemical sciences in transforming waste into valuable products0Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Selective Upcycling of Aromatic Polymer Waste into Light C6C9 Aromatics Over Ru‐Supported Catalysts6Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Efficient chemical recycling of mixed plastics by intramolecular glycolysis13Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Advancing chemical recycling for waste plastic conversion1Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene0Green and Sustainable Chemistry for a Circular Economy2Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst0Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Breaking the Yield‐Selectivity Trade‐Off in Polypropylene Upcycling via Ternary‐Active ZnAlO Nanocomposites0

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  1. Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels

    ACS Sustainable Chemistry & Engineering · 2024-04-03

    Xinru Zhou, Xinlei Han, Zhengyan Qu, Jiuxuan Zhang, Feng Zeng, Zhenchen Tang, Rizhi Chen

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  2. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

    JACS Au · 2024-06-04

    Simin Sun, Wenyu Huang

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  3. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

    Chem Catalysis · 2024-08-20

    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  4. Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling

    Nature Chemical Engineering · 2024-08-28

    Shibashish D. Jaydev, Antonio José Martín, David Garcia, Katia Chikri, Javier Pérez‐Ramírez

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  5. Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst

    Angewandte Chemie International Edition · 2024-11-13

    Wanying Han, Longfei Lin, Longfei Lin, Ziyu Cen, Yubin Ke, Qian Xu, Junfa Zhu, Xuelei Mei, Zhanghui Xia, Xinrui Zheng, Yaqin Wang, Yani Liu, Mingyuan He, Haihong Wu, Haihong Wu, Buxing Han

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  6. Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst

    Angewandte Chemie · 2024-11-13

    Wanying Han, Longfei Lin, Ziyu Cen, Yubin Ke, Qian Xu, Junfa Zhu, Xuelei Mei, Zhanghui Xia, Xinrui Zheng, Yaqin Wang, Yani Liu, Mingyuan He, Haihong Wu, Buxing Han

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  7. Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts

    ACS Sustainable Chemistry & Engineering · 2024-11-20

    Yan Mei, Jiuxuan Zhang, Zhengyan Qu, Feng Zeng, Hong Li Jiang, Zhenchen Tang, Weihong Xing, Rizhi Chen

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  8. Two-step conversion of waste plastic into light olefins and aromatics on metal-free carbon felt catalyst under radiofrequency heating

    Chemical Engineering Journal · 2024-11-29

    Cuong Duong‐Viet, Lai Truong‐Phuoc, Jean‐Mario Nhut, Lam Nguyen‐Dinh, Christophe Michon, Cuong Pham‐Huu, Cuong Pham‐Huu

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  9. Induction Heating for the Electrification of Catalytic Processes

    ChemSusChem · 2024-12-23

    Lai Truong‐Phuoc, Cuong Duong‐Viet, Jean‐Mario Nhut, Anastasia Pappa, Spyridon Zafeiratos, Cuong Pham‐Huu, Cuong Pham‐Huu

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  10. Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques

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    Acácio S. de Souza, Patrícia Garcia Ferreira, Iva Souza de Jesus, Rafael Portugal Rizzo Franco de Oliveira, Alcione Silva de Carvalho, Débora Omena Futuro, Vı́tor F. Ferreira

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  11. Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking

    Catalysis Science & Technology · 2025-01-01

    Ruoyan Bai, Juhong Nie, Roudan Lian, Jian Zhang, Maolin Zhang

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  12. From rags to riches: the role of the chemical sciences in transforming waste into valuable products

    RSC Sustainability · 2025-01-01

    Frank Butler

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  13. Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering

    Green Chemistry · 2025-01-01

    Parsa Pishva, Jinyao Tang, Yanlin Zhu, Jochen A. Lauterbach, Zhenmeng Peng

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  14. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  15. Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

    Angewandte Chemie International Edition · 2025-01-22

    Junsung Lee, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  16. Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports

    Industrial & Engineering Chemistry Research · 2025-03-12

    Fawaz Motolani, Rebekah J. Snellings, Sogand Aghamohammadi, Hee Jeung Oh, Gina A. Noh, Bert D. Chandler, Bryan D. Vogt

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  17. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  18. Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets

    Small · 2025-03-31

    Baogang Su, Mengjun Wang, Xiaofei Lai, Yong Xu

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  19. Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions

    JACS Au · 2025-04-16

    Sung Min Kim, Boda Yang, Oliver Y. Gutiérrez, Wei Zhang, Carlos Lizandara‐Pueyo, Piyush Ingale, Ivana Jevtovikj, Reni Grauke, János Szanyi, Huamin Wang, Stephan A. Schunk, Johannes A. Lercher

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  20. Selective Upcycling of Aromatic Polymer Waste into Light C6C9 Aromatics Over Ru‐Supported Catalysts

    ChemSusChem · 2025-06-02

    Arjun K. Manal, Jun Liang Zhao, Rajaram Bal, Rajendra Srivastava

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  21. Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent

    Journal of the Energy Institute · 2025-06-18

    Haifeng Xu, Cong Dong, Bingyan Sun, Kaige Wang, Bo Wang, Guanqun Luo

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  22. Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds

    Nature Chemistry · 2025-09-02

    Qingheng Lai, Xinrui Zhang, Shan Hao Jiang, Matthew D. Krzyaniak, Selim Alayoǧlu, Amol Agarwal, Yukun Liu, Wilson C. Edenfield, Takeshi Kobayashi, Yuyang Wang, Vinayak P. Dravid, Michael R. Wasielewski, Jeffrey T. Miller, Yosi Kratish, Tobin Jay Marks

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  23. Efficient chemical recycling of mixed plastics by intramolecular glycolysis

    AIChE Journal · 2025-09-03

    Yanfen Wu, Xin Zi Tang, Shuairen Qian, Helai Huang, Yizhen Che, Qikun Hu, Mingze Sun, Yi Lung Cheng, Zhiqiang Niu

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  24. Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst

    Journal of Catalysis · 2025-09-11

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  25. Advancing chemical recycling for waste plastic conversion

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  26. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

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  27. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

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  28. Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics

    Nature Communications · 2025-11-10

    Iris Nogueroles-Langa, Yuzhen Ge, Cecilia Salah, Shibashish D. Jaydev, Jordi Morales‐Vidal, Pol Sanz Berman, Henrik Eliasson, Rolf Erni, Gonzalo Guillén‐Gosálbez, Núria López, Antonio José Martín, Javier Pérez‐Ramírez

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  29. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025-12-10

    Fan Yuan, Hongshun Ran, Tingxi Chen, Yaxuan Jing

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  30. A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis

    Green Chemistry · 2025-12-26

    Chuanya Li, Qianfeng Zhou, Changhu Leng, Yongchao Wang, Chenyang Ma, Junlei Zhang, Zhijun Li

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  31. Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts

    Green Chemistry · 2026-01-01

    Junho Suh, Hyeongdong Jung, Junho Yoon, Jae‐Soon Choi, Jungup Bang, Do Heui Kim

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  32. Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization

    Advanced Science · 2026-02-03

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  33. Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene

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  34. Green and Sustainable Chemistry for a Circular Economy

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  35. Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2026-05-01

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  36. Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products

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  37. A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis

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  38. Breaking the Yield‐Selectivity Trade‐Off in Polypropylene Upcycling via Ternary‐Active ZnAlO Nanocomposites

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