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RESEARCH PAPER · ACS Catalysis · 2024

Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

Jessie A. Sun, Pavel A. Kots, Zachary R. Hinton, Nebojša Marinković, Lu Ma, Steven N. Ehrlich, Weiqing Zheng, Thomas H. III Epps, LaShanda T. J. Korley, Dionisios G. Vlachos

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Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product MicrostructureOriginalSynergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Sustainable recycling and upgrading of waste polytetrafluoroethylene: Current progress and prospect12Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation5Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Scalable upcycling of medical plastic waste using metals-doped hierarchically porous biocarbon for tunable fuel-grade hydrocarbons or H2-enriched fuel gas3Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling4Autonomous closed-loop optimization of n -butane hydrogenolysis: a case study for history-dependent heterogeneous catalytic reactions0Plastic Waste Conversion into Monomers Using Microwaves0Vapor-phase pillarization of MXenes for engineering hierarchical interlayer porosity1Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Depolymerization of Nylon-6 over a Supported Ruthenium Catalyst to ε-Caprolactam1Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst0Ambient-pressure conversion of plastic waste to jet fuel cycloalkanes by tandem hydropyrolysis and vapour-phase hydrogenation2Sustainable production of aviation fuel cycloalkanes from plastic waste under ambient-pressure conditions1Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Photocatalytic materials and strategies for plastic degradation and upcycling0

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  1. Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production

    Chemical Communications · 2024-01-01

    Arjun K. Manal, Atal Shivhare, Sharad V. Lande, Rajendra Srivastava

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  2. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

    JACS Au · 2024-06-04

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  3. Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation

    Frontiers of Chemical Science and Engineering · 2024-06-24

    Xiangkun Zhang, Bingyan Sun, Zhigang Zhao, Tan Li, Marc Mate, Kaige Wang

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  4. Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review

    Langmuir · 2024-08-07

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  5. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

    Chem Catalysis · 2024-08-20

    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  6. Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts

    ACS Sustainable Chemistry & Engineering · 2024-11-20

    Yan Mei, Jiuxuan Zhang, Zhengyan Qu, Feng Zeng, Hong Li Jiang, Zhenchen Tang, Weihong Xing, Rizhi Chen

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  7. Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling

    Nature Communications · 2024-11-29

    Taeeun Kwon, Byeongchan Ahn, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  8. Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems

    Chemical Engineering Journal Advances · 2024-12-28

    Zhuoming Feng, Siwon Lee, Raymond J. Gorte, John M. Vohs

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  9. Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites

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    Taeeun Kwon, J. S. PARK, Ki Hyuk Kang, Dae-Sung Jung, Wangyun Won, Insoo Ro

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  10. Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts

    EES Catalysis · 2025-01-01

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  11. Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts

    Green Chemistry · 2025-01-01

    Jessie A. Sun, Esun Selvam, Alexander Bregvadze, Weiqing Zheng, Dionisios G. Vlachos

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  12. Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts

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    Xiyan Huang, Weixin Meng, Diego A. Acevedo–Guzmán, Hongqi Wang, Balaji Sridharan, Petra Rudolf, Hero Jan Heeres, Jingxiu Xie

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  13. Sustainable recycling and upgrading of waste polytetrafluoroethylene: Current progress and prospect

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  14. Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation

    Journal of environmental chemical engineering · 2025-02-05

    Guanqun Luo, Xiangkun Zhang, Linjia Yin, Hong Xian, Kaige Wang

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  15. Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites

    Catalysts · 2025-03-31

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  16. Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications

    Journal of Catalysis · 2025-05-08

    Andy Simonson, Lydia Thies, David D. Hibbitts

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  17. Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent

    Journal of the Energy Institute · 2025-06-18

    Haifeng Xu, Cong Dong, Bingyan Sun, Kaige Wang, Bo Wang, Guanqun Luo

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  18. Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing

    Chem Catalysis · 2025-07-16

    Ali Kamali, Joshua M. Little, Song Luo, Amy Y. Chen, Akash Warty, Antara Bhowmick, Jorge Moncada, Evan P. Jahrman, Brandon C. Vance, Jong Kahk Keum, Taylor J. Woehl, Po‐Yen Chen, Dionisios G. Vlachos, Dongxia Liu

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  19. Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes

    Journal of the American Chemical Society · 2025-08-14

    Jiayang Zhao, Qikun Hu, Yuqi Wang, Yizhen Che, Zhiqiang Niu

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  20. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

    ACS Catalysis · 2025-09-23

    Zachary M. Gdowski, Rishi Raj, Aditya Bhan, K. Andre Mkhoyan, Mahesh K. Mahanthappa, Frank S. Bates

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  21. Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst

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    Jing Dai, Ziqi Fang, Huayue Yang, Zhengjian Li, Mingzhi Wang, Shuying Tian, Shumin Liu, Yanyan Jia, Mingshu Chen, Yun Zhao, Guangxu Chen

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  22. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

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    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  23. Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics

    Nature Communications · 2025-11-10

    Iris Nogueroles-Langa, Yuzhen Ge, Cecilia Salah, Shibashish D. Jaydev, Jordi Morales‐Vidal, Pol Sanz Berman, Henrik Eliasson, Rolf Erni, Gonzalo Guillén‐Gosálbez, Núria López, Antonio José Martín, Javier Pérez‐Ramírez

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  24. Scalable upcycling of medical plastic waste using metals-doped hierarchically porous biocarbon for tunable fuel-grade hydrocarbons or H2-enriched fuel gas

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  25. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

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  26. Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling

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  27. Autonomous closed-loop optimization of n -butane hydrogenolysis: a case study for history-dependent heterogeneous catalytic reactions

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  28. Plastic Waste Conversion into Monomers Using Microwaves

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  30. Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion

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  31. Depolymerization of Nylon-6 over a Supported Ruthenium Catalyst to ε-Caprolactam

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  32. Oxygen vacancy promoted C–H activation enhancing hydrogenolysis of polyethylene plastics over Ru/CeO2 catalyst

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  33. Ambient-pressure conversion of plastic waste to jet fuel cycloalkanes by tandem hydropyrolysis and vapour-phase hydrogenation

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  34. Sustainable production of aviation fuel cycloalkanes from plastic waste under ambient-pressure conditions

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  36. Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products

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  37. A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis

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