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RESEARCH PAPER · Applied Catalysis B: Environmental · 2023

Upcycling of polyvinyl chloride to hydrocarbon waxes via dechlorination and catalytic hydrogenation

Scott Svadlenak, Sophie Wojcik, Oluwafemi Ogunlalu, Makayla Vu, Maoz Dor, Bryan W. Boudouris, D. Wildenschild, Konstantinos A. Goulas

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Upcycling of polyvinyl chloride to hydrocarbon waxes via dechlorination and catalytic hydrogenationOriginalPrecise activation of C–C bonds for recycling and upcycling of plastics81Conversion of diverse post-consumer PVC waste materials to PE via dual catalytic tandem dehydrochlorination–hydrogenation14Conversion of waste poly(vinyl chloride) to branched polyethylene mediated by silylium ions29Revisiting poly(vinyl chloride) reactivity in the context of chemical recycling46Poly(vinyl chloride) Dechlorination Catalyzed by Zirconium10Chlorinated plastics offer unique opportunities and challenges in upcycling25A virtuous cycle for thermal treatment of polyvinyl chloride and fermentation of lignocellulosic biomass7Catalytic Dechlorination of Three Organochlorides by Recyclable Nano-Palladium-Engineered Natural Sponge with Formic Acid16Low-temperature dechlorination of polyvinyl chloride (PVC) for production of H 2 and carbon materials using liquid metal catalysts35Upvaluing chlorinated plastic wastes18Catalytic Upcycling of Polyolefins316Metal‐Catalyzed Polymer Dehydrochlorination and Hydrodefluorination1An integrated off-lattice kinetic Monte Carlo (KMC)-molecular dynamics (MD) framework for modeling polyvinyl chloride dehydrochlorination8Room-temperature co-upcycling of polyvinyl chloride and polypropylene50Beyond the Landfill: A critical review of techniques for End-of-Life Polyvinyl chloride (PVC) valorization37Hydrothermal dechlorination of polyvinyl chloride for solid fuel: A heterogeneous model based on in situ sampling and cross-section characterization6From Waste to Worth: Upcycling Plastic into High-Value Carbon-Based Nanomaterials42Dechlorination strategies for chemical recycling of polyvinyl chloride-containing plastic wastes0Layer-by-layer techniques incorporating upcycled TPEE: from waste to conductive, multi-responsive, self-healable, and highly-stretchable electronics5Enhancing Rate and Selectivity for Hydrodechlorination of Poly(Vinyl Chloride) with Rh Catalysts9Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides26Upcycling of Waste Plastics into Value-Added Chemicals6Relay Catalysis Enabling the Value‐Added Upgrading of Plastic Wastes2Synergistic co-pyrolysis of polyvinyl chloride and corn stalk for improved products and dechlorination behavior9Composite solid-state electrolyte from waste modacrylic fibers with multiple Li+ transport channels and enhanced interfacial stability for lithium metal batteries4Practically simple, catalyst-free, and scalable approach for all-component upcycling of mixed PVC/PA plastics2Synthesis and Properties of Poly(vinyl chloride)-b-polyethylene Multiblock Copolymers through the Hydrodechlorination of PVC with Silylium Ions14Integrated low-temperature PVC and polyolefin upgrading38Upcycling Waste Polyvinyl Chloride into Single‐Atom Catalysts for Versatile Electrocatalytic and Hydrogenation Reactions1Recent advances on electrocatalytic hydrodechlorination of chlorinated organic pollutants0Degradation and utilization of polyvinyl chloride (PVC): Challenges and opportunities toward a circular economy24Synergistic Chlorine-Mediated Co-Upcycling of polyvinyl chloride and waste biomass for sustainable furfurals production1Electrochemical Chlorine Shuttle from PVC Waste to Vinyl Ether Acceptors for the Synthesis of Biodegradable Polyester Precursors9Plastic waste recycling: an overview of the mechanical, chemical, and thermal technologies18Mechanism-Guided dechlorination of PVC-Containing resins in subcritical aqueous ammonia1Asymmetrically coordinated Co–N 3 B 1 single-atom catalysts for the selective hydrogenation of halonitrobenzenes0Microwave-assisted recycling of plastic waste into value-added chemicals: challenges, recent advances, and perspectives0Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe12Chemical Upcycling of Waste Chlorinated Plastics into α,ω-Dienes via Consecutive Dehydrochlorination-Hydrogenation with HCl Trapping and Metathesis1Elucidating the role of overlooked environmentally persistent free radicals and reactive chlorine species on photoaged chlorine-containing microplastics: New insights into formation mechanisms and health risks2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Achieving Near‐Complete Dechlorination of Poly(vinyl chloride) via Electrochemical Reduction0Coordination-Engineered Fe Single Atoms Enable Synergistic PVC Upcycling into Fuel-Range Hydrocarbons via Fenton-Like Pathway0Advances in Chemical Upcycling of Plastic Waste: Pathways to High-Value Products for a Sustainable Circular Economy0Enabling Downstream Recycling: Separation and Debromination of Polymeric Brominated Flame Retardants from Polystyrene1Enhanced Catalytic Dechlorination of Polyvinyl Chloride (PVC) and H2 Production Enabled by Synergistic Gaδ+/Ga0 Active Sites in Liquid Metal Particles0Copolymer microstructure evolution in hydrodechlorination of PVC: A triad kinetics model for sequence modification0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Precise activation of C–C bonds for recycling and upcycling of plastics

    Chemical Science · 2023-12-07

    Hongshun Ran, Shuo Zhang, Wenyi Ni, Yaxuan Jing

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  2. Conversion of diverse post-consumer PVC waste materials to PE via dual catalytic tandem dehydrochlorination–hydrogenation

    EES Catalysis · 2024-01-01

    Galahad O’Rourke, Alina A. Skorynina, Igor Beckers, Sam Van Minnebruggen, Christel Colemonts, Philippe Gabriels, Peter Van der Veken, Dirk E De Vos

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  3. Conversion of waste poly(vinyl chloride) to branched polyethylene mediated by silylium ions

    Chemical Science · 2024-01-01

    Zachary A. Wood, Eunice C. Castro, Angelyn N. Nguyen, Megan E. Fieser

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  4. Revisiting poly(vinyl chloride) reactivity in the context of chemical recycling

    Chemical Science · 2024-01-01

    Rahul Kant Jha, Bertrand J. Neyhouse, Morgan Sarah Young, Danielle E. Fagnani, Anne Jennifer McNeil

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  5. Poly(vinyl chloride) Dechlorination Catalyzed by Zirconium

    Chemistry - A European Journal · 2024-02-07

    Adrien T. Normand, Yue Wu, Tiffanie Régnier, Paul Fleurat‐Lessard, Yoann Rousselin, Benjamin Théron, Pierre Le Gendre, Mariolino Carta

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  6. Chlorinated plastics offer unique opportunities and challenges in upcycling

    Polymer International · 2024-02-19

    Ali Al Alshaikh, Jason E. Bara

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  7. A virtuous cycle for thermal treatment of polyvinyl chloride and fermentation of lignocellulosic biomass

    Applied Energy · 2024-03-15

    Jonghyun Park, Jun Ho Yim, Seong-Heon Cho, Sungyup Jung, Yiu Fai Tsang, Wei‐Hsin Chen, Young Jae Jeon, Eilhann E. Kwon

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  8. Catalytic Dechlorination of Three Organochlorides by Recyclable Nano-Palladium-Engineered Natural Sponge with Formic Acid

    Catalysts · 2024-07-03

    Mingyue Liu, Gang Chen, Zhenjun Song, Zhicai He, Aiguo Zhong, Mei Cui

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  9. Low-temperature dechlorination of polyvinyl chloride (PVC) for production of H 2 and carbon materials using liquid metal catalysts

    Science Advances · 2024-07-24

    Felipe Polo‐Garzon, Zili Wu, Yuanyuan Li, Junyan Zhang, Xinbin Yu, Elena Toups, Eddie Lopez Honorato, Joshua T. Damron, Jeffrey C. Foster, Yongqiang Q. Cheng, Luke L. Daemen, Anibal Javier Ramirez-Cuesta, Harry M. Meyer

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  10. Upvaluing chlorinated plastic wastes

    Interdisciplinary materials · 2024-08-14

    Shuyi Zhang, Hao Han, Muhan Cao, Yeping Xie, Jinxing Chen

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  11. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  12. Metal‐Catalyzed Polymer Dehydrochlorination and Hydrodefluorination

    ChemistrySelect · 2024-10-01

    Víctor Varela‐Izquierdo, Sourav Ghosh, Leila Hammoud, Pier‐Francesco Fazzini, Simon Guélen, Philippe Marion, Bruno N. Chaudret

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  13. An integrated off-lattice kinetic Monte Carlo (KMC)-molecular dynamics (MD) framework for modeling polyvinyl chloride dehydrochlorination

    Chemical Engineering Science · 2024-11-14

    Feranmi V. Olowookere, Christoffer Heath Turner

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  14. Room-temperature co-upcycling of polyvinyl chloride and polypropylene

    Nature Sustainability · 2024-11-22

    Zhiwen Gao, Yu Wang, Lei Yuan, Xinrui Shi, Yihao Shang, Jinpeng Jiang, Min Zhang, Shuhui Fang, Wei Zhang, Yue Liu

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  15. Beyond the Landfill: A critical review of techniques for End-of-Life Polyvinyl chloride (PVC) valorization

    Waste Management · 2024-12-09

    Mohammadhossein Havaei, Oğuzhan Akin, Andrea Locaspi, Robin John Varghese, Florent Minette, Eric Romers, Steven De Meester, Kevin M. Van Geem

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  16. Hydrothermal dechlorination of polyvinyl chloride for solid fuel: A heterogeneous model based on in situ sampling and cross-section characterization

    Journal of environmental chemical engineering · 2024-12-24

    Qisong Zhong, Dachao Ma, Mengxue Ling, Lu Ding, Cheng Liao, Hongchang Hu, Jinye Wei, Guozi Liu, Zheng Liu, Dongbo Wang, Qingge Feng

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  17. From Waste to Worth: Upcycling Plastic into High-Value Carbon-Based Nanomaterials

    Polymers · 2024-12-30

    Ahmed M. Abdelfatah, Mohamed Hosny, Ahmed S. Elbay, Nourhan El-Maghrabi, Manal Fawzy

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  18. Dechlorination strategies for chemical recycling of polyvinyl chloride-containing plastic wastes

    Elsevier eBooks · 2025-01-01

    Nan Zhou, Hao Yuan, Mingzhe Li

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  19. Layer-by-layer techniques incorporating upcycled TPEE: from waste to conductive, multi-responsive, self-healable, and highly-stretchable electronics

    Journal of Materials Chemistry A · 2025-01-01

    Chia-Wei Chang, Chun-Ting Chang, Jian‐Hua Ciou, Kai‐Chuan Kuo, Chia-Ti Wu, Lin Ji, Tse‐Yu Lo, Yu Chen, Huan-Wei Lin, Yu‐Hsuan Tseng, Meili Li, Che-Tseng Lin, Jiun‐Tai Chen

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  20. Enhancing Rate and Selectivity for Hydrodechlorination of Poly(Vinyl Chloride) with Rh Catalysts

    ChemSusChem · 2025-02-03

    Nancy G. Bush, Ayon Das, Jessica A. Bowen, Megan E. Fieser

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  21. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  22. Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides

    Journal of the American Chemical Society · 2025-03-21

    Esun Selvam, Zoé O. G. Schyns, Jessie A. Sun, Pavel A. Kots, Yeonsu Kwak, LaShanda T. J. Korley, Raúl F. Lobo, Dionisios G. Vlachos

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  23. Upcycling of Waste Plastics into Value-Added Chemicals

    Science for energy and environment. · 2025-03-26

    Xu Jin, Jing Zhang

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  24. Relay Catalysis Enabling the Value‐Added Upgrading of Plastic Wastes

    ChemCatChem · 2025-03-31

    Kaizhi Wang, Zehui Sun, Ting Yang, Wendi Guo, Feifan Gao, Mugeng Chen, Yongmei Liu, Heyong He, Yong Cao

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  25. Synergistic co-pyrolysis of polyvinyl chloride and corn stalk for improved products and dechlorination behavior

    Journal of Cleaner Production · 2025-04-14

    Yongfu Zeng, Enzheng Hu, Guangwen Xu, Zuohua Liu, Guocan Zheng, Dean Pan, Jianglong Yu, Xin Jia, Moshan Li, Youcai Ma

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  26. Composite solid-state electrolyte from waste modacrylic fibers with multiple Li+ transport channels and enhanced interfacial stability for lithium metal batteries

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  27. Practically simple, catalyst-free, and scalable approach for all-component upcycling of mixed PVC/PA plastics

    Waste Management · 2025-07-07

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  28. Synthesis and Properties of Poly(vinyl chloride)-b-polyethylene Multiblock Copolymers through the Hydrodechlorination of PVC with Silylium Ions

    Journal of the American Chemical Society · 2025-07-15

    Zachary A. Wood, Tyeshia Sapp, Bailey Eberle, Xuchun Wang, Samuel B. Hunt, Sarah J. Barber, Mary Dana Czarinah L. Cheng-Tan, Yunpu Zhao, Frédéric A. Perras, Massimiliano Delferro, Byeongdu Lee, Mark Dadmun, Megan E. Fieser

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  29. Integrated low-temperature PVC and polyolefin upgrading

    Science · 2025-08-14

    Wei Zhang, Boda Yang, Benjamin A. Jackson, Junbo Zhao, Honghong Shi, Donald M. Camaioni, Sung Min Kim, Huamin Wang, János Szanyi, Mal‐Soon Lee, Jingguang G. Chen, Johannes A. Lercher

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  30. Upcycling Waste Polyvinyl Chloride into Single‐Atom Catalysts for Versatile Electrocatalytic and Hydrogenation Reactions

    ChemCatChem · 2025-09-17

    Yuxuan Chen, Hai Feng Zhang, Zifeng Wu, Haofan Wang, Hongjuan Wang, Yonghai Cao, Jialong Zhang, Hao Yu

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  31. Recent advances on electrocatalytic hydrodechlorination of chlorinated organic pollutants

    Surfaces and Interfaces · 2025-10-01

    Xinran Ma, Dandan Li, Song Wu, Guangyin Fan, Yan Long

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  32. Degradation and utilization of polyvinyl chloride (PVC): Challenges and opportunities toward a circular economy

    Green Energy & Environment · 2025-10-28

    Rui Huang, Jiaolong Meng, Xuefeng Jiang

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  33. Synergistic Chlorine-Mediated Co-Upcycling of polyvinyl chloride and waste biomass for sustainable furfurals production

    Chemical Engineering Science · 2025-11-04

    Tingyong Wang, Xiaoxian Hu, Shengkai Huang, Zhixiong Zhuang, Xiaohua Deng, Rantao Dong, Wenjing Song, Quanxing Zheng, Weikun Lai

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  34. Electrochemical Chlorine Shuttle from PVC Waste to Vinyl Ether Acceptors for the Synthesis of Biodegradable Polyester Precursors

    Advanced Materials · 2025-11-12

    Sebastian Becker, Dominik Wördehoff, Dominik Weis, Simon Horsinka, Siegfried R. Waldvogel, Pol Besenius

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  35. Plastic waste recycling: an overview of the mechanical, chemical, and thermal technologies

    Journal of Engineering and Applied Science · 2025-12-01

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  36. Mechanism-Guided dechlorination of PVC-Containing resins in subcritical aqueous ammonia

    Chemical Engineering Science · 2025-12-24

    Zeng-Bao Liu, Xiao-Sa Liu, Zibin Huang, Jin-Yi Yang, Yan Li, Pei‐Qing Yuan

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  37. Asymmetrically coordinated Co–N 3 B 1 single-atom catalysts for the selective hydrogenation of halonitrobenzenes

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  38. Microwave-assisted recycling of plastic waste into value-added chemicals: challenges, recent advances, and perspectives

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  39. Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe

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  40. Chemical Upcycling of Waste Chlorinated Plastics into α,ω-Dienes via Consecutive Dehydrochlorination-Hydrogenation with HCl Trapping and Metathesis

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  41. Elucidating the role of overlooked environmentally persistent free radicals and reactive chlorine species on photoaged chlorine-containing microplastics: New insights into formation mechanisms and health risks

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  42. A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways

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  43. Achieving Near‐Complete Dechlorination of Poly(vinyl chloride) via Electrochemical Reduction

    ChemSusChem · 2026-05-18

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  44. Coordination-Engineered Fe Single Atoms Enable Synergistic PVC Upcycling into Fuel-Range Hydrocarbons via Fenton-Like Pathway

    Environmental Science & Technology · 2026-07-02

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  45. Advances in Chemical Upcycling of Plastic Waste: Pathways to High-Value Products for a Sustainable Circular Economy

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  46. Enabling Downstream Recycling: Separation and Debromination of Polymeric Brominated Flame Retardants from Polystyrene

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  47. Enhanced Catalytic Dechlorination of Polyvinyl Chloride (PVC) and H2 Production Enabled by Synergistic Gaδ+/Ga0 Active Sites in Liquid Metal Particles

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  48. Copolymer microstructure evolution in hydrodechlorination of PVC: A triad kinetics model for sequence modification

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  49. Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock

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