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RESEARCH PAPER · Applied Catalysis B: Environmental · 2023

Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures

Julia N. Hancock, Julie E. Rorrer

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Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperaturesOriginalQuantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Toward Intrinsic Catalytic Rates and Selectivities of Zeolites in the Presence of Limiting Diffusion and Deactivation50Converting Waste Plastic to Liquid Organic Hydrogen Carriers16Converting Waste Plastic to Liquid Organic Hydrogen Carriers1Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins17Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Hydrogen‐transfer strategy in lignin refinery: Towards sustainable and versatile value‐added biochemicals20Layered self-pillared zeolites convert polyethylene to gasoline6Catalytic Upcycling of Polyolefins316Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle28Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts35Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts6Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Tandem chemical hydrolysis and bioelectrochemical upcycling of waste polyethylene terephthalate (PET) for sustainable biobutanol and ethanol production ensuring plastics circularity23Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Effects of Pretreatment Conditions and Branched Alkanes on Mo/MCM-41 Catalysts in Tandem Alkane Cross-metathesis for Non-hydrogen Polyolefin Recycling3Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Green and efficient conversion of polypropylene wastes into Ni@CNTs hybrids and their application for fire resistant polycarbonate composites2CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Facile catalytic conversion of spent mulching films to light oil via Fe-modified Al2O31Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3In Situ Catalytic Pyrolysis of Spent Mulching Film over Fe/Ni/Co-Doped α-Al 2 O 3 for Light Oil and High-Value Aromatics1Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Polymer‐Based Recycling Strategies for Plastic Waste: A Comprehensive Review7Hydrogen-free reductive catalytic fractionation of biomass via synergistic solvent-catalyst interactions: mechanistic and kinetic insights0Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Low concentration pre-implanted Co sites bridged two-phase interface coordination for efficient conversion of polypropylene wastes in a hydrothermal-peroxymonosulfate process0Coming full circle: Biofuels, plastic waste, and the circular economy0

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41 direct citing papers saved.

  1. Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling

    Reaction Chemistry & Engineering · 2023-09-26

    Ziqiu Chen, Emmanuel Ejiogu, Baron Peters

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  2. Toward Intrinsic Catalytic Rates and Selectivities of Zeolites in the Presence of Limiting Diffusion and Deactivation

    ACS Catalysis · 2023-09-26

    Cole W. Hullfish, Jun Zhi Tan, Hayat I. Adawi, Michele L. Sarazen

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  3. Converting Waste Plastic to Liquid Organic Hydrogen Carriers

    Angewandte Chemie International Edition · 2023-11-20

    Mahdokht Soltani, Julie E. Rorrer

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  4. Converting Waste Plastic to Liquid Organic Hydrogen Carriers

    Angewandte Chemie · 2023-11-20

    Mahdokht Soltani, Julie E. Rorrer

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  5. Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles

    Angewandte Chemie · 2023-12-17

    Shibashish D. Jaydev, Antonio José Martín, Marc‐Eduard Usteri, Katia Chikri, Henrik Eliasson, Rolf Erni, Javier Pérez‐Ramírez

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  6. Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles

    Angewandte Chemie International Edition · 2023-12-18

    Shibashish D. Jaydev, Antonio José Martín, Marc‐Eduard Usteri, Katia Chikri, Henrik Eliasson, Rolf Erni, Javier Pérez‐Ramírez

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  7. Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins

    RSC Advances · 2024-01-01

    Guoqing Zhang, Qingguo Mao, Yiqun Yue, Ruitong Gao, Yajing Duan, Hui Du

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  8. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

    Energy & Fuels · 2024-01-22

    Abdulrahman Musa, E. A. Jaseer, Samir Barman, Néstor Garcı́a

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  9. Hydrogen‐transfer strategy in lignin refinery: Towards sustainable and versatile value‐added biochemicals

    ChemSusChem · 2024-01-31

    Yilin Li, Meng Liu, Qi Tang, Kaixia Liang, Yaxu Sun, Yanyan Yu, Yuhan Lou, Yongzhuang Liu, Haipeng Yu

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  10. Layered self-pillared zeolites convert polyethylene to gasoline

    Nature Chemistry · 2024-05-28

    Chris Torres, Julie E. Rorrer

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  11. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  12. Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling

    Nature Chemical Engineering · 2024-08-28

    Shibashish D. Jaydev, Antonio José Martín, David Garcia, Katia Chikri, Javier Pérez‐Ramírez

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  13. Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle

    ACS Applied Polymer Materials · 2024-09-20

    Alison J. Shapiro, Paul J. Brigandi, Maria Moubarak, Saurav S. Sengupta, Thomas H. III Epps

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  14. Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts

    Angewandte Chemie International Edition · 2024-10-07

    Ryan Helmer, Siddhesh S. Borkar, Aojie Li, Fatima Mahnaz, Jenna Vito, Michelle Bishop, Ashfaq Iftakher, M. M. Faruque Hasan, Srinivas Rangarajan, Manish Shetty

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  15. Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts

    Angewandte Chemie · 2024-10-07

    Ryan Helmer, Siddhesh S. Borkar, Aojie Li, Fatima Mahnaz, Jenna Vito, Michelle Bishop, Ashfaq Iftakher, M. M. Faruque Hasan, Srinivas Rangarajan, Manish Shetty

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  16. Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions

    Journal of Hazardous Materials · 2024-11-19

    Bingyan Sun, Haifeng Xu, Tan Li, Wenjie Guan, Kaige Wang

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  17. Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies

    Industrial & Engineering Chemistry Research · 2024-12-06

    Emmanuel Ejiogu, Baron Peters

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  18. Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques

    Molecules · 2024-12-29

    Acácio S. de Souza, Patrícia Garcia Ferreira, Iva Souza de Jesus, Rafael Portugal Rizzo Franco de Oliveira, Alcione Silva de Carvalho, Débora Omena Futuro, Vı́tor F. Ferreira

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  19. Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design

    Chemical Communications · 2025-01-01

    M.J. Kim, Insoo Ro

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  20. Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites

    Green Chemistry · 2025-01-01

    Taeeun Kwon, J. S. PARK, Ki Hyuk Kang, Dae-Sung Jung, Wangyun Won, Insoo Ro

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  21. Tandem chemical hydrolysis and bioelectrochemical upcycling of waste polyethylene terephthalate (PET) for sustainable biobutanol and ethanol production ensuring plastics circularity

    Green Chemistry · 2025-01-01

    Harishankar Kopperi, Vishnuvardhan Mamidi, G. Suresh, S. Venkata Mohan

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  22. Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters

    Polymer Degradation and Stability · 2025-01-27

    Thangaraj Baskaran, Yong-Kul Lee

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  23. Effects of Pretreatment Conditions and Branched Alkanes on Mo/MCM-41 Catalysts in Tandem Alkane Cross-metathesis for Non-hydrogen Polyolefin Recycling

    Korean Journal of Chemical Engineering · 2025-02-07

    Seung Ha Ryu, Hankyeul Kang, Jong Hun Kang

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  24. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  25. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  26. The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction

    Journal of Catalysis · 2025-03-21

    Selena Moore, Andrew Tran, Andreas Palmateer, Jose Naranjo Mendez, Dimitri Gatzios, Peter A. Eschbach, Joel Miscall, Lucas D. Ellis

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  27. Green and efficient conversion of polypropylene wastes into Ni@CNTs hybrids and their application for fire resistant polycarbonate composites

    Journal of environmental chemical engineering · 2025-04-02

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  28. CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor

    Nature Communications · 2025-08-21

    Yuqi Wang, Qikun Hu, Shuairen Qian, Jiayang Zhao, Yi Cheng, Jun Ma, Jing Zhang, Zhiqiang Niu

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  29. Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy

    Nature Chemical Engineering · 2025-10-14

    Tianrui Bi, Yinlin Chen, Longfei Lin, Xue Han, Yang Pan, Chengyuan Liu, Ziyu Cen, Cong Luo, Weilong Wen, Hunain Zulfiqar, Xinrui Zheng, Pascal Manuel, Qian Li, Ningning Wu, Junfeng Xiang, Sihai Yang⧫, Buxing Han

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  30. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

    Korean Journal of Chemical Engineering · 2025-10-20

    Taeeun Kwon, Jae Woo Kim, Insoo Ro

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  31. Facile catalytic conversion of spent mulching films to light oil via Fe-modified Al2O3

    Fuel · 2025-11-20

    Zhong-He Song, Imran Muhammad, Tie-Zhen Ren, Kenji Okitsu, Ablikemu Abulizi, Ai-Sha Nulahong, Zhi-Jun Ren

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  32. Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins

    Journal of Analytical and Applied Pyrolysis · 2025-12-17

    Wei Qiang, Kangzhou Wang, Wenlong Song, Tong Liu, Yongjun Jiang, Weijie Zhang, Chenlong Huang, Xiaowei Li, Jianli Zhang

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  33. In Situ Catalytic Pyrolysis of Spent Mulching Film over Fe/Ni/Co-Doped α-Al 2 O 3 for Light Oil and High-Value Aromatics

    Industrial & Engineering Chemistry Research · 2025-12-29

    Zhong-He Song, Imran Muhammad, Tie‐Zhen Ren, Abulikemu Abulizi, Kenji Okitsu

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  34. Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics

    The Innovation Energy · 2026-01-01

    Bingyan Sun, Bo Li, Marc Mate, Linjia Yin, Qihui Song, Xiaopeng Shi, Dingran Wang, Fawei Lin, Kaige Wang

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  35. Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control

    Chemical Engineering Journal · 2026-01-31

    Hyeongdong Jung, Junho Suh, Yong Hyun Lim, Hyungjoo Kim, Hyungjoo Kim, Inhak Song, Eunwon Lee, Jae‐Soon Choi, Jungup Bang, Do Heui Kim, Do Heui Kim

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  36. Polymer‐Based Recycling Strategies for Plastic Waste: A Comprehensive Review

    Environmental Quality Management · 2026-02-06

    Ishraga GalalEldin Abdalla Awad

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  37. Hydrogen-free reductive catalytic fractionation of biomass via synergistic solvent-catalyst interactions: mechanistic and kinetic insights

    Bioresource Technology · 2026-02-25

    Minjie Hou, Wu Lan, Qiqi Dai, Xu Zeng, Yan Xu, Danlu Zhang, Chuanfu Liu, Fengxia Yue

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  38. Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene

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  39. iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading

    ACS Sustainable Chemistry & Engineering · 2026-04-27

    Guojing Shi, Zhenlei Zhang, Yuliang Li, Xiaochun Zhu, Zhenchen Tang, Zhentao Chen, Y Chen, Jiaqi Feng, bingyu li, Xiangping Zhang

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  40. Low concentration pre-implanted Co sites bridged two-phase interface coordination for efficient conversion of polypropylene wastes in a hydrothermal-peroxymonosulfate process

    Journal of Alloys and Compounds · 2026-05-01

    Xin Wang, Guohang Zhou, Zhihong Ye, Duqiang Zhang, Lin Yuan

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  41. Coming full circle: Biofuels, plastic waste, and the circular economy

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