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RESEARCH PAPER · Energy & Fuels · 2024

Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

Abdulrahman Musa, E. A. Jaseer, Samir Barman, Néstor Garcı́a

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Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and OutlookOriginalChemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Perspectives on the Application of Waste Materials in Asphalt Based on Molecular Dynamics Simulations: A Review26Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Theoretical determination of a model molecule for the catalytic upcycling of polyolefins1Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Scalable Synthesis of Degradable Copolymers Containing α-Lipoic Acid via Miniemulsion Polymerization61Applications of nickel-containing structured microfibrous catalysts for the process of propane hydrogenolysis0Cr6+ Loaded Lewis Acidic Sn‐Beta Zeolites as Reusable Catalysts for Selective Production of Light Olefins via Polyolefin Cracking2Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Computational insights into hydrogen interaction with the Ru (1011) and Ru (1010) surfaces: implications for alkane and polyolefin hydrogenolysis1Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Hydrogenolysis and hydrocracking of biomass and plastic wastes to produce high-value products1Theoretical determination of a model molecule for the catalytic upcycling of polyethylene and polypropylene0Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation5Can the Hock Process Be Used to Produce Phenol from Polystyrene?27Using Nickel-Containing Structured Microfiber Catalysts in the Hydrogenolysis of Propane0Modern Methods of Obtaining Synthetic Oil from Unconventional Hydrocarbon Raw Materials: Technologies, Catalysts, and Development Prospects11Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Thermochemical conversion and gasification of high-density polyethylene (HDPE) in supercritical CO2: A sustainable approach to plastic waste management15Carbamate-bond breaking on bulk oxides realizes highly efficient polyurethane depolymerization15Future carbon footprint of municipal plastic waste treatment in china across the nexus of energy transition, bio-economy, and chemical recycling2Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Harnessing Biofilm-Mediated Plastic Biodegradation: Innovating Smart Material Design18A Review on Sustainable Upcycling of Plastic Waste Through Depolymerization into High-Value Monomer38The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Recent Progress in Sustainable Recycling of Waste Acrylonitrile–Butadiene–Styrene (ABS) Plastics16Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Comprehensive analysis of solvent-assisted liquefaction of polyethylene for fuel production and techno-economic evaluation0Microwave-assisted catalytic upcycling of polyolefin wastes into hydrogen and carbon nanotubes over Pt-promoted Fe/Ni bimetallic catalysts10Valorization of plastic waste into drop-in fuels: Economic and environmental perspectives16Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10CO2-assisted control of H2/CO ratio in plastic waste pyrolysis5Carbon–carbon bond cleavage for lignin and plastics deconstruction0Elucidating the formation of nanoplastics from plastic nurdles in hydrocarbon-contaminated water0Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis6Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Solar-Driven Upcycling of Polystyrene Enabled by Elemental Sulfur8Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Harnessing plant lignin for sustainable materials and chemicals: integrating biosynthesis, structural diversity, and circular bioeconomy perspectives5Ceria‐Based Catalysts for Sustainable Processing of Plastic Waste0Design of a Chitinase-Responsive, Depolymerizable Petroleum-Derived Polymer for Circular and Antifouling Materials0Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Hydrogenolytic depolymerization of red pine bark procyanidins: Effects on phenolic composition, antioxidant capacity, bioaccessibility, and cellular accumulation0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0

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  2. Perspectives on the Application of Waste Materials in Asphalt Based on Molecular Dynamics Simulations: A Review

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  4. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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  5. Theoretical determination of a model molecule for the catalytic upcycling of polyolefins

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  6. Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts

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  7. Scalable Synthesis of Degradable Copolymers Containing α-Lipoic Acid via Miniemulsion Polymerization

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  8. Applications of nickel-containing structured microfibrous catalysts for the process of propane hydrogenolysis

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  9. Cr6+ Loaded Lewis Acidic Sn‐Beta Zeolites as Reusable Catalysts for Selective Production of Light Olefins via Polyolefin Cracking

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  11. Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts

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  12. Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems

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  13. Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques

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  14. Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites

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  16. Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering

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  17. Hydrogenolysis and hydrocracking of biomass and plastic wastes to produce high-value products

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  22. Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation

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  34. Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds

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