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RESEARCH PAPER · Applied Catalysis B: Environmental · 2022

Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

Linxiao Chen, J. Moreira, Laura C. Meyer, Oliver Y. Gutiérrez, János Szanyi

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Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase CatalystOriginalHydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Aromatic production from high-density polyethylene over zinc promoted HZSM-563Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Precise activation of C–C bonds for recycling and upcycling of plastics81Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins17Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Hydrogen Spillover Is Regulating Minority Rh1 Active Sites on TiO2 in Room-Temperature Ethylene Hydrogenation7Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Catalytic Upcycling of Polyolefins316Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Confined metal-acid units for boosting benzene hydroalkylation via efficient activation of key intermediate8Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Tuning solvent strength can fractionate PVC into ultra-low molecular weight material with low dispersity6Upgrading of waste polyolefins with non-noble metal catalysts21Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Influence of catalyst acidity of spent FCC catalyst and TiO2 on product distribution in microwave assisted LDPE cracking5Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics9Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts3Dual-catalyst system without supported metals toward polyethylene waste upcycling3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Hydrogen-rich gas and value-added hydrocarbon production from LDPE via microwave-assisted catalytic pyrolysis using Ni and Zn supported catalysts0Turning debris into diesel: room-temperature synthesis of FeO6 AlO6PO4 AlPO4 integrated framework catalyst for waste plastic-to-diesel cracking0Oligomerization and co-oligomerization of waste polypropylene cracking products to sustainable aviation fuel components0Collaborative Pt–Ni Sites Enable CO-Tolerant Hydrocracking for Upcycling Polyolefin Waste1Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor

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  2. Aromatic production from high-density polyethylene over zinc promoted HZSM-5

    Applied Catalysis B: Environmental · 2023-08-09

    Kezhen Qian, Wenmin Tian, Lijie Yin, Zixu Yang, Fei-Xiang Tian, Dezhen Chen

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  3. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

    Angewandte Chemie International Edition · 2023-10-06

    Qingyun Kang, Mingyu Chu, Panpan Xu, Xuchun Wang, Shiqi Wang, Muhan Cao, Oleksandr Ivasenko, Tsun‐Kong Sham, Qiao Zhang, Qiming Sun, Jinxing Chen

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  4. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

    Angewandte Chemie · 2023-10-06

    Qingyun Kang, Mingyu Chu, Panpan Xu, Xuchun Wang, Shiqi Wang, Muhan Cao, Oleksandr Ivasenko, Tsun‐Kong Sham, Qiao Zhang, Qiming Sun, Jinxing Chen

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  5. Precise activation of C–C bonds for recycling and upcycling of plastics

    Chemical Science · 2023-12-07

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  6. Ni-based catalysts supported on Hbeta zeolite for the hydrocracking of waste polyolefins

    RSC Advances · 2024-01-01

    Guoqing Zhang, Qingguo Mao, Yiqun Yue, Ruitong Gao, Yajing Duan, Hui Du

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  7. Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production

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    Arjun K. Manal, Atal Shivhare, Sharad V. Lande, Rajendra Srivastava

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  8. Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste

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  9. Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect

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  10. Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts

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  11. Layered Double Hydroxide Derivatives for Polyolefin Upcycling

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  12. Hydrogen Spillover Is Regulating Minority Rh1 Active Sites on TiO2 in Room-Temperature Ethylene Hydrogenation

    ACS Catalysis · 2024-04-26

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  13. Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics

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  14. Catalytic Upcycling of Polyolefins

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  15. Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling

    Nature Chemical Engineering · 2024-08-28

    Shibashish D. Jaydev, Antonio José Martín, David Garcia, Katia Chikri, Javier Pérez‐Ramírez

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  16. Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts

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  17. Confined metal-acid units for boosting benzene hydroalkylation via efficient activation of key intermediate

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  18. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

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  19. Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems

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  20. Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design

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  21. Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts

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  22. Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts

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  23. Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels

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  24. Tuning solvent strength can fractionate PVC into ultra-low molecular weight material with low dispersity

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  25. Upgrading of waste polyolefins with non-noble metal catalysts

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  27. Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters

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  28. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

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  29. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

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  30. Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets

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  31. Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions

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  32. Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters

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  33. Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters

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  34. Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste

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  35. Influence of catalyst acidity of spent FCC catalyst and TiO2 on product distribution in microwave assisted LDPE cracking

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  36. Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics

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  37. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

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  38. Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts

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  39. Dual-catalyst system without supported metals toward polyethylene waste upcycling

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  40. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

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  43. Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking

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  44. Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics

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  45. Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 4

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