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RESEARCH PAPER · ChemCatChem · 2022

Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage

Shenglu Lu, Yaxuan Jing, Shengchao Jia, Mohsen Shakouri, Yongfeng Hu, Xiaohui Liu, Yong Quan Guo, Yanqin Wang

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Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond CleavageOriginalPhotothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Coproduction of Glyceric Acid and Glycolic Acid from Biomass-Based Sugars over a Ru/Co3O4 Catalyst23Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Ambient-temperature α-pinene hydrogenation to cis-pinane over Ru/CeO2-H catalyst via the dimethyl-up configuration2Synergistic Catalysis for Recycling and Upcycling of Plastics35Methods for Carbon Mass Closure in Polyolefin Hydrocracking6NbOx-Based Catalysts for Biomass Conversion: Progress in the Past 20 Years18Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Carbon–carbon bond cleavage for lignin and plastics deconstruction0Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Mechanistic insights into plasma–thermal field coupling over Ru/CeO 2 for enhanced ammonia decomposition1Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Ni Supported on Urea‐Modified LaFeO 3 Perovskite for Efficient Hydrogenolysis of Polyethylene Plastics2Ceria‐Based Catalysts for Sustainable Processing of Plastic Waste0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0

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  1. Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions

    Nature Communications · 2023-07-15

    Yingxuan Miao, Yunxuan Zhao, Geoffrey I. N. Waterhouse, Run Shi, Li‐Zhu Wu, Tierui Zhang

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  2. Upcycling of polyethylenes by catalysis

    Unknown journal · 2023-07-20

    Adamu Aminu Idris

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  3. Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts

    Applied Catalysis A General · 2023-09-01

    Ajay Tomer, Mazharul M. Islam, Mounib Bahri, Donald R. Inns, Troy D. Manning, John B. Claridge, Nigel D. Browning, C. Richard A. Catlow, Alberto Roldán, Alexandros P. Katsoulidis, Matthew J. Rosseinsky

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  4. Precise activation of C–C bonds for recycling and upcycling of plastics

    Chemical Science · 2023-12-07

    Hongshun Ran, Shuo Zhang, Wenyi Ni, Yaxuan Jing

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  5. Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst

    Energy Conversion and Management · 2023-12-15

    Ruizhe Chen, Leilei Cheng, Jing Gu, Haoran Yuan, Yong Chen

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  6. Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production

    Chemical Communications · 2024-01-01

    Arjun K. Manal, Atal Shivhare, Sharad V. Lande, Rajendra Srivastava

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  7. Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts

    Chem & Bio Engineering · 2024-01-04

    Yong Yuan, Zhenhua Xie, Kevin K. Turaczy, Sooyeon Hwang, Jiahua Zhou, Jingguang G. Chen

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  8. Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect

    Chemical Engineering Journal · 2024-03-11

    Leilei Cheng, Shaonan Tian, Dong Sheng Liang, Jing Gu, Ruizhe Chen, Xueru Chen, Haoran Yuan, Yong Chen

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  9. Layered Double Hydroxide Derivatives for Polyolefin Upcycling

    Journal of the American Chemical Society · 2024-04-02

    Mingyu Chu, Xianpeng Wang, Xuchun Wang, Panpan Xu, Zhang Lin, Shengming Li, Kun Feng, Jun Bo Zhong, Lu Wang, Youyong Li, Le He, Muhan Cao, Qiao Zhang, Lifeng Chi, Jinxing Chen

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  10. Coproduction of Glyceric Acid and Glycolic Acid from Biomass-Based Sugars over a Ru/Co3O4 Catalyst

    ACS Catalysis · 2024-05-01

    Yancheng Liu, Shiwei Zhou, Xiaoyan Wang, Jingying Qin, Changwei Hu, Jianmei Li

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  11. Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions

    ChemSusChem · 2024-05-02

    Gao Li, Xia Zhong, Jie Liu, Junnan Chen, Ziru Wang, Ying Zhang, Deli Wang, Mozaffar Shakeri, Xia Zhang, Bingsen Zhang

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  12. Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics

    Chemical Engineering Journal · 2024-07-28

    Mingyu Chu, Qingyun Kang, Ping Hu, Qiao Zhang, Jinxing Chen

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  13. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  14. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

    Chem Catalysis · 2024-08-20

    Jueun Kim, Simin Sun, Donghyeon Kim, Byung Gwan Park, Hojeong Lee, Wenyu Huang, Kwangjin An

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  15. Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts

    Journal of Materials Chemistry A · 2024-12-10

    Donald R. Inns, Megan Carr, Mounib Bahri, Ajay Tomer, Troy D. Manning, Nigel D. Browning, Simon A. Kondrat, John B. Claridge, Alexandros P. Katsoulidis, Matthew J. Rosseinsky

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  16. Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite

    Nano Letters · 2025-02-13

    Li Gao, Ziru Wang, Yumeng Zhang, Xia Zhong, Ying Zhang, Mozaffar Shakeri, Zhuangzhi Zhi, Xia Zhang, Bingsen Zhang

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  17. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  18. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  19. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

    Advanced Sustainable Systems · 2025-03-20

    Sahil Kumar, Devanshu Sajwan, Devendra Sharma, Venkata Krishnan

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  20. Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst

    Nature Communications · 2025-03-21

    Jicong Yan, Guanna Li, Zhanwu Lei, Xiaolu Yuan, Junting Li, Xiaoru Wang, Bo Wang, Bo Wang, Fuping Tian, Tao Hu, Lei Huang, Yujia Ding, Xiaoke Xi, Feng Zhu, Shuo Zhang, Jiong Li, Yu Chen, Ruiguo Cao, Xiang Wang, Xiang Wang

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  21. Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites

    Catalysts · 2025-03-31

    Qing Bo Du, Xin Chun Shang, Yangyang Yuan, Xiong Su, Yanqiang Huang

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  22. Ambient-temperature α-pinene hydrogenation to cis-pinane over Ru/CeO2-H catalyst via the dimethyl-up configuration

    Chemical Engineering Journal · 2025-04-12

    Yu-Xuan Fu, Shuyi Huang, Ming-Shuai Sun, Yan Zhou, Dandan Cai, Wenshuai Zhu, Wei Hui, Duan‐Jian Tao

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  23. Synergistic Catalysis for Recycling and Upcycling of Plastics

    ACS Catalysis · 2025-05-07

    Hongshun Ran, Xinyang Sun, Mengying Zheng, Yaxuan Jing

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  24. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

    JACS Au · 2025-07-24

    Anna E. Brenner, Griffin Drake, Gregg T. Beckham, Yuriy Román‐Leshkov

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  25. NbOx-Based Catalysts for Biomass Conversion: Progress in the Past 20 Years

    ACS Catalysis · 2025-08-26

    Yaxuan Jing, Xiaohui Liu, Qineng Xia, Lin Dong, Yong Quan Guo, Yanqin Wang

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  26. Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst

    Journal of Catalysis · 2025-09-11

    Masazumi Tamura, Yuna Sasano, SMA Hakim Siddiki, Masato Akatsuka, Pengru Chen, Yusuke Kita

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  27. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

    Chemistry - A European Journal · 2025-11-02

    Yukari Yamazaki, Xiongjie Jin, Weihan Sun, Satoshi Yamamoto, Katsutoshi Nomoto, Kohei Takahashi, Hiroki Miura, Tetsuya Shishido, Akira Nakayama, Kyoko Nozaki

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  28. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025-12-10

    Fan Yuan, Hongshun Ran, Tingxi Chen, Yaxuan Jing

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  29. Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling

    Green Chemistry · 2026-01-01

    Ruoyan Bai, Roudan Lian, Jian Zhang, Maolin Zhang

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  30. Carbon–carbon bond cleavage for lignin and plastics deconstruction

    Chemical Society Reviews · 2026-01-01

    Davide Rigo, Brandon L. Frey, Alison Sy-min Chang, Marcos G. Farpón, Erik T. Ouellette, Yuriy Román‐Leshkov, Gregg T. Beckham, Joseph S. M. Samec

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  31. Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts

    Green Chemistry · 2026-01-01

    Junho Suh, Hyeongdong Jung, Junho Yoon, Jae‐Soon Choi, Jungup Bang, Do Heui Kim

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  32. Mechanistic insights into plasma–thermal field coupling over Ru/CeO 2 for enhanced ammonia decomposition

    Journal of Materials Chemistry A · 2026-01-01

    Kaibin Xia, Yuhui Du, Junhui Liang, Zhen Shen, Xiaoqi Fei, Jiahui Hou, Hangning Chen, Chenhao Du, Liuqi Wang, Da Chen

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  33. Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts

    Chemical Communications · 2026-01-01

    Zeyuan Zhu, Junhong Liu, Hongyu Wang, Qiao Hu, Dong Liang, Ling Zhang, Zhichao Tao, Jiajing Pei, Xi Liu, Liwei Chen

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  34. Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles

    Science China Chemistry · 2026-01-27

    Qi Zhang, Xiang Wang

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  35. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

    Fuel · 2026-02-26

    Sudipta Nayak, Rajat Singhal, S. M. A. Hakim Siddiki, Ken Motokura, Navya Subray Bhat, Navneet Kumar Gupta

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  36. Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling

    Engineering · 2026-03-01

    Ruoxi Zhang, Aaron David Sadow, Wenyu Huang

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  37. Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering

    Journal of Catalysis · 2026-03-02

    Qinge Fan, Ziyi zhang, Penglong Wang, Penglong Wang, Jicong Yan, Yongna Zhang, Caixia Feng, Li Wang, Li Wang, 常志显, Xiang Wang, Ruifeng Chong

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  38. Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis

    AIChE Journal · 2026-03-16

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  39. Ni Supported on Urea‐Modified LaFeO 3 Perovskite for Efficient Hydrogenolysis of Polyethylene Plastics

    ChemCatChem · 2026-05-01

    Jueun Kim, Donghyeon Kim, Junsu Kim, Changhun Hur, Tae Heon Kim, Daewon Oh, Kwangjin An

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  40. Ceria‐Based Catalysts for Sustainable Processing of Plastic Waste

    Advanced Energy and Sustainability Research · 2026-05-29

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  41. Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst

    Angewandte Chemie · 2026-09-07

    Qianyue Feng, Mingyu Chu, Zhongyu Li, Yeping Xie, Qiao Zhang, Jinxing Chen, Ding Ma

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  42. Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst

    Angewandte Chemie International Edition · 2026-09-07

    Qianyue Feng, Mingyu Chu, Zhongyu Li, Yeping Xie, Qiao Zhang, Jinxing Chen, Ding Ma

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