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RESEARCH PAPER · ACS Sustainable Chemistry & Engineering · 2023

Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts

Siddhesh S. Borkar, Ryan Helmer, Suraj Panicker, Manish Shetty

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Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt CatalystsOriginalQuantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Converting Waste Plastic to Liquid Organic Hydrogen Carriers16Converting Waste Plastic to Liquid Organic Hydrogen Carriers1Precise activation of C–C bonds for recycling and upcycling of plastics81Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex12Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex3Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Selective Hydrogenolysis Conversion of Polyethylene into Alkyl Oil Over Iridium‐based Catalyst9Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts35Tandem Methanolysis and Catalytic Transfer Hydrogenolysis of Polyethylene Terephthalate to p‐Xylene Over Cu/ZnZrO x Catalysts6Efficient polycarbonate plastic upcycling into jet fuel cycloalkanes over a bifunctional MoCo/NiC hetero-catalyst12Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Upgrading of waste polyolefins with non-noble metal catalysts21Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation5Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Synergistic Catalysis for Recycling and Upcycling of Plastics35Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Long-lived metal-zeolite catalysts for polyolefin aromatization via synergistic tandem dehydroaromatization and hydrogenolysis12Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Unveiling the role of Ni-Re catalyst on diverse supports for efficient hydrogenation of levulinic acid to γ-valerolactone under near atmospheric H2 pressure8Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Engineered BDH–NOx co-expression in Escherichia coli enables highly efficient in vivo cascade catalysis for the transformation of racemic epoxides to α-hydroxyketones0Data-Driven Discovery of Bimetallic Nanoparticles Catalysts for the Hydrogenolysis of Polyethylene3Research progress of high value utilization of waste polyethylene plastics6Catalytic valorization of polyolefins: from catalysts and processes to reactors0Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Circularity in polyethylene waste management through multidimensional integration3Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Compressed CO 2 -Assisted Catalytic Hydrocracking of Polyethylene over Ru-Loaded Zeolites0Application of green dissolution separation and recycling of waste polyester/cotton/polyurethane blended fabric1NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Ni Supported on Urea‐Modified LaFeO 3 Perovskite for Efficient Hydrogenolysis of Polyethylene Plastics2Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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