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RESEARCH PAPER · ACS Central Science · 2019

Upcycling Single-Use Polyethylene into High-Quality Liquid Products

Gokhan Celik, Robert M. Kennedy, Ryan A. Hackler, Magali S. Ferrandon, Akalanka Tennakoon, Smita Patnaik, Anne M. LaPointe, Salai Cheettu Ammal, Andreas Heyden, Frédéric A. Perras, Marek Pruski, Susannah L. Scott, Kenneth Reinhard Poeppelmeier, Aaron David Sadow, Massimiliano Delferro

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Upcycling Single-Use Polyethylene into High-Quality Liquid ProductsOriginalPlastic upcycling83Scalable upcycling of thermoplastic polyolefins into vitrimers through transesterification164Beyond Mechanical Recycling: Giving New Life to Plastic Waste1886Die nächste Generation des Recyclings – neues Leben für Kunststoffmüll77Luminescent carbon dots obtained from polymeric waste66The Use of Heterogeneous Catalysis in the Chemical Valorization of Plastic Waste223100th Anniversary of Macromolecular Science Viewpoint: Toward Catalytic Chemical Recycling of Waste (and Future) Plastics309Catalytic upcycling of high-density polyethylene via a processive mechanism526Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatization889Low-temperature catalytic upgrading of waste polyolefinic plastics into liquid fuels and waxes331100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers281Conversion of Polyolefin Waste to Liquid Alkanes with Ru-Based Catalysts under Mild Conditions412Catalytic methods for chemical recycling or upcycling of commercial polymers370Non-thermal plasma-assisted hydrogenolysis of polyethylene to light hydrocarbons62Microbial synthesis of vanillin from waste poly(ethylene terephthalate)232Tandem Heterogeneous Catalysis for Polyethylene Depolymerization via an Olefin-Intermediate Process171Catalytic processing of plastic waste on the rise622Arresting Elevated-Temperature Creep and Achieving Full Cross-Link Density Recovery in Reprocessable Polymer Networks and Network Composites via Nitroxide-Mediated Dynamic Chemistry107Catalytic hydrocracking of synthetic polymers into grid-compatible gas streams79Valorisation of plastic waste via metal-catalysed depolymerisation62Catalytic carbon-carbon bond cleavage and carbon-element bond formation give new life for polyolefins as biodegradable surfactants81Plastic waste to fuels by hydrocracking at mild conditions584Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalyst211Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future325Recent Progress in the Chemical Upcycling of Plastic Wastes301Integrating Emerging Polymer Chemistries for the Advancement of Recyclable, Biodegradable, and Biocompatible Electronics166Potential Chemicals from Plastic Wastes57Spontaneous Electric Fields Play a Key Role in Thermochemical Catalysis at Metal−Liquid Interfaces81Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities177Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts265Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia180A review on metal-organic frameworks photoelectrochemistry: A headlight for future applications150Upcycling to Sustainably Reuse Plastics305Chemical and biological catalysis for plastics recycling and upcycling1204Upcycling and catalytic degradation of plastic wastes334Depolymerization of Hydroxylated Polymers via Light-Driven C–C Bond Cleavage112Plastic waste upcycling toward a circular economy425Why is Recycling of Postconsumer Plastics so Challenging?381Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia296Chemical recycling of plastic waste via thermocatalytic routes159Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts83Rapid colonization and biodegradation of untreated commercial polyethylene wrap by a new strain of Bacillus velezensis C571Catalytic Amination of Polylactic Acid to Alanine211Chemical Upcycling of Polyethylene to Value-Added α,ω-Divinyl-Functionalized Oligomers92Design principles for intrinsically circular polymers with tunable properties217Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes305Managing Plastic Waste─Sorting, Recycling, Disposal, and Product Redesign640From plastic waste to wealth using chemical recycling: A review304Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study146Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer Reactions63Conversion of plastic waste into high-value lubricants: techno-economic analysis and life cycle assessment74Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes134Expanding plastics recycling technologies: chemical aspects, technology status and challenges616Marine waste upcycling—recovery of nylon monomers from fishing net waste using seashell waste-derived catalysts in a CO 2 -mediated thermocatalytic process64How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics Recycling401From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials276Nanocatalyzed upcycling of the plastic wastes for a circular economy125Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins169Catalytic carbon and hydrogen cycles in plastics chemistry78Upgrading waste plastic derived pyrolysis gas via chemical looping cracking–gasification using Ni–Fe–Al redox catalysts72Embedding ZnCdS@ZnIn2S4 into thiazole-modified g-C3N4 by electrostatic self-assembly to build dual Z-scheme heterojunction with spatially separated active centers for photocatalytic H2 evolution and ofloxacin degradation95The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis217Rational Design of Chemical Catalysis for Plastic Recycling396Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61NbOx-Based Catalysts for the Activation of C–O and C–C Bonds in the Valorization of Waste Carbon Resources83Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis114Solar energy-driven upcycling of plastic waste on direct Z-scheme heterostructure of V-substituted phosphomolybdic acid/g-C3N4 nanosheets142Cyanamide as a Highly Efficient Organocatalyst for the Glycolysis Recycling of PET102Innovations Toward the Valorization of Plastics Waste66Polyolefin Innovations toward Circularity and Sustainable Alternatives97Environmental toxicity and decomposition of polyethylene286Microwave-initiated MAX Ti3AlC2-catalyzed upcycling of polyolefin plastic wastes: Selective conversion to hydrogen and carbon nanofibers for sodium-ion battery68A unified view on catalytic conversion of biomass and waste plastics595Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts144Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts140A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium108Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts130Catalytic strategies for upvaluing plastic wastes210Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst79Catalytic deconstruction of waste polyethylene with ethylene to form propylene421Chemical Recycling of Polyethylene by Tandem Catalytic Conversion to Propylene262RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Microplastic materials in the environment: Problem and strategical solutions205Multicomponent magnetic nanoparticle engineering: the role of structure-property relationship in advanced applications106Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons176Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism122Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117A state-of-the-art review on waste plastics-derived aviation fuel: Unveiling the heterogeneous catalytic systems and techno-economy feasibility of catalytic pyrolysis79Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst84Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review273Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes60Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Catalytic Chemical Recycling of Post-Consumer Polyethylene189Recent advances in plastic recycling and upgrading under mild conditions147A comprehensive review of sustainable approaches for synthetic lubricant components67Converting Plastic Wastes to Naphtha for Closing the Plastic Loop188Micro- and nano-plastics (MNPs) as emerging pollutant in ground water: Environmental impact, potential risks, limitations and way forward towards sustainable management214Review of polymer technologies for improving the recycling and upcycling efficiency of plastic waste273Ultrasmall amorphous zirconia nanoparticles catalyse polyolefin hydrogenolysis177Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation311Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment85PF 6 − Pseudohalides Anion Based Metal‐Free Perovskite Single Crystal for Stable X‐Ray Detector to Attain Record Sensitivity77Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins115A two-stage strategy for upcycling chlorine-contaminated plastic waste142Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites70Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook205Catalytic approaches for the removal of microplastics from water: Recent advances and future opportunities73Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Cellulose-Based Ionic Conductor: An Emerging Material toward Sustainable Devices235Optimization of the process parameters of catalytic plastic pyrolysis for oil production using design of experiment approaches: A review102Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions172SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins63Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants354Additive manufacturing for sustainability and circular economy: needs, challenges, and opportunities for 3D printing of recycled polymeric waste150Solar-driven photocatalysis for recycling and upcycling plastics123Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals135Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Precise activation of C–C bonds for recycling and upcycling of plastics81Characterization of polymer properties and identification of additives in commercially available research plastics111Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle107Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Circular olefin copolymers made de novo from ethylene and α-olefins83Synthesis and Deconstruction of Polyethylene-type Materials195A state-of-the-art review of multilayer packaging recycling: Challenges, alternatives, and outlook149Layered Double Hydroxide Derivatives for Polyolefin Upcycling102Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy60Recent advances in magnetic nanoparticles: Key applications, environmental insights, and future strategies57Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions103Advances in Nonreactive Polymer Compatibilizers for Commodity Polyolefin Blends102Catalytic Upcycling of Polyolefins317Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals81Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Plastic recycling: Challenges and opportunities89Poly(vinyl chloride) (PVC): an updated review of its properties, polymerization, modification, recycling, and applications73Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Current methods for plastic waste recycling: Challenges and opportunities63Advanced Catalysts for the Chemical Recycling of Plastic Waste90Highly selective upcycling of plastic mixture waste by microwave-assisted catalysis over Zn/b-ZnO68Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73Co-recycling of plastics and other waste materials71High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65

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