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RESEARCH PAPER · Chem · 2021

Isolated metal atoms and clusters for alkane activation: Translating knowledge from enzymatic and homogeneous to heterogeneous systems

Lichen Liu, Avelino Corma

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Isolated metal atoms and clusters for alkane activation: Translating knowledge from enzymatic and homogeneous to heterogeneous systemsOriginalAcidic hierarchical porous ZSM-5 assembled palladium catalyst: A green substitute to transform primary amides to nitriles25Striding the threshold of an atom era of organic synthesis by single-atom catalysis145Amino induced high-loading atomically dispersed Co sites on N-doped hollow carbon for efficient CO 2 transformation15Surface science approach to the heterogeneous cycloaddition of CO2 to epoxides catalyzed by site-isolated metal complexes and single atoms: a review71General Descriptors for CO 2 -Assisted Selective C–H/C–C Bond Scission in Ethane76Role of Ni species in ZnO supported on Silicalite-1 for efficient propane dehydrogenation20A Career in Catalysis: Avelino Corma25Atomic Insight into the Local Structure and Microenvironment of Isolated Co-Motifs in MFI Zeolite Frameworks for Propane Dehydrogenation238Kinetics of two-step catalytic sequence on nanoclusters with limited cluster occupancy6A Single‐Atom Cobalt Catalyst for the Fluorination of Acyl Chlorides at Parts‐per‐Million Catalyst Loading89A Single‐Atom Cobalt Catalyst for the Fluorination of Acyl Chlorides at Parts‐per‐Million Catalyst Loading11Solid catalysts for the dehydrogenation of long-chain alkanes: lessons from the dehydrogenation of light alkanes and homogeneous molecular catalysis32Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187A Heterogeneous Single Atom Cobalt Catalyst for Highly Efficient Acceptorless Dehydrogenative Coupling Reactions36Post‐Synthetic Surface Modification of Metal–Organic Frameworks and Their Potential Applications190Electronic and structural engineering of supported single atomic layer, low-nuclearity palladium catalysts for conversion of levulinic acid to 1,4-pentanediol24Size-Dependent Structures and Catalytic Properties of Supported Bimetallic PtSn Catalysts for Propane Dehydrogenation Reaction73Synergic Effect of Isolated Ce 3+ and Pt δ+ Species in UiO-66(Ce) for Heterogeneous Catalysis34New trends in the catalytic utilization of alkane resources in a carbon-neutral society3Catalysts: Materials4Cyclohexane Oxidative Dehydrogenation on Graphene-Oxide-Supported Cobalt Ferrite Nanohybrids: Effect of Dynamic Nature of Active Sites on Reaction Selectivity15Characterization of Organic Linker‐Containing Porous Materials as New Emerging Heterogeneous Catalysts2State-of-the-art strategies for the synthesis of zeolite-encapsulated subnanometric metal clusters12Promoting the dehydrogenation of light alkanes with a carbon-based membrane reactor3Catalytic Hydrogenolysis by Atomically Dispersed Iron Sites Embedded in Chemically and Redox Non-innocent N-Doped Carbon28Heterogeneous Iridium-Catalyzed Carbene N–H Bond Insertion with α-Alkyl Diazo Esters29Catalysis paves the way to a new era of the petrochemical industry12Solvent-free selective hydrogenation of nitroaromatics to azoxy compounds over Co single atoms decorated on Nb2O5 nanomeshes91Enhancing enzymatic catalysis efficiency: Immobilizing laccase on HHSS for synergistic bisphenol A adsorption and biodegradation through optimized external surface utilization6Isolated Pt Atoms Stabilized by Ga2O3 Clusters Confined in ZSM-5 for Nonoxidative Activation of Ethane12Dry Reforming of Methane to Syngas Mediated by Rhodium–Cobalt Oxide Cluster Anions Rh2CoO–10Chemical looping for upgrading light alkanes: oxygen carriers, reaction kinetics, and reactor design12Tuning the Selectivity in the Nonoxidative Alkane Dehydrogenation Reaction by Potassium-Promoted Zeolite-Encapsulated Pt Catalysts18Engineering Multi‐Site Platinum Ensembles Synergistically Boosts Catalysis5A Cerium‐Naphthazarin Catecholate MOF as a Heterogeneous Photocatalyst for Selective Functionalization of Alkanes13A Cerium‐Naphthazarin Catecholate MOF as a Heterogeneous Photocatalyst for Selective Functionalization of Alkanes2Isolated Cr Active Centers in the Beta Zeolite Framework for Propane Dehydrogenation21Synergy principle of single active centers and microenvironment for Cr-MFI-catalyzed alkane dehydrogenation16Local coordination environment of isolated Fe sites in zeolite affects the catalytic performance for propane dehydrogenation3Activity descriptor and volcano plots in Lewis acid zeolites for dehydrogenation reactions2Catalysts history, importance, and types0Entropy−Driven Design Principle of High−Performance Pt−Based Propane Dehydrogenation Catalysts1Silica‐Supported Mononuclear Methyl‐Platinum Complexes Stabilized by Trimethylphosphine—Synthesis, Structure, and Reactions Under Reducing Conditions0

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  1. Acidic hierarchical porous ZSM-5 assembled palladium catalyst: A green substitute to transform primary amides to nitriles

    Applied Catalysis B: Environmental · 2021-10-25

    Zhongmiao Chen, Wei Chen, Lei Zhang, Wenqian Fu, Guoren Cai, Anmin Zheng, Tiandi Tang

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  2. Striding the threshold of an atom era of organic synthesis by single-atom catalysis

    Chem · 2021-11-24

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  3. Amino induced high-loading atomically dispersed Co sites on N-doped hollow carbon for efficient CO 2 transformation

    Chemical Communications · 2022-01-01

    Ruirui Yun, Tuanhui Li, Beibei Zhang, Lei He, Shoujie Liu, Can Yu, Zheng Chen, Shizhong Luo

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  4. Surface science approach to the heterogeneous cycloaddition of CO2 to epoxides catalyzed by site-isolated metal complexes and single atoms: a review

    Green Chemical Engineering · 2022-02-05

    Valerio D’Elia, Arjan W. Kleij

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  5. General Descriptors for CO 2 -Assisted Selective C–H/C–C Bond Scission in Ethane

    Journal of the American Chemical Society · 2022-02-08

    Zhenhua Xie, Xuelong Wang, Xiaobo Chen, Ping Liu, Jingguang G. Chen

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  6. Role of Ni species in ZnO supported on Silicalite-1 for efficient propane dehydrogenation

    Chinese Journal of Chemical Engineering · 2022-03-01

    Bofeng Zhang, Mingxia Song, Hongwang Liu, Guozhu Li, Sibao Liu, Li Wang, Xiangwen Zhang, Guozhu Liu

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  7. A Career in Catalysis: Avelino Corma

    ACS Catalysis · 2022-06-01

    Mercedes Boronat, María José Climent, Patricia Concepción, Urbano Díaz, Hermenegildo Garcı́a, Sara Iborra, Antonio Leyva‐Pérez, Lichen Liu, Agustı́n Martı́nez, Cristina Martı́nez, Manuel Moliner, Joaquín Pérez‐Pariente, Fernando Rey, Enrique Sastre, Pedro Serna, Susana Valencia

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  8. Atomic Insight into the Local Structure and Microenvironment of Isolated Co-Motifs in MFI Zeolite Frameworks for Propane Dehydrogenation

    Journal of the American Chemical Society · 2022-06-28

    Zhong‐Pan Hu, Gangqiang Qin, Jingfeng Han, Wenna Zhang, Nan Wang, Yijun Zheng, Qike Jiang, Te Ji, Zhong‐Yong Yuan, Jianping Xiao, Yingxu Wei, Zhongmin Liu

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  9. Kinetics of two-step catalytic sequence on nanoclusters with limited cluster occupancy

    Chemical Engineering Journal · 2022-07-21

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  10. A Single‐Atom Cobalt Catalyst for the Fluorination of Acyl Chlorides at Parts‐per‐Million Catalyst Loading

    Angewandte Chemie International Edition · 2022-08-24

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  11. A Single‐Atom Cobalt Catalyst for the Fluorination of Acyl Chlorides at Parts‐per‐Million Catalyst Loading

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  12. Solid catalysts for the dehydrogenation of long-chain alkanes: lessons from the dehydrogenation of light alkanes and homogeneous molecular catalysis

    Science China Chemistry · 2022-10-18

    Hongliu Wan, Nengfeng Gong, Lichen Liu

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  13. Converting Plastic Wastes to Naphtha for Closing the Plastic Loop

    Journal of the American Chemical Society · 2023-01-12

    Lin Li, Hu Luo, Zilong Shao, Haozhi Zhou, Junwen Lu, Junjun Chen, Chaojie Huang, Shunan Zhang, Xiaofang Liu, Lin Xia, Jiong Li, Hui Wang, Yuhan Sun

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  14. A Heterogeneous Single Atom Cobalt Catalyst for Highly Efficient Acceptorless Dehydrogenative Coupling Reactions

    Small · 2023-02-09

    Zhijun Li, Xiaowen Lu, Rufang Zhao, Siqi Ji, Mingyang Zhang, Joseph Hugh Horton, Yang Wang, Qian Xu, Junfa Zhu

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  15. Post‐Synthetic Surface Modification of Metal–Organic Frameworks and Their Potential Applications

    Small Methods · 2023-02-15

    Leidy Figueroa–Quintero, David Villalgordo‐Hernández, José J. Delgado‐Marín, Javier Narciso, Vijay Kumar Velisoju, Pedro Castaño, Jorge Gascón, Enrique V. Ramos–Fernández

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  16. Electronic and structural engineering of supported single atomic layer, low-nuclearity palladium catalysts for conversion of levulinic acid to 1,4-pentanediol

    Chemical Engineering Journal · 2023-03-27

    Xiaowen Lu, Tingting Luo, Mingyang Zhang, Joseph Hugh Horton, Qiong Wu, Wei Wu, Man Qiao, Yu Wang, Zhijun Li

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  17. Size-Dependent Structures and Catalytic Properties of Supported Bimetallic PtSn Catalysts for Propane Dehydrogenation Reaction

    ACS Catalysis · 2023-05-16

    Hongliu Wan, Lixiang Qian, Nengfeng Gong, Huaming Hou, Xiaomeng Dou, Lirong Zheng, Liang Zhang, Lichen Liu

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  18. Synergic Effect of Isolated Ce 3+ and Pt δ+ Species in UiO-66(Ce) for Heterogeneous Catalysis

    ACS Catalysis · 2023-06-26

    Sergio Rojas‐Buzo, Benjamin Bohigues, Davide Salusso, Avelino Corma, Manuel Moliner, Silvia Bordiga

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  19. New trends in the catalytic utilization of alkane resources in a carbon-neutral society

    Chem Catalysis · 2023-07-01

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  20. Catalysts: Materials

    Elsevier eBooks · 2023-08-04

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  21. Cyclohexane Oxidative Dehydrogenation on Graphene-Oxide-Supported Cobalt Ferrite Nanohybrids: Effect of Dynamic Nature of Active Sites on Reaction Selectivity

    ACS Catalysis · 2023-10-05

    Shashikant A. Kadam, Stefania Sandoval, Zdenĕk Bastl, Karolína Simkovičová, Libor Kvı́tek, Juraj Jašík, Joanna Elzbieta Olszowka, Stanislav Valtera, Mykhailo Vaidulych, Jaroslava Morávková, Petr Sazama, David Kubička, Arnaud Travert, Jeroen A. van Bokhoven, Alessandro Fortunelli, Armin Kleibert, Martin Kalbáč, Štefan Vajda

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  22. Characterization of Organic Linker‐Containing Porous Materials as New Emerging Heterogeneous Catalysts

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  23. State-of-the-art strategies for the synthesis of zeolite-encapsulated subnanometric metal clusters

    Inorganic Chemistry Frontiers · 2024-01-01

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  24. Promoting the dehydrogenation of light alkanes with a carbon-based membrane reactor

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  25. Catalytic Hydrogenolysis by Atomically Dispersed Iron Sites Embedded in Chemically and Redox Non-innocent N-Doped Carbon

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  26. Heterogeneous Iridium-Catalyzed Carbene N–H Bond Insertion with α-Alkyl Diazo Esters

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  27. Catalysis paves the way to a new era of the petrochemical industry

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  28. Solvent-free selective hydrogenation of nitroaromatics to azoxy compounds over Co single atoms decorated on Nb2O5 nanomeshes

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  29. Enhancing enzymatic catalysis efficiency: Immobilizing laccase on HHSS for synergistic bisphenol A adsorption and biodegradation through optimized external surface utilization

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    Hong-Xia Yu, Lijun Feng, Mohamed Abbas, Xue Liang, Tianjing Zhang, Guiping Yang, Yong Liu, Meisong Xu, Yan An, Wanliang Yang

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  30. Isolated Pt Atoms Stabilized by Ga2O3 Clusters Confined in ZSM-5 for Nonoxidative Activation of Ethane

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  31. Dry Reforming of Methane to Syngas Mediated by Rhodium–Cobalt Oxide Cluster Anions Rh2CoO–

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  32. Chemical looping for upgrading light alkanes: oxygen carriers, reaction kinetics, and reactor design

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  33. Tuning the Selectivity in the Nonoxidative Alkane Dehydrogenation Reaction by Potassium-Promoted Zeolite-Encapsulated Pt Catalysts

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  34. Engineering Multi‐Site Platinum Ensembles Synergistically Boosts Catalysis

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  35. A Cerium‐Naphthazarin Catecholate MOF as a Heterogeneous Photocatalyst for Selective Functionalization of Alkanes

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  36. A Cerium‐Naphthazarin Catecholate MOF as a Heterogeneous Photocatalyst for Selective Functionalization of Alkanes

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  37. Isolated Cr Active Centers in the Beta Zeolite Framework for Propane Dehydrogenation

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  38. Synergy principle of single active centers and microenvironment for Cr-MFI-catalyzed alkane dehydrogenation

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  39. Local coordination environment of isolated Fe sites in zeolite affects the catalytic performance for propane dehydrogenation

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  40. Activity descriptor and volcano plots in Lewis acid zeolites for dehydrogenation reactions

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  41. Catalysts history, importance, and types

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  42. Entropy−Driven Design Principle of High−Performance Pt−Based Propane Dehydrogenation Catalysts

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  43. Silica‐Supported Mononuclear Methyl‐Platinum Complexes Stabilized by Trimethylphosphine—Synthesis, Structure, and Reactions Under Reducing Conditions

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