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RESEARCH PAPER · Advanced Science · 2021

Integrating Emerging Polymer Chemistries for the Advancement of Recyclable, Biodegradable, and Biocompatible Electronics

Jerika A. Chiong, Helen Tran, Yangju Lin, Yu Qing Zheng, Zhenan Bao

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Integrating Emerging Polymer Chemistries for the Advancement of Recyclable, Biodegradable, and Biocompatible ElectronicsOriginalDesign of biodegradable and biocompatible conjugated polymers for bioelectronics104Emerging electrochemical sensors for life healthcare49A Composite Microfiber for Biodegradable Stretchable Electronics9One-Shot synthesis of heterografted brush copolymers through orthogonal Ring-Opening polymerization and atom transfer radical polymerization3Recent Progress in Materials Chemistry to Advance Flexible Bioelectronics in Medicine132Super‐Hydrophilic Zwitterionic Polymer Surface Modification Facilitates Liquid Transportation of Microfluidic Sweat Sensors33Acrylate and Methacrylate Polymers’ Applications: Second Life with Inexpensive and Sustainable Recycling Approaches57Citric acid-based degradable polyester elastomers coated with silver nanowires for sustainable soft sensors16Design of hydrogel-based wearable EEG electrodes for medical applications78Recyclable thermoset polymers: beyond self-healing3Synthesis of multiple stimuli-responsive degradable block copolymers via facile carbonyl imidazole-induced postpolymerization modification15Impact of Molecular Design on Degradation Lifetimes of Degradable Imine-Based Semiconducting Polymers83Biodegradable Elastomers and Gels for Elastic Electronics131Strategies for body-conformable electronics306Khaya gum – a natural and eco-friendly biopolymer dielectric for low-cost organic field-effect transistors (OFETs)17Tough, transparent, biocompatible and stretchable thermoplastic copolymer with high stability and processability for soft electronics623R Electronics: Scalable Fabrication of Resilient, Repairable, and Recyclable Soft‐Matter Electronics103Environmentally adaptive and durable hydrogels toward multi-sensory application54Microfluidic Invasion Chemotaxis Platform for 3D Neurovascular Co-Culture14Biodegradable Polymer Composites for Electrophysiological Signal Sensing22Biodegradable germanium electronics for integrated biosensing of physiological signals37Mn(II) & Gd(III) deferrioxamine complex contrast agents & temozolomide cancer prodrug immobilized on folic acid targeted graphene/polyacrylic acid nanocarrier: MRI efficiency, drug stability & interactions with cancer cells13PEDOT-NHS as a Versatile Conjugated Polyelectrolyte for Bioelectronics1Flavonoid-based polymeric nanoparticles: A promising approach for cancer and diabetes treatment28Biodegradable polymeric materials for flexible and degradable electronics52Ion-Incorporative, Degradable Nanocellulose Crystal Substrate for Sustainable Carbon-Based Electronics15Stable water-floating transistor with recyclability1Bio-based vitrimeric elastomers enable completely sustainable triboelectric nanogenerator14Fully Recyclable Liquid‐Metal‐Based Multi‐Layer Thermally Triggered Transient Electronic Devices15Mg/Zn metal‐air primary batteries using silk fibroin‐ionic liquid polymer electrolytes4Multifunctional 3D platforms for rapid hemostasis and wound healing: Structural and functional prospects at biointerfaces10Toward Sustainable Wearable Electronic Textiles227Smart Fibers for Self-Powered Electronic Skins162Versatile Poly(3,4-ethylenedioxythiophene) Polyelectrolytes for Bioelectronics by Incorporation of an Activated Ester23Tough, Bio‐disintegrable and Stretchable Substrate Reinforced with Nanofibers for Transient Wearable Electronics32A biocompatible and fully erodible conducting polymer enables implanted rechargeable Zn batteries27Degradable semiconducting polymers without long-range order for on-demand degradation of transient electronics19Tailoring the mechanical properties of benzothiadiazole-based semiconducting polymers through chalcogen atom substitution10The future of electronic materials is…degradable!15Toward a new generation of permeable skin electronics52光遗传学用多功能光纤0脑机接口技术的基础研究：神经元与二极管0Engineering Multi‐Scale Organization for Biotic and Organic Abiotic Electroactive Systems13Natural gums and their derivatives based hydrogels: in biomedical, environment, agriculture, and food industry67Polydimethylsiloxane-coated textiles with minimized microplastic pollution67Biobased, Degradable, and Conjugated Poly(Azomethine)s53Flame-retardant fibre-particle-polymer semiconductive networks for physically transient supercapacitors and chemiresistors11Using Wool Keratin as a Structural Biomaterial and Natural Mediator to Fabricate Biocompatible and Robust Bioelectronic Platforms57Selective Laser Sintering for Electrically Conductive Poly(dimethylsiloxane) Composites with Self-Healing Lattice Structures25Exploration of a Cellulose-Based Biocompatible Gate Dielectric for Low-Voltage Organic Transistors15Fabrication of Eco‐Friendly Wearable Strain Sensor Arrays via Facile Contact Printing for Healthcare Applications29Preparation of PLA / PEG @ SDS microfibers‐based nonwovens via melt‐blown process parameters: Wound dressings with enhanced water wetting performance5Chemically Recyclable Conjugated Polymer and One‐Shot Preparation of Thermally Stable and Efficient Bulk‐Heterojunction from Recycled Monomer24A transparent, self-adhesive and fully recyclable conductive PVA based hydrogel for wearable strain sensor36Applications of flexible electronics related to cardiocerebral vascular system31Robust polyurethane materials with synergistic ionic and metal-ligand crosslinking double networks for specific Cu-ion removal15Advances in Bioresorbable Triboelectric Nanogenerators90Recent Advance in Stretchable Self‐Powered Piezoelectric Sensors: Trends, Challenges, and Solutions17Deamination of Polyols from the Glycolysis of Polyurethane30Sponge-like biodegradable polypyrrole-modified biopolymers for selective adsorption of basic red 46 and crystal violet dyes from single and binary component systems52Direct Arylation Polymerization of Degradable Imine-Based Conjugated Polymers26Recyclable/degradable materials via the insertion of labile/cleavable bonds using a comonomer approach98Circular Polydiketoenamine Elastomers with Exceptional Creep Resistance via Multivalent Cross-Linker Design20Leaf-Inspired Asymmetrically Hierarchical Architecture Engineered Full-Paper Integrated Tactile Array for Ultra-Stable Sensory Augmentation0Towards sustainable, solution-processed organic field-effect transistors using cashew gum as the gate dielectric8Thienoisoindigo-based recyclable conjugated polymers for organic electronics28Magnetically aware actuating composites: Sensing features as inspiration for the next step in advanced magnetic soft robotics17Electrical and Thermal Properties of Polymer Nanocomposites0Block copolymer for skin-compatible electronics1Electronic Plastic (E-plastic) and Their Biodegradation1Polymer design for solid-state batteries and wearable electronics49Printed magnetoresistive sensors for recyclable magnetoelectronics19Polymers and Biopolymers in Sensing2Organic Electrochemical Transistors for Biomarker Detections116Revolutionizing Papertronics: Advanced Green, Tunable, and Flexible Components and Circuits20Carbon-Based Composites with Biodegradable Matrix for Flexible Paper Electronics16Environmentally friendly and degradable organic neuromorphic vision sensors23Design and Development of Transient Sensing Devices for Healthcare Applications45A bio-based, sweat-resistant and markedly sensitive iontronic skin for advancing central sleep apnea monitoring18Hydrogel-Gated FETs in Neuromorphic Computing to Mimic Biological Signal: A Review10An injectable, self-healable, and reusable PEDOT:PSS/PVA hydrogel patch electrode for epidermal electronics59Evolution of Musculoskeletal Electronics12Mechanically Robust Reversibly Cross‐Linked Polymers with Closed‐Loop Recyclability for Use in Flexible Printed Circuit Boards41Development of Degradable Polymers with Controlled Degradation and Applications to Transient Organic Solar Cells7Degradable heteroaromatic polyazomethines for organic field-effect transistor applications6Bulge-Free and Homogeneous Metal Line Jet Printing with StarJet Technology6Skin-inspired soft bioelectronic materials, devices and systems407Metal-organic framework single crystal for in-memory neuromorphic computing with a light control19Wireless Frequency‐Multiplexed Acoustic Array‐Based Acoustofluidics6Challenges in Polymer Recycling1Transparent, Bioelectronic, Natural Polymer AgNW Nanocomposites Inspired by Caviar3A Laminated Strategy Enabled Sustainable Tactile Array with Ultra‐Stable Sensory Augmentation17Electronic skin based on natural biodegradable polymers for human motion monitoring18Modulating the Oxidation Degree of Linear Polyethyleneimine for Preparation of Highly Efficient and Low-cytotoxicity Degradable Gene Delivery Carriers8A Recyclable Ionogel with High Mechanical Robustness Based on Covalent Adaptable Networks56Closing the loop of polyurethane adhesives: Acidolysis process optimization10Highly Stretchable and Breathable Dry Bioelectrode with Low Impedance for Electrophysiological Monitoring17Key Advances in Solution Blow Spinning of Polylactic-Acid-Based Materials: A Prospective Study on Uses and Future Applications17Nanomaterials for Flexible Neuromorphics105Introduction to flexible electronics0Living electronics in cellulose zoogleal mats7Covalent Adaptable Networks for Sustainable Soft Electronic Sensors and Actuators20Electro-ferroelectric characterization of nicotinium tetrachloridocuprate( ii ) memristor for prospective neuromorphic applications0From the synthesis of wearable polymer sensors to their potential for reuse and ultimate fate22Multifunctional high-mobility polymer semiconductors: design, synthesis and applications2Reticular framework materials as versatile platforms for controllable polymer synthesis22Rise of polycatecholamine ultrathin films: From synthesis to smart applications0Sustainable Waste Electrical and Electronics Equipment Recycling in Nigeria, Policies and Emerging Technologies9Ecobuoys for Scalable Oceanography2Liquid-based encapsulation for implantable bioelectronics across broad pH environments28From Printed Devices to Vertically Stacked, 3D Flexible Hybrid Systems40Imine‐Based Polymeric Mixed Ionic–Electronic Conductors Featuring Degradability and Biocompatibility for Transient Bioinspired Electronics24Imine‐Based Polymeric Mixed Ionic–Electronic Conductors Featuring Degradability and Biocompatibility for Transient Bioinspired Electronics0Biodegradable Chitosan-Based Stretchable Electronics with Recyclable Silver Nanowires15Great carbon nano materials based composites for electronic skin: Intelligent sensing, and self-powered nano generators36Technological trajectories in circular economy: Bridging patent analytics with sustainable development goals19Smart Dust for Chemical Mapping14Toward an Internet of Things Circular Economy Using Printed Circuits on Reusable Steel Substrates7Depolymerizable Thermosetting Dielectric Elastomers Toughened by Sacrificial Hydrogen Bonds for Sustainable Capacitive Strain‐Sensor25Design and Development of Biocompatible, Flexible, and Biodegradable Collagen-Based Organic Field-Effect Transistors9432 Chemical recycling of polymer matrix composites0Natural Biopolymer Materials for Flexible Implantable Electronics1Transplacental transfer of p-phenylenediamine antioxidants: Insights from human gestational exposure and an optimized BeWo cell monolayer model5Bioinspired Multi‐Function Conversion Based on Recyclable Phase Change Polymers0Non-volatile resistive switching and electronic synapse based on zinc oxide (ZnO) and perovskites embedded inside a polyvinyl alcohol (PVA) polymer matrix for neuromorphic computing1Utilization of Chitosan as an Excipient in Pharmaceutical Formulations: Systematic Literature Review0Advanced Materials in Responsible Electronics: Innovations for Sustainability, Health, and Circularity13Robust and Biodegradable Heterogeneous Electronics with Customizable Cylindrical Architecture for Interference-Free Respiratory Rate Monitoring13Hybrid living electronic skin for proactive scarless wound healing3Synthesis and Characterization of Itaconic Acid Cross‐Linked Poly(glycerol sebacate) with Enhanced Tunable Elastomeric Properties0A review on the formulation and performance of epoxidized vegetable oil-based vitrimer: stoichiometric calculations, curing agent functionalities and catalyst efficiency6Biorefinery approach for lithium battery waste: Mechanochemical production of GQD membranes and advanced aquaculture wastewater treatment1Synthesis of Degradable Polyimines Through Deborylative Polycondensation0Synthesis of Degradable Polyimines Through Deborylative Polycondensation1Emerging Triboelectric Nanogenerators for In‐Body Implantation5Electrolyte design strategies for next-generation supercapacitors and metal-ion batteries11Recycling soft wearable electronics for circularity and sustainability: From materials to recovery pathways4Evaluating capacitance modulation in conformable few-layer MoS 2 /organic metal–insulator–semiconductor structures0Degradable organic neuromorphic transistors: Emerging progress in optoelectronically co‐reconfigurable devices for sustainable electronics4Bioactive and biodegradable materials for supercapacitors1A Comprehensive Review on Biodegradable Materials and Technologies for Transient Electronics12Sustainable bio-based smart and intelligent composites: A review7Bio-based PEDOT: nanocellulose hybrids as efficient hole-transport layers for photoelectrochemical devices0Catalyst-free polyesterification enables the formation of multifunctional and sustainable polyesters3Intent vs. Practice: A Comparative Study of Sustainable Electronics Perception and Behavior Using Survey and Online Review Data0Noble-metal-free recyclable electronic nanoinks for wireless wearable sensors3Recent trends and the need for organic semiconductors for a sustainable future0Resorbable Polymer Nanocomposites: Current Developments and Future Perspectives0Advances in conductive supramolecular hydrogels for applications in wearable electronics15Integrating natural materials in organic field-effect transistors toward sustainable electronics3

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