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RESEARCH PAPER · Angewandte Chemie International Edition · 2020

Beyond Mechanical Recycling: Giving New Life to Plastic Waste

Ina Vollmer, Michael J. F. Jenks, Mark C. P. Roelands, Robin J. White, Toon van Harmelen, Paul J. de Wild, Gerard P. van der Laan, Florian Meirer, Jos T. F. Keurentjes, Bert Marc Weckhuysen

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Beyond Mechanical Recycling: Giving New Life to Plastic WasteOriginalHighly Efficient Solid‐State Hydrolysis of Waste Polyethylene Terephthalate by Mechanochemical Milling and Vapor‐Assisted Aging137Mechanical Recycling of Packaging Plastics: A Review1639Catalytic upcycling of high-density polyethylene via a processive mechanism524Possibilities and limitations of biotechnological plastic degradation and recycling431Waste Polypropylene Plastic Recycling toward Climate Change Mitigation and Circular Economy: Energy, Environmental, and Technoeconomic Perspectives214Creating value from plastic waste125Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatization879Recycling of multilayer plastic packaging materials by solvent-targeted recovery and precipitation435Towards the Circular Economy: Converting Aromatic Plastic Waste Back to Arenes over a Ru/Nb2O5 Catalyst397Low-energy catalytic methanolysis of poly(ethyleneterephthalate)318100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers280Polyolefin thermoplastic elastomers from polymerization catalysis: Advantages, pitfalls and future challenges326Selective Chemical Upcycling of Mixed Plastics Guided by a Thermally Stable Organocatalyst242Catalytic methods for chemical recycling or upcycling of commercial polymers368Chemolytic depolymerisation of PET: a review704Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Propane to olefins tandem catalysis: a selective route towards light olefins production285Reductive depolymerization as an efficient methodology for the conversion of plastic waste into value-added compounds111Pyrolysis-catalysis of different waste plastics over Fe/Al2O3 catalyst: High-value hydrogen, liquid fuels, carbon nanotubes and possible reaction mechanisms251Plastic recycling in a circular economy; determining environmental performance through an LCA matrix model approach411Tandem Heterogeneous Catalysis for Polyethylene Depolymerization via an Olefin-Intermediate Process166Catalytic processing of plastic waste on the rise613Biocatalysis in the Recycling Landscape for Synthetic Polymers and Plastics towards Circular Textiles116Closed-loop recycling of polyethylene-like materials753H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen127Biodegradation and up-cycling of polyurethanes: Progress, challenges, and prospects248Catalytic Hydrogenation of Polyurethanes to Base Chemicals: From Model Systems to Commercial and End-of-Life Polyurethane Materials131The Chemical Recycling of Polyesters for a Circular Plastics Economy: Challenges and Emerging Opportunities425Plastic Waste Conversion over a Refinery Waste Catalyst173Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Recent Progress in the Chemical Upcycling of Plastic Wastes298Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Deactivation and Regeneration of Zeolite Catalysts Used in Pyrolysis of Plastic Wastes—A Process and Analytical Review172Toward polymer upcycling—adding value and tackling circularity719Upcycling to Sustainably Reuse Plastics301Conversion of Polyethylene Waste into Gaseous Hydrocarbons via Integrated Tandem Chemical–Photo/Electrocatalytic Processes167Enzymatic depolymerization of highly crystalline polyethylene terephthalate enabled in moist-solid reaction mixtures156Progress in the catalytic glycolysis of polyethylene terephthalate238Upcycling and catalytic degradation of plastic wastes332Depolymerization of Hydroxylated Polymers via Light-Driven C–C Bond Cleavage111Thermochemical Recycling of Waste Plastics by Pyrolysis: A Review241Why is Recycling of Postconsumer Plastics so Challenging?381Recent Advancements in Plastic Packaging Recycling: A Mini-Review151A new strategy to prepare fully bio-based poly(lactic acid) composite with high flame retardancy, UV resistance, and rapid degradation in soil179Hydrolysis of waste polyethylene terephthalate catalyzed by easily recyclable terephthalic acid228Plastic waste and its management strategies for environmental sustainability795Recycling of multi-material multilayer plastic packaging: Current trends and future scenarios308Catalytic Amination of Polylactic Acid to Alanine208Innovations to decarbonize materials industries189A review of the plastic value chain from a circular economy perspective279Polyolefins and Polystyrene as Chemical Resources for a Sustainable Future: Challenges, Advances, and Prospects246Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes301Managing Plastic Waste─Sorting, Recycling, Disposal, and Product Redesign636A comprehensive experimental investigation of plastic waste pyrolysis oil quality and its dependence on the plastic waste composition239Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality449The metabolic potential of plastics as biotechnological carbon sources – Review and targets for the future152Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Fermentation for the production of biobased chemicals in a circular economy: a perspective for the period 2022–2050146How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics Recycling398Biodegradation of plastics for sustainable environment256From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Insight into Chemical Recycling of Flexible Polyurethane Foams by Acidolysis145Electro-Reforming Polyethylene Terephthalate Plastic to Co-Produce Valued Chemicals and Green Hydrogen203Green Chemistry, Biocatalysis, and the Chemical Industry of the Future197A review on catalytic pyrolysis of plastic wastes to high-value products533Recyclable, malleable and intrinsically flame-retardant epoxy resin with catalytic transesterification118Assessing the feasibility of chemical recycling via steam cracking of untreated plastic waste pyrolysis oils: Feedstock impurities, product yields and coke formation147Recycling of Plastics in the United States: Plastic Material Flows and Polyethylene Terephthalate (PET) Recycling Processes176Assessment of Performance and Challenges in Use of Commercial Automated Sorting Technology for Plastic Waste165Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Solar thermal catalysis for sustainable and efficient polyester upcycling166Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework116Chemical Recycling of Polystyrene to Valuable Chemicals via Selective Acid-Catalyzed Aerobic Oxidation under Visible Light364Critical advances and future opportunities in upcycling commodity polymers1324Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Rational Design of Chemical Catalysis for Plastic Recycling391Plastic Waste Management Strategies and Their Environmental Aspects: A Scientometric Analysis and Comprehensive Review230Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Photocatalytic Conversion of Plastic Waste: From Photodegradation to Photosynthesis260Preparation and mechanism study of a high efficiency bio-based flame retardant for simultaneously enhancing flame retardancy, toughness and crystallization rate of poly (lactic acid)127Electrocatalytic Valorization of Poly(ethylene terephthalate) Plastic and CO 2 for Simultaneous Production of Formic Acid344Biodegradation of polyethylene and polystyrene: From microbial deterioration to enzyme discovery369Closing the Carbon Loop in the Circular Plastics Economy115Polyethylene Terephthalate (PET) Bottle-to-Bottle Recycling for the Beverage Industry: A Review515Sustainable polymers354Photocatalytic upcycling of poly(ethylene terephthalate) plastic to high-value chemicals149Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Current Prospects for Plastic Waste Treatment163A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry135Pyrolysis technology for plastic waste recycling: A state-of-the-art review481A unified view on catalytic conversion of biomass and waste plastics584Catalytic strategies for upvaluing plastic wastes209Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources130A Highly Dynamic Covalent Polymer Network without Creep: Mission Impossible?183Recyclable and malleable thermosets enabled by activating dormant dynamic linkages196Catalytic deconstruction of waste polyethylene with ethylene to form propylene419Sustainable Design of Structural and Functional Polymers for a Circular Economy159Trash to Treasure: Photoreforming of Plastic Waste into Commodity Chemicals and Hydrogen over MoS 2 -Tipped CdS Nanorods271Mixed plastics waste valorization through tandem chemical oxidation and biological funneling635Microplastic materials in the environment: Problem and strategical solutions201Pyrolysis for plastic waste management: An engineering perspective122Photothermal Catalytic Polyester Upcycling over Cobalt Single‐Site Catalyst129Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Removing microplastics from aquatic environments: A critical review178Using waste poly(vinyl chloride) to synthesize chloroarenes by plasticizer-mediated electro(de)chlorination192Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Progress and perspective for conversion of plastic wastes into valuable chemicals395Sustainable cycloaliphatic polyurethanes: from synthesis to applications170Advancing bio-based materials for sustainable solutions to food packaging130“Functional upcycling” of polymer waste towards the design of new materials226Circularity in polymers: addressing performance and sustainability challenges using dynamic covalent chemistries112Photochemical aerobic upcycling of polystyrene plastics to commodity chemicals using anthraquinone as the photocatalyst117Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210Techno-economic analysis and life cycle assessment of mixed plastic waste gasification for production of methanol and hydrogen139Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Recycling of wind turbine blades through modern recycling technologies: A road to zero waste171Challenges and opportunities of light olefin production via thermal and catalytic pyrolysis of end-of-life polyolefins: Towards full recyclability220Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309How much can chemical recycling contribute to plastic waste recycling in Europe? An assessment using material flow analysis modeling131Enzymes’ Power for Plastics Degradation589Mechanochemical Degradation and Recycling of Synthetic Polymers167A critical review and future perspective of plastic waste recycling165Carbon Deposit Analysis in Catalyst Deactivation, Regeneration, and Rejuvenation252Depolymerization of plastics by means of electrified spatiotemporal heating330Catalytic disconnection of C–O bonds in epoxy resins and composites365Chemical recycling technologies for PVC waste and PVC-containing plastic waste: A review213Electrochemical Production of Glycolate Fuelled By Polyethylene Terephthalate Plastics with Improved Techno‐Economics136A focused review on recycling and hydrolysis techniques of polyethylene terephthalate205Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Designing a circular carbon and plastics economy for a sustainable future489Sustainable polyurethanes: toward new cutting-edge opportunities275Polyethylene terephthalate (PET) recycling: A review355Chemical recycling of plastic waste for sustainable polymer manufacturing – A critical review115Synthesis and Deconstruction of Polyethylene-type Materials194Light-driven polymer recycling to monomers and small molecules112Recyclable and (Bio)degradable Polyesters in a Circular Plastics Economy400Cu Promoted the Dynamic Evolution of Ni-Based Catalysts for Polyethylene Terephthalate Plastic Upcycling140The refinery of the future341Photocatalysis toward Microplastics Conversion: A Critical Review148Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136Designed to Degrade: Tailoring Polyesters for Circularity168Recent Developments in Technology for Sorting Plastic for Recycling: The Emergence of Artificial Intelligence and the Rise of the Robots128Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144Plastic recycling: A panacea or environmental pollution problem314Catalytic Upcycling of Polyolefins316Sustainable Solutions Through Innovative Plastic Waste Recycling Technologies159A comprehensive review of polyurethane: Properties, applications and future perspectives119

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