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RESEARCH PAPER · ACS Macro Letters · 2020

100th Anniversary of Macromolecular Science Viewpoint: Toward Catalytic Chemical Recycling of Waste (and Future) Plastics

Joshua C. Worch, Andrew P. Dove

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100th Anniversary of Macromolecular Science Viewpoint: Toward Catalytic Chemical Recycling of Waste (and Future) PlasticsOriginalSummating potential and action potential ratio in Meniere's disease before and after treatment.26100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers280Catalytic methods for chemical recycling or upcycling of commercial polymers368Capturing ethylene glycol with dimethyl carbonate towards depolymerisation of polyethylene terephthalate at ambient temperature84Estrogenic activity of lignin-derivable alternatives to bisphenol A assessed via molecular docking simulations24Facile fabrication of degradable polyurethane thermosets with high mechanical strength and toughness via the cross-linking of triple boron–urethane bonds79Heterodinuclear catalysts Zn( ii )/M and Mg( ii )/M, where M = Na( i ), Ca( ii ) or Cd( ii ), for phthalic anhydride/cyclohexene oxide ring opening copolymerisation27On the use of catalysis to bias reaction pathways in out-of-equilibrium systems36Photo-crosslinking polymers by dynamic covalent disulfide bonds80Recent developments towards performance-enhancing lignin-based polymers90Synthesis and melt-spinning of partly bio-based thermoplastic poly(cycloacetal-urethane)s toward sustainable textiles28The synthesis of degradable sulfur-containing polymers: precise control of structure and stereochemistry72The chemistry of chemical recycling of solid plastic waste via pyrolysis and gasification: State-of-the-art, challenges, and future directions697Synthesis of polymers containing vicinal tricarbonyl moiety and construction of reversible crosslinking–decrosslinking polymer system4The Chemical Recycling of Polyesters for a Circular Plastics Economy: Challenges and Emerging Opportunities425100th Anniversary of Macromolecular Science Viewpoints21Backbone-Degradable Vinyl Acetate Latex: Coatings for Single-Use Paper Products41Roadmap to Biodegradable Plastics—Current State and Research Needs260Recent Progress in the Chemical Upcycling of Plastic Wastes298Depolymerization of P(PDMS11MA) Bottlebrushes via Atom Transfer Radical Polymerization with Activator Regeneration96Switchable Polymerization Catalysis Using a Tin(II) Catalyst and Commercial Monomers to Toughen Poly( l -lactide)30New sustainable flame retardant DOPO-NH-functionalized polyamide 6 and filament yarn77Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Quantification of PP contamination in recycled PE by TREF analysis for improved the quality and circularity of plastics49Complete Degradation of a Conjugated Polymer into Green Upcycling Products by Sunlight in Air74Toward polymer upcycling—adding value and tackling circularity719Recent Advancements in Photocatalytic Valorization of Plastic Waste to Chemicals and Fuels60Tough and Thermally Recyclable Semiaromatic Polyesters by Ring-Opening Polymerization of Benzo-thia-caprolactones98A green and high-yield route to recycle waste masks into CNTs/Ni hybrids via catalytic carbonization and their application for superior microwave absorption97From Lab to Market: Current Strategies for the Production of Biobased Polyols199Chemically recyclable thermoplastics from reversible-deactivation polymerization of cyclic acetals481Selective degradation of styrene-contained plastics catalyzed by iron under visible light0Why is Recycling of Postconsumer Plastics so Challenging?381Selective Degradation of Styrene‐Related Plastics Catalyzed by Iron under Visible Light**190Catalytic Synergy Using Al(III) and Group 1 Metals to Accelerate Epoxide and Anhydride Ring-Opening Copolymerizations80Reversible-Addition Fragmentation Chain Transfer Step-Growth Polymerization69Design principles for intrinsically circular polymers with tunable properties217Polyolefins and Polyethylene Terephthalate Package Wastes: Recycling and Use in Composites55Metal-Catalyzed Switching Degradation of Vinyl Polymers via Introduction of an “In-Chain” Carbon–Halogen Bond as the Trigger69Alcoholysis of PET catalyzed by bimidazolium cationic zinc acetate deep eutectic solvent4Biobased High-Performance Aromatic–Aliphatic Polyesters with Complete Recyclability188Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis100Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis15Sustainability of Synthetic Plastics: Considerations in Materials Life-Cycle Management92A sustainable approach for the synthesis of recyclable cyclic CO 2 -based polycarbonates56Recent advances in dynamic nuclear polarization-enhanced NMR spectroscopy for organic polymers6Recent progress in ionic liquid-assisted processing and extraction of biopolymers3Reversible addition–fragmentation chain transfer step-growth polymerization with commercially available inexpensive bis-maleimides24Understanding the Structure–Polymerization Thermodynamics Relationships of Fused-Ring Cyclooctenes for Developing Chemically Recyclable Polymers113Simple Approach to Macrocyclic Carbonates with Fast Polymerization Rates and Their Polymer-to-Monomer Regeneration62Sugar-Based Polymers with Stereochemistry-Dependent Degradability and Mechanical Properties60A “Polymer to Polymer” Chemical Recycling of PLA Plastics by the “DE–RE Polymerization” Strategy104Advancing the Development of Recyclable Aromatic Polyesters by Functionalization and Stereocomplexation112Advancing the Development of Recyclable Aromatic Polyesters by Functionalization and Stereocomplexation14Rapid and Controlled Polymerization of Bio‐sourced δ‐Caprolactone toward Fully Recyclable Polyesters and Thermoplastic Elastomers21Rapid and Controlled Polymerization of Bio‐sourced δ‐Caprolactone toward Fully Recyclable Polyesters and Thermoplastic Elastomers137The Frontier of Plastics Recycling: Rethinking Waste as a Resource for High‐Value Applications68A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling32A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling0Redesigned Hybrid Nylons with Optical Clarity and Chemical Recyclability127Mechanically Robust Supramolecular Plastics with Energy-Saving and Highly Efficient Closed-Loop Recyclability56Chemical Upcycling of Poly(bisphenol A carbonate) Plastic Catalyzed by ZnX 2 via an Amino-Alcoholysis Strategy46Zinc-Mediated Allylation-Lactonization One-Pot Reaction to Methylene Butyrolactones: Renewable Monomers for Sustainable Acrylic Polymers with Closed-Loop Recyclability27Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Use of heterogeneous catalysis in sustainable biofuel production2Photocatalytic Conversion of Plastic Waste: From Photodegradation to Photosynthesis260Degradable, Recyclable, Water-Resistant, and Eco-Friendly Poly(vinyl alcohol)-Based Supramolecular Plastics80Unifying Step-Growth Polymerization and On-Demand Cascade Ring-Closure Depolymerization via Polymer Skeletal Editing9Functionalizable and Chemically Recyclable Thermoplastics from Chemoselective Ring‐Opening Polymerization of Bio‐renewable Bifunctional α‐Methylene‐δ‐valerolactone98Functionalizable and Chemically Recyclable Thermoplastics from Chemoselective Ring‐Opening Polymerization of Bio‐renewable Bifunctional α‐Methylene‐δ‐valerolactone11Chemical Upcycling of Poly(3-hydroxybutyrate) into Bicyclic Ether–Ester Monomers toward Value-Added, Degradable, and Recyclable Poly(ether ester)45Sustainable polymers354Catalyst-Free Approach for the Degradation of Bio- and CO2-Sourced Polycarbonates: A Step toward a Circular Plastic Economy15Intrinsically Re-curable Photopolymers Containing Dynamic Thiol-Michael Bonds45Organocatalyzed chemo-selective one-pot upcycling of polyester-block-polycarbonate3Modulating Polymerization Thermodynamics of Thiolactones Through Substituent and Heteroatom Incorporation84Closed-loop chemical recycling of cross-linked polymeric materials based on reversible amidation chemistry4Selective, Sequential, and “One-Pot” Depolymerization Strategies for Chemical Recycling of Commercial Plastics and Mixed Plastics135Polyolefin Innovations toward Circularity and Sustainable Alternatives96A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry135A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry16Analytical and numerical simulations of depolymerization based on discrete model: A chain‐end scission scenario24Breaking C─C Bonds and Preserving C─O Bonds in Aromatic Plastics and Lignin via a Reversing Bond Energy Cleavage Strategy49Simultaneously achieving super toughness and reinforcement of immiscible high-density polyethylene/poly(ethylene terephthalate) composite via oriented spherical crystal structure17Dynamically Cross‐Linking Soybean Oil and Low‐Molecular‐Weight Polylactic Acid toward Mechanically Robust, Degradable, and Recyclable Supramolecular Plastics130Dithioacetal Polymers Capable of Chemical Recycling to Macrocyclic Monomers and Formation of Vitrimers0Structures of the co‐branching reactive products of isotactic polypropylene with high‐density polyethylene and the effect on the in situ compatibilization of mixed recycled materials7Dithioacetal Polymers Capable of Chemical Recycling to Macrocyclic Monomers and Formation of Vitrimers0Novel efficient method of chemical upcycling of waste poly(ethylene terephthalate) bottles by acidolysis with adipic acid under microwave irradiation11Chemical Recycling3Photocycloadditions for the Design of Reversible Photopolymerizations9A circular polyester platform based on simple gem-disubstituted valerolactones175How Dispersity from Step-Growth Polymerization Affects Polymer Dynamics from Coarse-Grained Molecular Simulations12Strong and Tough Supramolecular Covalent Adaptable Networks with Room‐Temperature Closed‐Loop Recyclability222Using waste poly(vinyl chloride) to synthesize chloroarenes by plasticizer-mediated electro(de)chlorination192Chemical recycling and upcycling of poly(Bisphenol A carbonate) via metal acetate catalyzed glycolysis19Well-Defined and Highly Effective Nickel Catalysts Coordinated on Tridentate SNO Schiff-Base Derivatives for Alternating Copolymerization of Epoxides and Anhydrides6Closed-loop chemical recycling of cross-linked polymeric materials based on reversible amidation chemistry158Catalytic Chemical Recycling of Post-Consumer Polyethylene188Rapid and Selective Photo‐degradation of Polymers: Design of an Alternating Copolymer with an o‐Nitrobenzyl Ether Pendant22Rapid and Selective Photo‐degradation of Polymers: Design of an Alternating Copolymer with an o‐Nitrobenzyl Ether Pendant0“Functional upcycling” of polymer waste towards the design of new materials226Chemically recyclable fluorescent polyesters via the ring-opening copolymerization of epoxides and anhydrides11Glycolysis of Polyethylene Glycol Terephthalate Over Cr2o3/Sio2 Catalyst0Imidazolium triflimide-based Brønsted acidic ionic liquid as organocatalyst to trigger the cationic ring-opening polymerization of cyclotrisiloxanes10Recycling waste sources into nanocomposites of graphene materials: Overview from an energy-focused perspective46Selective deconstruction of mixed plastics by a tailored organocatalyst70The advent of recyclable CO 2 -based polycarbonates47Study on the surface properties of the regenerated polyurethane foam micropowder via cryogenic pulverization and its application14Advances in the Synthesis of Chemically Recyclable Polymers50Microplastics toxicity, detection, and removal from water/wastewater71Turning Polyethylene Waste to Hydrocarbons Using a Sustainable Acidic Carbocatalyst5Mechanistic insights into the pyrolysis of poly (vinyl chloride)41Chemical upcycling of poly(lactide) plastic waste to lactate ester, lactide and new poly(lactide) under Mg-catalysis condition32Depolymerization of Polyesters by Transesterification with Ethanol Using (Cyclopentadienyl)titanium Trichlorides19pH‐Responsive and Recyclable Hydrogels for Gas Releasing and Scavenging12Methanol Synthesis Catalyst Waste as the Principal Component of New Sustainable Cementless Concrete0Photoredox-Catalyzed Plastic Waste Conversion: Nonselective Degradation versus Selective Synthesis110Trends in Polyester Upcycling for Diversifying a Problematic Waste Stream50Study on zinc oxide‐creatinine hybrid catalyst for efficient lactide synthesis with low racemization6Enzymes’ Power for Plastics Degradation589Ring-Opening Polymerization of a Seven-Membered Lactone toward a Biocompatible, Degradable, and Recyclable Semi-aromatic Polyester60Chemically Recyclable Dithioacetal Polymers via Reversible Entropy‐Driven Ring‐Opening Polymerization**5Chemically Recyclable Dithioacetal Polymers via Reversible Entropy‐Driven Ring‐Opening Polymerization**66Recent Advances in Catalytic Chemical Recycling of Polyolefins104Personal protective equipment and micro-nano plastics: A review of an unavoidable interrelation for a global well-being hazard23TM-Free and TM-Catalyzed Mechanosynthesis of Functional Polymers9Ultra-High-Molecular-Weight Poly(Dioxolane): Enhancing the Mechanical Performance of a Chemically Recyclable Polymer95One‐Pot Synthesis of Depolymerizable δ‐Lactone Based Vitrimers49Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance63Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance4Preparation of high-molecular-weight polylactide by ring-opening polymerization of l-lactide using base/bisurea binary organocatalyst4Recycling of both resin and fibre from wind turbine blade waste via small molecule-assisted dissolution54Alkane metathesis over immobilized pincer-ligated iridium complexes: Effect of support nature4Chemically recyclable copolyesters from bio-renewable monomers: controlled synthesis and composition-dependent applicable properties50Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Dynamic Covalent Adaptable Polyimide Hybrid Dielectric Films with Superior Recyclability86Eco-friendly passive radiative cooling using recycled packaging plastics21Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Crystalline Stereoregular Poly(ether-ester) via MeAl[Salen]-Catalyzed Well-Controlled Ring-Opening Polymerization of Enantiopure Cyclic Ether-Ester Monomer22A facile alternative strategy of upcycling mixed plastic waste into vitrimers43Bulk depolymerization of poly(methyl methacrylate) via chain-end initiation for catalyst-free reversion to monomer142Ionic Liquid‐Assisted Depolymerization of Condensation Polymers: A Review18Understanding Alkali Cation-Assisted Ring-Opening Polymerization of Macrocyclic Carbonate: Kinetics and Thermodynamics4Regulating cationic polymerization: From structural control to life cycle management51Chemical Upcycling of PET into a Morpholine Amide as a Versatile Synthetic Building Block27Closed-Loop Recyclable Vinylogous Carbamothioate-Based Covalent Adaptable Networks28Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Elucidating the Effect of Amine Charge State on Poly(β-amino ester) Degradation Using Permanently Charged Analogs11Synthesis of High Molecular Weight Biobased Aliphatic Polyesters Exhibiting Tensile Properties Beyond Polyethylene25

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