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RESEARCH PAPER · Chem Catalysis · 2021

Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalyst

Chuhua Jia, Shaoqu Xie, Wanli Zhang, Nadia N. Intan, Janani Sampath, Jim Pfaendtner, Hongfei Lin

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Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalystOriginalSachet Economy: Big Problems in Small Packets20Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123A novel process for the upcycling of waste polyolefins to high-value fuels and chemicals2Upcycling and catalytic degradation of plastic wastes332Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Degradation of sulfonated polyethylene by a bio-photo-fenton approach using glucose oxidase immobilized on titanium dioxide65Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Towards low-temperature catalysts for sustainable fuel from plastic: A review20Catalytic production of diesel-like oils from plastic wastes6Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst42Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions44Catalytic cascade vapor-phase hydrotreatment of plastic waste into fuels and its sustainability assessment18Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Polyethylene Upcycling to Fuels: Narrowing the Carbon Number Distribution in N-Alkanes by Tandem Hydropyrolysis/Hydrocracking56The reductive catalytic upcycling of polyolefin plastic waste17TOWARDS A CIRCULAR ECONOMY: LIQUID-FED FAST PYROLYSIS OF WASTE POLYOLEFIN PLASTICS1From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Catalytic carbon and hydrogen cycles in plastics chemistry78The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Upgrading of polyethylene to hydrocarbon fuels over the Fe-modified Pt/Al2O3 catalysts at a mild condition without external H245Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of Polyolefins49Solar-driven catalytic plastic upcycling87Solvothermal liquefaction of waste polyurethane using supercritical toluene in presence of noble metal catalysts14Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts143Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Current progress in thermochemical conversion of plastics into jet-fuel hydrocarbons and recommendations for COVID-19 waste management25A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Low-temperature upcycling of PET waste into high-purity H2 fuel in a one-pot hydrothermal system with in situ CO2 capture33Catalytic pyrolysis of high-density polyethylene over nickel-waste chicken eggshell/HZSM-523RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Upcycling plastic waste into high value-added chemicals under mild conditions1Photothermal Catalytic Polyester Upcycling over Cobalt Single‐Site Catalyst129Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Pyrolytic Depolymerization Mechanisms for Post-Consumer Plastic Wastes22Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Efficient H 2 Production from PET Plastic Wastes over Mesoporous Carbon-Supported Ru-ZnO Catalysts in a Mild Pure-Water System32“Functional upcycling” of polymer waste towards the design of new materials226Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Closing carbon and nitrogen cycles and addressing a critical global challenge: From seafood waste to sustainable chemicals14Catalytic degradation of microplastics21Conversion of Polyethylene to High-Yield Fuel Oil at Low Temperatures and Atmospheric Initial Pressure6Solid waste biomass as a potential feedstock for producing sustainable aviation fuel: A systematic review174Strategic use of thermo-chemical processes for plastic waste valorization23Chemical recycling of plastic waste as a mean to implement the circular economy model in the European Union51Recent Advances in Catalytic Chemical Recycling of Polyolefins104Assembly strategies for polyethylene-degrading microbial consortia based on the combination of omics tools and the “Plastisphere”34Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR25Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101A two-stage strategy for upcycling chlorine-contaminated plastic waste141Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Catalytic cracking of low-density polyethylene dissolved in various solvents: product distribution and coking behavior9Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Upcycling of polyvinyl chloride to hydrocarbon waxes via dechlorination and catalytic hydrogenation50Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Ni-catalyzed carbon–carbon bonds cleavage of mixed polyolefin plastics waste42Chemical recycling of polyolefins: a closed-loop cycle of waste to olefins126Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Catalytic microwave-assisted pyrolysis of plastic waste to produce naphtha for a circular economy35Effect of Hydrogen Spillover on the Ru/TiO2-Catalyzed Guaiacol Hydrodeoxygenation: Rutile vs Anatase TiO2100Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Dual-Doped Nickel Sulfide for Electro-Upgrading Polyethylene Terephthalate into Valuable Chemicals and Hydrogen Fuel130Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Quantitative analyses of products and rates in polyethylene depolymerization and upcycling11Visualizing the Structure, Composition and Activity of Single Catalyst Particles for Olefin Polymerization and Polyolefin Decomposition16Visualizing the Structure, Composition and Activity of Single Catalyst Particles for Olefin Polymerization and Polyolefin Decomposition2Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Economic feasibility of catalytic cracking of polymer waste for fuel production0Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26End-of-Life Plastics Management: A Review7Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Thermodynamic and Kinetic Insights into Hydrogen Adsorption and Dissociation on the Ru (0001) Surface under STM and Catalytic Conditions11Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture17Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins39Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38A multiscale investigation of polypropylene glycol polymer upcycling to propionaldehyde via catalytic cracking on acid sites of mesoporous Y zeolites2Direct amination of poly( p -phenylene oxide) to substituted anilines over bimetallic Pd–Ru catalysts13Recycling tendencies in plastic waste management for environmental sustainability1Sustainable management and diversification of problematic wastes: prospects and challenges1Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Depolymerization of Plastic Waste2Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27A state-of-the-art review of multilayer packaging recycling: Challenges, alternatives, and outlook150High-purity H2 production from mixed PVC/PET plastic wastes through tandem hydrothermal depolymerization and aqueous phase reforming9Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Solvent-Regulated Tandem Oxidative Degradation of Polyethylene to Multifunctional Chemicals17Hydrogenolysis of Poly(Ethylene‐co‐Vinyl Alcohol) and Related Polymer Blends over Ruthenium Heterogeneous Catalysts7Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6Complete hydrogenolysis of mixed plastic wastes101Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264Innovative carbon nanotubes-bridging strategy valorizes plastic waste into high-quality H2-rich syngas while suppressing CO2 emissions21Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Coupling pyrolysis and catalytic reforming of waste plastics for syngas production over confined Ni within silicalite-1 catalysts5Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst12Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Synthesis of biosurfactants from polyethylene waste via an integrated chemical and biological process3Efficient Photolytic Breakdown of Waste Polystyrene Foam Using an “All-in-One” Photo-HAT Reagent at Ambient Conditions21Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Chemical recycling of post-consumer polyester wastes using a tertiary amine organocatalyst9Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Selective Hydrogenolysis Conversion of Polyethylene into Alkyl Oil Over Iridium‐based Catalyst9Catalytic recycling of plastics into value-added products28Effect of CeO2 morphology and Ru impregnation method on CH4 selectivity reduction in polyethylene waste conversion to liquid fuels and lubricants15Efficient polycarbonate plastic upcycling into jet fuel cycloalkanes over a bifunctional MoCo/NiC hetero-catalyst12Roles of carbon dioxide in the conversion of biomass or waste plastics8Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Plasmonic Copper‐Ruthenium Superstructure for Efficient Photothermal Conversion and Plastic Recycling39Hydroconversion of waste polyethylene plastics under mild conditions using mechanically mixed bifunctional catalysts: Impact of metal-acid balance and proximity9Upcycling of Plastic Waste0Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2

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  5. Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes

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  6. Degradation of sulfonated polyethylene by a bio-photo-fenton approach using glucose oxidase immobilized on titanium dioxide

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  40. Catalytic pyrolysis of high-density polyethylene over nickel-waste chicken eggshell/HZSM-5

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  41. RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts

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  42. Upcycling plastic waste into high value-added chemicals under mild conditions

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  43. Photothermal Catalytic Polyester Upcycling over Cobalt Single‐Site Catalyst

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  45. Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism

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  46. Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy

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  47. Pyrolytic Depolymerization Mechanisms for Post-Consumer Plastic Wastes

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