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RESEARCH PAPER · JACS Au · 2020

Conversion of Polyolefin Waste to Liquid Alkanes with Ru-Based Catalysts under Mild Conditions

Julie E. Rorrer, Gregg T. Beckham, Yuriy Román‐Leshkov

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Conversion of Polyolefin Waste to Liquid Alkanes with Ru-Based Catalysts under Mild ConditionsOriginalCatalytic Hydrogenolysis of Polyolefins into Alkanes46Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Probing β-alkyl elimination and selectivity in polyolefin hydrogenolysis through DFT17Catalytic carbon-carbon bond cleavage and carbon-element bond formation give new life for polyolefins as biodegradable surfactants81Breaking C–C Bonds via Electrochemically Mediated Hydrogen Atom Transfer Reactions1Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalyst208Recent Progress in the Chemical Upcycling of Plastic Wastes298Spontaneous Electric Fields Play a Key Role in Thermochemical Catalysis at Metal−Liquid Interfaces81Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts262Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Chemical and biological catalysis for plastics recycling and upcycling1198Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Recent Advancements in Plastic Packaging Recycling: A Mini-Review151Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Towards a Plastic Circular Economy: Bio-derived Plastics and their End-of-life Strategies6Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts82Catalytic Amination of Polylactic Acid to Alanine208International Open Access Week and JACS Au1Towards low-temperature catalysts for sustainable fuel from plastic: A review20Design principles for intrinsically circular polymers with tunable properties217Polyolefins and Polyethylene Terephthalate Package Wastes: Recycling and Use in Composites55Managing Plastic Waste─Sorting, Recycling, Disposal, and Product Redesign636Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst42Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions44Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer Reactions63Assessment of acidity and the zeolite porous structure on hydrocracking of HDPE30Catalytic cascade vapor-phase hydrotreatment of plastic waste into fuels and its sustainability assessment18Catalytic conversion of SPW and products upgrading9Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Polyethylene Upcycling to Fuels: Narrowing the Carbon Number Distribution in N-Alkanes by Tandem Hydropyrolysis/Hydrocracking56Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution22The reductive catalytic upcycling of polyolefin plastic waste17TOWARDS A CIRCULAR ECONOMY: LIQUID-FED FAST PYROLYSIS OF WASTE POLYOLEFIN PLASTICS1Synthesis–Structure–Activity Relationship in Cu-MOR for Partial Methane Oxidation: Al Siting via Inorganic Structure-Directing Agents18Synthesis and Characterization of Mesoporous Silica Nanoparticles Loaded with Pt Catalysts22Non-thermal plasma-assisted rapid hydrogenolysis of polystyrene to high yield ethylene76Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Catalytic carbon and hydrogen cycles in plastics chemistry78A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling32A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling0The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Trendbericht Technische Chemie 20224Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Artificial enzymic architecture for catalytic polyolefin upcycling3Reactive Molecular Dynamics Simulations of the Depolymerization of Polyethylene Using Graphene-Oxide-Supported Platinum Nanoparticles12Biodegradation of polyethylene and polystyrene: From microbial deterioration to enzyme discovery369Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling32Unleashing the Power of Knowledge Extraction from Scientific Literature in Catalysis27Innovations Toward the Valorization of Plastics Waste65Chemical Recycling of Polyethylene by Tandem Catalytic Monomerization to Propylene0Polyolefin Innovations toward Circularity and Sustainable Alternatives96A unified view on catalytic conversion of biomass and waste plastics584Cascade degradation and upcycling of polystyrene waste to high-value chemicals113Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts143Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Chemical Recycling of Polyethylene by Tandem Catalytic Conversion to Propylene259Recycling and Upgrading Utilization of Polymer Plastics †34RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Upcycling disposable face masks into fuel range iso-alkanes through hydropyrolysis coupled with vapor-phase hydrocracking13JACS Au and International Open Access Week 20220Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Cascade upcycling polystyrene waste into ethylbenzene over Fe2N @ C42Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Fundamental, application and opportunities of single atom catalysts for Li-S batteries155Progress and perspective for conversion of plastic wastes into valuable chemicals395Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Polyethylene in Dead-End Silica Nanopores: Forces and Mobility from Non-Equilibrium Statistical Mechanics and Exchange Spectroscopy Nuclear Magnetic Resonance6Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Co-pyrolysis of pinewood and HDPE: pyrolysis characteristics and kinetic behaviors study11Converting plastic waste to fuel and fine chemicals5Functionalization of polyethylene with hydrolytically-stable ester groups6Heterogeneous Pt-catalyzed transfer dehydrogenation of long-chain alkanes with ethylene7Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Sustainable production of styrene from catalytic recycling of polystyrene over potassium promoted Fe–Al 2 O 3 catalyst13Turning Polyethylene Waste to Hydrocarbons Using a Sustainable Acidic Carbocatalyst5Catalytic degradation of microplastics21Polyethylene Valorization by Combined Chemical Catalysis with Bioconversion by Plastic-Enriched Microbial Consortia26Ultrasmall amorphous zirconia nanoparticles catalyse polyolefin hydrogenolysis176Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene38Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Strategic use of thermo-chemical processes for plastic waste valorization23Analysis of the Scale of Global Human Needs and Opportunities for Sustainable Catalytic Technologies42Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways31Machine Learning and Informatics Based Elucidation of Reaction Pathways for Upcycling Model Polyolefin to Aromatics11Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Enhanced degradation of polyethylene terephthalate plastics by CdS/CeO2 heterojunction photocatalyst activated peroxymonosulfate143Microwave‐Assisted Synthesis of SrTiO3 Nanocuboids without TiCl46Sustainable catalytic strategies for the transformation of plastic wastes into valued products53Techno-Economic and Life Cycle Analyses of Thermochemical Upcycling Technologies of Low-Density Polyethylene Waste116Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Toward a unified metric of catalyst comparison in polymer hydrogenolysis3Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Mechanocatalytic Oxidative Cracking of Poly(ethylene) Via a Heterogeneous Fenton Process38Upcycling waste polycarbonate plastics into jet fuels over NiCo/C by catalytic tandem hydropyrolysis/hydrodeoxygenation31Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process7Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process73Zeolite Supported Pt for Depolymerization of Polyethylene by Induction Heating18Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47Retrieving back plastic wastes for conversion to value added petrochemicals: opportunities, challenges and outlooks86Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Deconvoluting the roles of polyolefin branching and unsaturation on depolymerization reactions over acid catalysts34Ab Initio Thermochemistry of Highly Flexible Molecules for Thermal Decomposition Analysis22Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide4A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina23Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Heterogenous electromediated depolymerization of highly crystalline polyoxymethylene43Upcycling of non-biodegradable plastics by base metal photocatalysis115Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Circular plastics technologies: open loop recycling of waste plastics into new chemicals0Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Transition Metal Catalysts for Depolymerization0Conversion of polyethylene to gasoline: Influence of porosity and acidity of zeolites14Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8

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  46. Trendbericht Technische Chemie 2022

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  49. Rational Design of Chemical Catalysis for Plastic Recycling

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  50. Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review

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