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RESEARCH PAPER · Science Advances · 2021

Plastic waste to fuels by hydrocracking at mild conditions

Sibao Liu, Pavel A. Kots, Brandon C. Vance, Andrew Danielson, Dionisios G. Vlachos

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Plastic waste to fuels by hydrocracking at mild conditionsOriginalNanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts262The Power of the United Nations Sustainable Development Goals in Sustainable Chemistry and Engineering Research72Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Upcycling and catalytic degradation of plastic wastes332Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Thermochemical Recycling of Waste Plastics by Pyrolysis: A Review241Why is Recycling of Postconsumer Plastics so Challenging?381Recent Advancements in Plastic Packaging Recycling: A Mini-Review151Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Catalytic Amination of Polylactic Acid to Alanine208Conversion of plastic waste into fuels: A critical review177Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes301Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Controlling Nucleation Pathways in Zeolite Crystallization: Seeding Conceptual Methodologies for Advanced Materials Design155Catalytic hydrocracking of heavy wax from pyrolysis of plastic wastes using Pd/Hβ for naphtha-ranged hydrocarbon production44A sustainable approach for the synthesis of recyclable cyclic CO 2 -based polycarbonates56Antioxidant-induced transformations of a metal-acid hydrocracking catalyst in the deconstruction of polyethylene waste69Co-Pyrolysis Behaviors of Coal and Polyethylene by Combining In-Situ Py-Tof-Ms and Reactive Molecular Dynamics50Conversion of plastic waste into high-value lubricants: techno-economic analysis and life cycle assessment73Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Plastic Waste Upgrade to Olefins Via Mild Slurry Microwave Pyrolysis Over Solid Acids71Polyethylene Upcycling to Fuels: Narrowing the Carbon Number Distribution in N-Alkanes by Tandem Hydropyrolysis/Hydrocracking56Upcycling waste polyvinyl chloride: One-pot synthesis of valuable carbon materials and pipeline-quality syngas via pyrolysis in a closed reactor70From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Recent Progress on Sulfated Nanozirconia as a Solid Acid Catalyst in the Hydrocracking Reaction55Catalytic carbon and hydrogen cycles in plastics chemistry78Upgrading waste plastic derived pyrolysis gas via chemical looping cracking–gasification using Ni–Fe–Al redox catalysts70Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Rational Design of Chemical Catalysis for Plastic Recycling391Upgrading of polyethylene to hydrocarbon fuels over the Fe-modified Pt/Al2O3 catalysts at a mild condition without external H245Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Recycled (Bio)Plastics and (Bio)Plastic Composites: A Trade Opportunity in a Green Future51Transformation of Biopharmaceutical Manufacturing Through Single-Use Technologies: Current State, Remaining Challenges, and Future Development54Innovations Toward the Valorization of Plastics Waste65Removal of microplastics and nanoplastics from urban waters: Separation and degradation164Solar-driven catalytic plastic upcycling87Catalytic reforming of polyethylene pyrolysis vapors to naphtha range hydrocarbons with low aromatic content over a high silica ZSM-5 zeolite57Coking-Resistant Polyethylene Upcycling Modulated by Zeolite Micropore Diffusion271Pyrolysis technology for plastic waste recycling: A state-of-the-art review481Microwave-initiated MAX Ti3AlC2-catalyzed upcycling of polyolefin plastic wastes: Selective conversion to hydrogen and carbon nanofibers for sodium-ion battery68A unified view on catalytic conversion of biomass and waste plastics584Upcycling of Plastic Wastes and Biomass for Sustainable Graphitic Carbon Production: A Critical Review72Breaking C─C Bonds and Preserving C─O Bonds in Aromatic Plastics and Lignin via a Reversing Bond Energy Cleavage Strategy49Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts143Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Plastic Waste Recycling, Applications, and Future Prospects for a Sustainable Environment142Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Microplastic materials in the environment: Problem and strategical solutions201Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Sustainable Conversion of Microplastics to Methane with Ultrahigh Selectivity by a Biotic–Abiotic Hybrid Photocatalytic System111Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Process Simulation and Life Cycle Assessment of Waste Plastics: A Comparison of Pyrolysis and Hydrocracking50Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Progress and perspective for conversion of plastic wastes into valuable chemicals395Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes59Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Defective nickel sulfide hierarchical structures for efficient electrochemical conversion of plastic waste to value-added chemicals and hydrogen fuel69Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210A comprehensive review of sustainable approaches for synthetic lubricant components67Ti–Fe2O3/Ni(OH) as an efficient and durable photoanode for the photoelectrochemical catalysis of PET plastic to formic acid64Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Engineering nanoscale H supply chain to accelerate methanol synthesis on ZnZrOx136Challenges and opportunities of light olefin production via thermal and catalytic pyrolysis of end-of-life polyolefins: Towards full recyclability220Ultrasmall amorphous zirconia nanoparticles catalyse polyolefin hydrogenolysis176Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Valorization of waste biodegradable polyester for methyl methacrylate production111A Thermo-Catalytic Pyrolysis of Polystyrene Waste Review: A Systematic, Statistical, and Bibliometric Approach48Recent Advances in Catalytic Chemical Recycling of Polyolefins104Molecular Views on Mechanisms of Brønsted Acid-Catalyzed Reactions in Zeolites244Sustainable catalytic strategies for the transformation of plastic wastes into valued products53Waste to energy: Trends and perspectives71Depolymerization of plastics by means of electrified spatiotemporal heating330Techno-Economic and Life Cycle Analyses of Thermochemical Upcycling Technologies of Low-Density Polyethylene Waste116Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Chemical recycling technologies for PVC waste and PVC-containing plastic waste: A review213Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47Retrieving back plastic wastes for conversion to value added petrochemicals: opportunities, challenges and outlooks86Plastic Recycling: A Review on Life Cycle, Methods, Misconceptions, and Techno‐Economic Analysis60Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Recent advances in plastic waste pyrolysis for liquid fuel production: Critical factors and machine learning applications69Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113A two-stage strategy for upcycling chlorine-contaminated plastic waste141Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Review and recommendations for sustainable pathways of recycling commodity plastic waste across different economic regions51Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants349From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Toward Intrinsic Catalytic Rates and Selectivities of Zeolites in the Presence of Limiting Diffusion and Deactivation50Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering55Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Chemically recyclable polyolefin-like multiblock polymers201Microplastic removal and management strategies for wastewater treatment plants160Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Rational design principles of single-atom catalysts for hydrogen production and hydrogenation58Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Recent advances in liquid fuel production from plastic waste via pyrolysis: Emphasis on polyolefins and polystyrene59Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Highly Selective Upgrading of Polyethylene into Light Aromatics via a Low-Temperature Melting-Catalysis Strategy55Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45A review on value-addition to plastic waste towards achieving a circular economy76Synthesis and Deconstruction of Polyethylene-type Materials194Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166Complete hydrogenolysis of mixed plastic wastes101Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264Catalytic Consequences of Hierarchical Pore Architectures within MFI and FAU Zeolites for Polyethylene Conversion54A review on liquid fuel produced from microwave-assisted pyrolysis of plastic waste48Microwave‐Assisted Pyrolysis‐A New Way for the Sustainable Recycling and Upgrading of Plastic and Biomass: A Review46Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Recycling polyolefin plastic waste at short contact times via rapid joule heating93Electrocatalytic upcycling of plastic waste: Progress, challenges, and future53Catalytic Upcycling of Polyolefins316Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Plastic recycling: Challenges and opportunities88Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Current methods for plastic waste recycling: Challenges and opportunities64Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Circular plastic economy for sustainable development: current advances and future perspectives49Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Catalytic Upgrading of Plastic Wastes into High-Value Carbon Nanomaterials: Synthesis and Applications59Co-recycling of plastics and other waste materials70In-line NMR guided orthogonal transformation of real-life plastics63High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65A review of the pathways, limitations, and perspectives of plastic waste recycling46

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