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RESEARCH PAPER · Science · 2020

Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatization

Fan Zhang, Manhao Zeng, Ryan D. Yappert, Jia‐Kai Sun, Yu-Hsuan Lee, Anne M. LaPointe, Baron Peters, Mahdi M. Abu‐Omar, Susannah L. Scott

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Polyethylene upcycling to long-chain alkylaromatics by tandem hydrogenolysis/aromatizationOriginalCreating value from plastic waste125100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers280Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Tandem In 2 O 3 -Pt/Al 2 O 3 catalyst for coupling of propane dehydrogenation to selective H 2 combustion309Catalytic pyrolysis of plastic wastes in a continuous microwave assisted pyrolysis system for fuel production309Catalytic carbon-carbon bond cleavage and carbon-element bond formation give new life for polyolefins as biodegradable surfactants81Plastic waste to fuels by hydrocracking at mild conditions577Microplastics release from victuals packaging materials during daily usage81Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalyst208Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Recent Progress in the Chemical Upcycling of Plastic Wastes298Spontaneous Electric Fields Play a Key Role in Thermochemical Catalysis at Metal−Liquid Interfaces81Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts262Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Complete Degradation of a Conjugated Polymer into Green Upcycling Products by Sunlight in Air74Chemical aspects of polymer recycling128IsPETase- and IsMHETase-Catalyzed Cascade Degradation Mechanism toward Polyethylene Terephthalate81Chemical and biological catalysis for plastics recycling and upcycling1198Upcycling and catalytic degradation of plastic wastes332Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Depolymerization of Hydroxylated Polymers via Light-Driven C–C Bond Cleavage111Chemically recyclable thermoplastics from reversible-deactivation polymerization of cyclic acetals481Electrocatalytic upcycling of polyethylene terephthalate to commodity chemicals and H2 fuel768MIXed plastics biodegradation and UPcycling using microbial communities: EU Horizon 2020 project MIX-UP started January 202070Why is Recycling of Postconsumer Plastics so Challenging?381Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Achieving net-zero greenhouse gas emission plastics by a circular carbon economy579Catalytic Amination of Polylactic Acid to Alanine208Chemical Upcycling of Polyethylene to Value-Added α,ω-Divinyl-Functionalized Oligomers92Polyolefins and Polystyrene as Chemical Resources for a Sustainable Future: Challenges, Advances, and Prospects246Design principles for intrinsically circular polymers with tunable properties217Managing Plastic Waste─Sorting, Recycling, Disposal, and Product Redesign636Sustainable Bioplastic Made from Biomass DNA and Ionomers103Towards high-performance sustainable polymers via isomerization-driven irreversible ring-opening polymerization of five-membered thionolactones177From plastic waste to wealth using chemical recycling: A review300Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality101Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality449Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Upcycling waste polyvinyl chloride: One-pot synthesis of valuable carbon materials and pipeline-quality syngas via pyrolysis in a closed reactor70From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269A review on catalytic pyrolysis of plastic wastes to high-value products533Photoreforming of plastic waste poly (ethylene terephthalate) via in-situ derived CN-CNTs-NiMo hybrids178Highly efficient electrocatalytic hydrogen evolution coupled with upcycling of microplastics in seawater enabled via Ni3N/W5N4 janus nanostructures166Non-thermal plasma-assisted rapid hydrogenolysis of polystyrene to high yield ethylene76Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Catalytic carbon and hydrogen cycles in plastics chemistry78Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Critical advances and future opportunities in upcycling commodity polymers1324Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Computer-designed repurposing of chemical wastes into drugs86The future of green energy and chemicals: Rational design of catalysis routes129Biodegradation of polyethylene and polystyrene: From microbial deterioration to enzyme discovery369Converting waste PET plastics into automobile fuels and antifreeze components260Sustainable polymers354Integrated strategy for the synthesis of aromatic building blocks via upcycling of real-life plastic wastes142Bridging Plastic Recycling and Organic Catalysis: Photocatalytic Deconstruction of Polystyrene via a C–H Oxidation Pathway211Maximizing noble metal utilization in solid catalysts by control of nanoparticle location242Distance for Communication between Metal and Acid Sites for Syngas Conversion108End-of-Life Management Options for Agricultural Mulch Films in the United States—A Review72Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Coking-Resistant Polyethylene Upcycling Modulated by Zeolite Micropore Diffusion271Environmental toxicity and decomposition of polyethylene286Pyrolysis technology for plastic waste recycling: A state-of-the-art review481First-Generation Organic Reaction Intermediates in Zeolite Chemistry and Catalysis107A unified view on catalytic conversion of biomass and waste plastics584Catalytic oxidation of polystyrene to aromatic oxygenates over a graphitic carbon nitride catalyst260Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Catalytic strategies for upvaluing plastic wastes209Catalytic deconstruction of waste polyethylene with ethylene to form propylene419Chemical Recycling of Polyethylene by Tandem Catalytic Conversion to Propylene259Bio-oil and biochar from the pyrolytic conversion of biomass: A current and future perspective on the trade-off between economic, environmental, and technical indicators144RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Recycling plastic using a hybrid process70Microplastic materials in the environment: Problem and strategical solutions201A circular polyester platform based on simple gem-disubstituted valerolactones175Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Degradation of low density polyethylene by Bacillus species85Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Catalytic Chemical Recycling of Post-Consumer Polyethylene188Recent advances in plastic recycling and upgrading under mild conditions147Recent development of end-of-life strategies for plastic in industry and academia: bridging their gap for future deployment72Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Review of polymer technologies for improving the recycling and upcycling efficiency of plastic waste271Electrocatalytic Upcycling of Biomass and Plastic Wastes to Biodegradable Polymer Monomers and Hydrogen Fuel at High Current Densities540Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Valorization of waste biodegradable polyester for methyl methacrylate production111Recent Advances in Catalytic Chemical Recycling of Polyolefins104Electrical Pulse‐Driven Periodic Self‐Repair of Cu‐Ni Tandem Catalyst for Efficient Ammonia Synthesis from Nitrate211Dynamic crosslinking compatibilizes immiscible mixed plastics245Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process73Acetolysis of waste polyethylene terephthalate for upcycling and life-cycle assessment study205Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113A two-stage strategy for upcycling chlorine-contaminated plastic waste141Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers94Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants349Upcycling of non-biodegradable plastics by base metal photocatalysis115From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Co-upcycling of polyvinyl chloride and polyesters199Chemically recyclable polyolefin-like multiblock polymers201Catalytic depolymerization of polyester plastics toward closed-loop recycling and upcycling127Removal of polyethylene terephthalate plastics waste via Co–CeO2 photocatalyst–activated peroxymonosulfate strategy91Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Photocatalytic production of ethylene and propionic acid from plastic waste by titania-supported atomically dispersed Pd species112Characterization of polymer properties and identification of additives in commercially available research plastics112Fundamental, technical and environmental overviews of plastic chemical recycling88Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Leveraging mechanochemistry for sustainable polymer degradation87Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Tandem Chemical Depolymerization and Photoreforming of Waste PET Plastic to High-Value-Added Chemicals148Circular olefin copolymers made de novo from ethylene and α-olefins83A review on value-addition to plastic waste towards achieving a circular economy76Synthesis and Deconstruction of Polyethylene-type Materials194Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Light-driven polymer recycling to monomers and small molecules112Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166Coupling Waste Plastic Upgrading and CO 2 Photoreduction to High-Value Chemicals by a Binuclear Re–Ru Heterogeneous Catalyst77Complete hydrogenolysis of mixed plastic wastes101Nano/micro-plastic, an invisible threat getting into the brain73In-situ catalytic pyrolysis of polyethylene to co-produce BTX aromatics and H2 by Ni/ZSM-5 in the rotary reactor with solid heat carriers70Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions102Designed to Degrade: Tailoring Polyesters for Circularity168Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Upcycling of Polyolefins316Polyolefin waste to light olefins with ethylene and base-metal heterogeneous catalysts151Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Perspectives on Plastic Waste Management: Challenges and Possible Solutions to Ensure Its Sustainable Use108Plastic recycling: Challenges and opportunities88Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100State-of-the-art and perspectives of hydrogen generation from waste plastics80Advanced Catalysts for the Chemical Recycling of Plastic Waste90Incorporating Ordered Indium Sites into Rhodium for Ultra‐Low Potential Electrocatalytic Conversion of Ethylene Glycol to Glycolic Acid71Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73

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