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RESEARCH PAPER · Materials Horizons · 2020

Catalytic methods for chemical recycling or upcycling of commercial polymers

Sophia C. Kosloski-Oh, Zachary A. Wood, Yvonne Manjarrez, Juan Pablo de los Rios, Megan E. Fieser

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Catalytic methods for chemical recycling or upcycling of commercial polymersOriginalNanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Plastic waste to drug intermediate: targeted cleavage of C–O bonds in polyphenylene oxide to 3,5-dimethyl phenol31H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen127Catalytic Hydrogenation of Polyurethanes to Base Chemicals: From Model Systems to Commercial and End-of-Life Polyurethane Materials131The Chemical Recycling of Polyesters for a Circular Plastics Economy: Challenges and Emerging Opportunities425Heterogeneous Metal Azolate Framework-6 (MAF-6) Catalysts with High Zinc Density for Enhanced Polyethylene Terephthalate (PET) Conversion134Plastic Waste Conversion over a Refinery Waste Catalyst173Plastic Waste Conversion over a Refinery Waste Catalyst12Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Recent Progress in the Chemical Upcycling of Plastic Wastes298Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Harnessing autocatalytic reactions in polymerization and depolymerization15The Critical Importance of Adopting Whole-of-Life Strategies for Polymers and Plastics21Low strain, more gain2Why is Recycling of Postconsumer Plastics so Challenging?381Recent Advancements in Plastic Packaging Recycling: A Mini-Review151ED-ROP of macrocyclic oligomers: A synthetic tool for multicomponent polymer materials2Evaluation of Manganese Catalysts for the Hydrogenative Deconstruction of Commercial and End‐of‐Life Polyurethane Samples52Zn(II)- and Mg(II)-Complexes of a Tridentate {ONN} Ligand: Application to Poly(lactic acid) Production and Chemical Upcycling of Polyesters72Towards a Plastic Circular Economy: Bio-derived Plastics and their End-of-life Strategies6A Single Catalyst for Promoting Reverse Processes: Synthesis and Chemical Degradation of Polylactide49Polyolefins and Polystyrene as Chemical Resources for a Sustainable Future: Challenges, Advances, and Prospects246Amino Acid-Based Cholinium Ionic Liquids as Sustainable Catalysts for PET Depolymerization97Towards recycling purpose: Converting PET plastic waste back to terephthalic acid using pH-responsive phase transfer catalyst29Controlling degradation and recycling of carbon fiber reinforced bismaleimide resin composites via selective cleavage of imide bonds40A computational study of the mechanism of chloroalkane dechlorination with Rh( i ) complexes7A recyclable process between a monomer and polyester with a natural catalyst13Chemically recyclable polymer materials: polymerization and depolymerization cycles212Cosolvent-promoted selective non-aqueous hydrolysis of PET wastes and facile product separation93Homoleptic phenoxy-imine pyridine zinc complexes: efficient catalysts for solvent free synthesis and chemical degradation of polyesters34Integration of upcycling and closed-loop recycling through alternative cyclization–depolymerization33Optimisation of PET glycolysis by applying recyclable heterogeneous organocatalysts112How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics Recycling398Simple Approach to Macrocyclic Carbonates with Fast Polymerization Rates and Their Polymer-to-Monomer Regeneration62From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Sugar-Based Polymers with Stereochemistry-Dependent Degradability and Mechanical Properties60The Life Cycle of Polymer Materials: Problems and Prospects13Versatile Chemical Recycling Strategies: Value‐Added Chemicals from Polyester and Polycarbonate Waste87Sulfonic acid group functionalized Brönsted acidic ionic liquid catalyzed depolymerization of poly(ethylene terephthalate) in water18Zinc-doped ferrite nanoparticles as magnetic recyclable catalysts for scale-up glycolysis of poly(ethylene terephthalate) wastes32Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Solar thermal catalysis for sustainable and efficient polyester upcycling166The Frontier of Plastics Recycling: Rethinking Waste as a Resource for High‐Value Applications68Critical Evaluation of Life Cycle Assessment Analyses of Plastic Waste Pyrolysis59The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Chemical Recycling of Polystyrene to Valuable Chemicals via Selective Acid-Catalyzed Aerobic Oxidation under Visible Light364Chemical Upcycling of Poly(bisphenol A carbonate) Plastic Catalyzed by ZnX 2 via an Amino-Alcoholysis Strategy46Biodegradable Copolyesters with Unexpected Highly Blocky Microstructures and Enhanced Thermal Properties24Modulating local environment of Ni with W for synthesis of carbon nanotubes and hydrogen from plastics32Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Photocatalytic Conversion of Plastic Waste: From Photodegradation to Photosynthesis260High-performance epoxy covalent adaptable networks enabled by alicyclic anhydride monoesters15Recycled (Bio)Plastics and (Bio)Plastic Composites: A Trade Opportunity in a Green Future51Closing the Carbon Loop in the Circular Plastics Economy115Fabrication of high-performance HDPE/CWPF blend film via the assistance of OBC and solid-state drawing8Spotting Trends in Organocatalyzed and Other Organomediated (De)polymerizations and Polymer Functionalizations2Spotting Trends in Organocatalyzed and Other Organomediated (De)polymerizations and Polymer Functionalizations33Catalyst-Free Approach for the Degradation of Bio- and CO2-Sourced Polycarbonates: A Step toward a Circular Plastic Economy15Synchronous degradation and decolorization of colored poly(ethylene terephthalate) fabrics for the synthesis of high purity terephthalic acid53The upcycling of polyethylene terephthalate using protic ionic liquids as catalyst50The organic chemistry behind the recycling of poly(bisphenol‐A carbonate) for the preparation of chemical precursors: A review31Influence of the catalytic system on the methanolysis of polyethylene terephthalate at mild conditions: A systematic investigation44Changes in physicochemical and leachate characteristics of microplastics during hydrothermal treatment of sewage sludge101Precisely Tailoring and Renewing Polymers: An Efficient Strategy for Polymer Recycling6Selective, Sequential, and “One-Pot” Depolymerization Strategies for Chemical Recycling of Commercial Plastics and Mixed Plastics135tert-Amyl Alcohol-Mediated Deconstruction of Polyurethane for Polyol and Aniline Recovery64Theoretical Study on the Hydrogenolysis of Polyurethanes to Improve the Catalytic Activities14Versatile levulinic acid-derived dynamic covalent thermosets enabled by in situ generated imine and multiple hydrogen bonds59Efficient chemical recycling of waste polyethylene terephthalate55Recycling and Upgrading Utilization of Polymer Plastics †34Nachhaltiges Design von Struktur‐ und Funktionspolymeren für die Kreislaufwirtschaft6Sustainable Design of Structural and Functional Polymers for a Circular Economy159Defining Circular Economy Principles for Biobased Products49Trash to Treasure: Photoreforming of Plastic Waste into Commodity Chemicals and Hydrogen over MoS 2 -Tipped CdS Nanorods271The Contribution of Commercial Metal Amides to the Chemical Recycling of Waste Polyesters11Mixed plastics waste valorization through tandem chemical oxidation and biological funneling635Synthesis of photosensitive catalysts with wide-band absorption and ability to enhance the degradation of polyester fabric wastes15New insights into urethane alcoholysis enable chemical full recycling of blended fabric waste65Chemical recycling and upcycling of poly(Bisphenol A carbonate) via metal acetate catalyzed glycolysis19Méthodes catalytiques innovantes de réduction de liaisons carbone-oxygène appliquées à la dépolymérisation réductrice des plastiques oxygénés0Recycling of Plastic Waste: A Systematic Review Using Bibliometric Analysis66Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Polyethylene in Dead-End Silica Nanopores: Forces and Mobility from Non-Equilibrium Statistical Mechanics and Exchange Spectroscopy Nuclear Magnetic Resonance6Upgrading Polyurethanes into Functional Ureas through the Asymmetric Chemical Deconstruction of Carbamates71Impact of the presence of common polymer additives in thermal and catalytic polyethylene decomposition37“Functional upcycling” of polymer waste towards the design of new materials226A COMPLEX APPROACH TO THE UTILIZATION OF ORGANOCHLORINE COMPOUNDS IN TERMS OF VINYL CHLORIDE PRODUCTION WASTES0Bio-based upcycling of poly(ethylene terephthalate) waste to UV-curable polyurethane acrylate17Catalytic routes towards polystyrene recycling109Chemical upcycling of poly(bisphenol A carbonate) to vinylene carbonates through organocatalysis25Cholinium-based ionic liquid catalysts for polyethylene terephthalate glycolysis: understanding the role of solvent and a reappraisal of the cation contribution11Cooperative effects of Schiff base binuclear zinc complexes on the synthesis of aliphatic and semi-aromatic polyesters6Efficient synthesis of camphor-based polycarbonates: a direct route to recyclable polymers10Electroreforming injects a new life into solid waste39Leveraging Chemolysis to Confront the Raise of Emerging Polyester Waste: A Sustainable Strategy Alongside Biological Degradation0Magnetic hollow micro-sized nanoaggregates for synergistically accelerating PET glycolysis44Photochemical aerobic upcycling of polystyrene plastics to commodity chemicals using anthraquinone as the photocatalyst117Selective chemical disassembly of elastane fibres and polyurethane coatings in textiles40Selective deconstruction of mixed plastics by a tailored organocatalyst70Sustainable production of styrene from catalytic recycling of polystyrene over potassium promoted Fe–Al 2 O 3 catalyst13Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210Techno-economic analysis and life cycle assessment of mixed plastic waste gasification for production of methanol and hydrogen139Transport limitations in polyolefin cracking at the single catalyst particle level66Understanding the important variables to optimize glycolysis of polyethylene terephthalate with lanthanide-containing ionic liquids11Depolymerization of robust polyetheretherketone to regenerate monomer units using sulfur reagents26Chemical Recycling of Polyurethane Waste via a Microwave-Assisted Glycolysis Process75Integrated Approach to the Utilization of Organochlorine Compounds by the Example of Vinyl Chloride Production Waste4Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309A renewable lignin-based thermoplastic adhesive for steel joining25Enzymes’ Power for Plastics Degradation589Ring-Opening Polymerization of a Seven-Membered Lactone toward a Biocompatible, Degradable, and Recyclable Semi-aromatic Polyester60Upcycling of Polybutadiene Facilitated by Selenium‐Mediated Allylic Amination23Upcycling of Polybutadiene Facilitated by Selenium‐Mediated Allylic Amination4A Thermo-Catalytic Pyrolysis of Polystyrene Waste Review: A Systematic, Statistical, and Bibliometric Approach48Plastic-Waste-Derived Char as an Additive for Epoxy Composite12Chemical Recycling Processes of Waste Polyethylene Terephthalate Using Solid Catalysts197Recent Advances in Catalytic Chemical Recycling of Polyolefins104Rational design of photo− /electro−catalytic systems for the transformation of plastic wastes51Sustainable catalytic strategies for the transformation of plastic wastes into valued products53The future for biochemical recycling of poly(ethylene terephthalate): From lab to process13Fabrication of high-strength and multi-recyclable supramolecular polysiloxane by incorporating quadruple hydrogen bonds into main-chains for adhesive and oil-water separation21Catalyst Design to Address Nylon Plastics Recycling4Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Upcycling of plastic and tire waste toward use as modifier for asphalt binder16Solvent‐Free Heterogeneous Catalytic Hydrogenation of Polyesters to Diols48Solvent‐Free Heterogeneous Catalytic Hydrogenation of Polyesters to Diols6Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR25Retrieving back plastic wastes for conversion to value added petrochemicals: opportunities, challenges and outlooks86From source to disposal: Cracking the code for sustainable polymers13POLYMERS RECYCLING: UPCYCLING TECHNIQUES. AN OVERVIEW10Recent Advances in the Photoreforming of Plastic Waste: Principles, Challenges, and Perspectives40Selective depolymerization of PET to monomers from its waste blends and composites at ambient temperature97Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Novel catalysts in catalytic upcycling of common polymer wastes26Photocatalytic Upcycling of Plastic Waste: Mechanism, Integrating Modus, and Selectivity77Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Closed-Loop Recycling of Polyols from Thermoset Polyurethanes by tert -Amyl Alcohol-Mediated Depolymerization of Flexible Foams52Chemical Recycling of Flexible Polyurethane Foams by Aminolysis to Recover High-Quality Polyols103Catalytic Fabric Recycling: Glycolysis of Blended PET with Carbon Dioxide and Ammonia59Facile, high-efficiency, and low-cost depolymerization of PA6 to ϵ-caprolactam enables closed-loop chemical recycling39Molecular oxygen-assisted in defect-rich ZnO for catalytic depolymerization of polyethylene terephthalate25A short-cut method for analysis of catalyst performances in pyrolytic reactor7Vitrimer chemistry for 4D printing formulation28Ionic Liquid‐Assisted Depolymerization of Condensation Polymers: A Review182023 Highlights in Interface Science and Engineering: A Collection of Virtual Special Issues4One-pot methanolysis of poly(ethylene terephthalate) enabled by isopropanol-assisted CO2 hydrogenation18Hydroxylation-Depolymerization of Oxyphenylene-Based Super Engineering Plastics To Regenerate Arenols22Reclaiming Monomers from Waste Polyester Textiles with 4d Metal-Doped ZnO and g-C 3 N 4 Nanocomposites1Synthesis of Metal–Organic Frameworks through Enzymatically Recycled Polyethylene Terephthalate35Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12

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  46. Chemical Recycling of Polystyrene to Valuable Chemicals via Selective Acid-Catalyzed Aerobic Oxidation under Visible Light

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  47. Chemical Upcycling of Poly(bisphenol A carbonate) Plastic Catalyzed by ZnX 2 via an Amino-Alcoholysis Strategy

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  48. Biodegradable Copolyesters with Unexpected Highly Blocky Microstructures and Enhanced Thermal Properties

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  49. Modulating local environment of Ni with W for synthesis of carbon nanotubes and hydrogen from plastics

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  50. Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis

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