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RESEARCH PAPER · Cell Reports Physical Science · 2020

Catalytic Hydrocracking of Synthetic Polymers into Grid-Compatible Gas Streams

Wei‐Tse Lee, Félix D. Bobbink, Antoine P. van Muyden, Kun‐Han Lin, Clémence Corminbœuf, Reza R. Zamani, Paul J. Dyson

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Catalytic Hydrocracking of Synthetic Polymers into Grid-Compatible Gas StreamsOriginalApplication of natural zeolite for recycling of polymer waste0Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Recent Advancements in Plastic Packaging Recycling: A Mini-Review151Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Towards a Plastic Circular Economy: Bio-derived Plastics and their End-of-life Strategies6Product composition and coke deposition in the hydrocracking of polystyrene blended with vacuum gasoil27Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions44Expanding plastics recycling technologies: chemical aspects, technology status and challenges610The reductive catalytic upcycling of polyolefin plastic waste17The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Rational Design of Chemical Catalysis for Plastic Recycling391Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling32Innovations Toward the Valorization of Plastics Waste65Breaking C─C Bonds and Preserving C─O Bonds in Aromatic Plastics and Lignin via a Reversing Bond Energy Cleavage Strategy49Catalytic strategies for upvaluing plastic wastes209Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Catalytic degradation of microplastics21Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals61Recent Advances in Catalytic Chemical Recycling of Polyolefins104Plastic Recycling: A Review on Life Cycle, Methods, Misconceptions, and Techno‐Economic Analysis60A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Hydroformylation of pyrolysis oils to aldehydes and alcohols from polyolefin waste195Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26End-of-Life Plastics Management: A Review7Precise activation of C–C bonds for recycling and upcycling of plastics81Bridging the Gap Between Academia and Chemical Industry through Entrepreneurship: An Account on the Case of Hydrogen-assisted Catalytic Plastic Waste Valorisation0Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey4Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Complete hydrogenolysis of mixed plastic wastes101Highly efficient removal of contaminant from typical dye wastewater by using individual AOPs-A/O processes: Design, performance, and mechanism14Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Assessing the Binding of Plastics Additives at Brønsted Acid Sites of Zeolites4Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Towards circularity of plastics: A materials informatics perspective15Efficient Hydrocracking of Waste Polyethylene into Branched Liquid Fuels over Low Pt‐loaded Nb2O5 Catalyst5Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Upgrading of waste polyolefins with non-noble metal catalysts21Recovery of chemicals and energy through thermo-chemical processing of plastic waste33A Mini-review on Development for the Direct Catalytic Hydroconversion of Polypropylene to Liquid and Gaseous Hydrocarbons for Fuels and Chemicals1Emerging Biochemical Conversion for Plastic Waste Management: A Review8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upcycling of Waste Plastics into Value-Added Chemicals6Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Boosting upcycling polypropylene waste to propylene via microwave catalysis18Nanocatalytic upcycling of plastic waste: Advances in selective conversion technologies for sustainable high-value products recovery13Net-Zero Upcycling of Mixed Polyolefins by Spatially Homogeneous Joule Heating7Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Polyethylene and Polypropylene Pyrolysis Using Fe3+-Modified Kaolin Catalyst for Enhanced Gas and Pyrolysis Oil Production5Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Direct Catalytic Conversion of Waste Lipids to Biomethane Over Rutile TiO 2 ‐Supported Ru Catalyst0Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Ceria‐Based Catalysts for Sustainable Processing of Plastic Waste0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0

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  3. Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes

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  6. Towards a Plastic Circular Economy: Bio-derived Plastics and their End-of-life Strategies

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  9. Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions

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  18. Breaking C─C Bonds and Preserving C─O Bonds in Aromatic Plastics and Lignin via a Reversing Bond Energy Cleavage Strategy

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  20. Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons

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  21. Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy

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  32. SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

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