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RESEARCH PAPER · Applied Catalysis B: Environmental · 2021

Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia

Brandon C. Vance, Pavel A. Kots, Cong Wang, Zachary R. Hinton, Caitlin M. Quinn, Thomas H. III Epps, LaShanda T. J. Korley, Dionisios G. Vlachos

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Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconiaOriginalNanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Antioxidant-induced transformations of a metal-acid hydrocracking catalyst in the deconstruction of polyethylene waste69The reductive catalytic upcycling of polyolefin plastic waste17Upcycling Hdpe by Co-Hydrocracking it with Vgo Over a Ptpd/Hy Catalyst. Effects of the Reaction Time0Recent Progress on Sulfated Nanozirconia as a Solid Acid Catalyst in the Hydrocracking Reaction55Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Rational Design of Chemical Catalysis for Plastic Recycling391Upgrading of polyethylene to hydrocarbon fuels over the Fe-modified Pt/Al2O3 catalysts at a mild condition without external H245Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Unleashing the Power of Knowledge Extraction from Scientific Literature in Catalysis27Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Kinetic modeling of the hydrocracking of polystyrene blended with vacuum gasoil22A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Microwave assisted heating of plastic waste: Effect of plastic/susceptor (SiC) contacting patterns33Biologically bound nickel accelerated de-polymerization of polyethylene to high value hydrocarbons and hydrogen12Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Conformations of polyolefins on platinum catalysts control product distribution in plastics recycling29Gasoline-range hydrocarbon production from hydrocracking of LDPE plastic waste utilizing nickel-promoted sulfated nanozirconia catalyst1Understanding Polymer-Porous Solid Interactions Based on Small Gas Molecule Adsorption Behavior18Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Challenges and opportunities of light olefin production via thermal and catalytic pyrolysis of end-of-life polyolefins: Towards full recyclability220Study on the role of the reaction time in the upcycling of HDPE by co-hydrocracking it with VGO7Chemical Upcycling of Waste Plastics to High Value‐Added Products via Pyrolysis: Current Trends, Future Perspectives, and Techno‐Feasibility Analysis33Strategic use of thermo-chemical processes for plastic waste valorization23Recent Advances in Catalytic Chemical Recycling of Polyolefins104Microwave‐Assisted Synthesis of SrTiO3 Nanocuboids without TiCl46Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Chemical Looping Dry Reforming of Methane over Ni-Modified WO 3 /ZrO 2 : Cooperative Work of Dispersed Tungstate Species and Ni over the ZrO 2 Surface30Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47Plastic Recycling: A Review on Life Cycle, Methods, Misconceptions, and Techno‐Economic Analysis60Tuning High-Density Polyethylene Hydrocracking through Mordenite Zeolite Crystal Engineering38Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide4Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Hydrocracking of polyethylene to hydrocarbon fuels over Pt/USY catalysts: Assessment of the hydrogen donors28Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Quantitative analyses of products and rates in polyethylene depolymerization and upcycling11Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Bifunctional catalyst with high efficiency for converting hydrocarbons: The enhanced diffusion between micro and meso-pores15Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey4Direct amination of poly( p -phenylene oxide) to substituted anilines over bimetallic Pd–Ru catalysts13Identification of coke species on Fe/USY catalysts used for recycling polyethylene into fuels18Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters21Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Population Balance Equations for Reactive Separation in Polymer Upcycling20Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45The catalytic pyrolysis of waste polyolefins by zeolite-based catalysts: A critical review on the structure-acidity synergies of catalysts47Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Selective Hydrocracking of Waste Polyolefins toward Gasoline-Range Liquid Fuels via Tandem Catalysis over a Cerium-Promoted Pt/HY Catalyst37Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Hydrogenolysis of Poly(Ethylene‐co‐Vinyl Alcohol) and Related Polymer Blends over Ruthenium Heterogeneous Catalysts7Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31A direct polymeric carbon nitride/tungsten oxide Z‐scheme heterostructure for efficient photocatalytic hydrogen generation via reforming of plastics into value‐added chemicals46Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Catalytic Deconstruction of Ethylene Vinyl Acetate Copolymer and Polyethylene Mixtures via Hydroconversion: Challenges and Solutions8Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Assessing the Binding of Plastics Additives at Brønsted Acid Sites of Zeolites4Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Catalytic Upcycling of Polyolefins316Tracking Chain Populations and Branching Structure during Polyethylene Deconstruction Processes12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Key Terms in Plastic Waste Transformation Reactions3Transformation of Polyolefinic Plastics to Chemicals by Catalytic Decomposition0Upcycling of polyethylene waste to biodegradable adhesive and coating via Baeyer-Villiger reaction: A new view on oxidation-fracture mechanism and structure-function relationship10Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Efficient Hydrocracking of Waste Polyethylene into Branched Liquid Fuels over Low Pt‐loaded Nb2O5 Catalyst5One-pot catalytic conversion of polyethylene wastes to gasoline through a dual-catalyst system41Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst27Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst6Chain-length-controllable upcycling of polyolefins to sulfate detergents41Upcycling of Plastic Waste0Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Confined metal-acid units for boosting benzene hydroalkylation via efficient activation of key intermediate8Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Suitable properties of the HY zeolite of NiW/HY catalysts for the hydroprocessing of a plastic pyrolysis oil/vacuum gas oil (PPO/VGO) blend14Upcycling of waste plastics: strategies, status-quo, and prospects3Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Intensification & Scale-up of Waste Plastic Upcycling to Lubricants Conversion0Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides26The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Upcycling of Waste Plastics into Value-Added Chemicals6Zeolites in the epoch of catalytic recycling plastic waste: Toward circular economy and sustainability20Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Synergistic Catalysis for Recycling and Upcycling of Plastics35Catalytic pyrolysis of low-density polyethylene to produce sustainable aviation fuel fractions: Improving isomerized alkane selectivity via magnetic metal-modified HY zeolites6Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13One-Step Production of Isoalkane-Rich Sustainable Aviation Fuel Fractions via Catalytic Pyrolysis of Low-Density Polyethylene over Y-Type Zeolite10A Minimalist Design for a Dual-Catalyst System for High-Efficiency Conversion of Waste Plastics into Liquid Fuel Products27Decoupling the catalytic features of an Fe2O3/USY catalyst in polyethylene pyrolysis using machine learning2Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics9Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Thermal desorption and coke deposition studies of spent zeolite catalysts in the hydrocracking of expanded polystyrene waste8Zeolite Embedment in a Mesoporous Matrix for Producing High-Quality Gasoline in the Hydrocracking of Prehydrotreated Light Cycle Oil (LCO)1Impact of Acid Sites in ZSM-5 Zeolites on the Selective Catalytic Oxi-Upcycling of High-Density Polyethylene to Dicarboxylic Acid under Mild Conditions16Nanocatalytic upcycling of plastic waste: Advances in selective conversion technologies for sustainable high-value products recovery13Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11TiO 2 ‐Supported Ru–Fe Catalysts for the Hydrodeoxygenation of Bis(2‐hydroxyethyl) Terephthalate (BHET) Prepared by the Glycolysis of Polyethylene Terephthalate (PET)1Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2Selective hydrocracking of polystyrene waste over Pt- and Ru-supported zeolite catalysts into high yield LPG and ethylbenzene4Synergistic Metal-Acid Unit for Boosting Tandem Catalysis via Efficient Transformation of the Key Intermediate4Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking11Carbon–carbon bond cleavage for lignin and plastics deconstruction0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Solvent-free recycling of polystyrene waste into valuable mono-aromatics over a Ni/NbO x catalyst0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2

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  4. Antioxidant-induced transformations of a metal-acid hydrocracking catalyst in the deconstruction of polyethylene waste

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  42. Tuning High-Density Polyethylene Hydrocracking through Mordenite Zeolite Crystal Engineering

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  43. Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics

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  44. Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide

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  47. Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts

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  48. Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity

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  49. Upcycling of polyethylenes by catalysis

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  50. SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

    Applied Catalysis B: Environmental · 2023-07-23

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