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RESEARCH PAPER · Macromolecules · 2020

Hydrogenolysis of Linear Low-Density Polyethylene during Heterogeneous Catalytic Hydrogen–Deuterium Exchange

S. Piril Ertem, Chinomso E. Onuoha, Huiqun Wang, Marc A. Hillmyer, Theresa M. Reineke, Timothy P. Lodge, Frank S. Bates

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Hydrogenolysis of Linear Low-Density Polyethylene during Heterogeneous Catalytic Hydrogen–Deuterium ExchangeOriginalNanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Deuteration and Polymers: Rich History with Great Potential100Recent Progress in the Chemical Upcycling of Plastic Wastes298Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution22Ring opening copolymerization of δ-valerolactone with 2-methyl-1,3-dioxane-4-one towards poly(3-hydroxypropionate- co -5-hydroxyvalerate) copolyesters7A Reductive Deuteration Approach to the Efficient Synthesis of Deuterated Polymers4Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of Polyolefins49Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Catalytic deconstruction of waste polyethylene with ethylene to form propylene419Upcycling Polystyrene84Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes59Advances in the Catalytic Hydrogenation and Properties of Unsaturated Polymers42Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR25Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Upcycling of polyethylenes by catalysis0Threading-the-Needle: Compatibilization of HDPE/ i PP blends with butadiene-derived polyolefin block copolymers63Enhancing Kerosene Selectivity of Fischer-Tropsch Synthesis by Periodical Pore Drainage Via Hydrogenolysis4Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Transition Metal Catalysts for Depolymerization0Solar-driven photocatalysis for recycling and upcycling plastics122Synthesis of Deuterated and Sulfurated Polymers by Inverse Vulcanization: Engineering Infrared Transparency via Deuteration35Hydrogen production, storage, and transportation: recent advances214Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex12Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex3Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Effect of reaction media on hydrogenolysis of polyethylene plastic waste: Polymer-surface interactions in small alkane/polymer blends35Catalytic chemical recycling and upcycling of polyolefin plastics27Copolymerization of Olefins and Conjugated Dienes: A Promising Approach to Produce Recyclable Polyolefins14Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Tracking Chain Populations and Branching Structure during Polyethylene Deconstruction Processes12Optimization of nickel-based catalysts for hydrogenolysis of light paraffins using machine learning5Photothermocatalytic Wet Reforming of Waste Plastics to Syngas45Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics9Nanocatalytic upcycling of plastic waste: Advances in selective conversion technologies for sustainable high-value products recovery13Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Decarboxylation-Triggered Polymer Deconstruction11Catalytic valorization of polyolefins: from catalysts and processes to reactors0Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Hydrogenation Kinetics Study: Precise Control of C=C Bonds in Polyisoprene (PI)-Containing Block Copolymers via Diimide Hydrogenation1Catalyst-free, microdroplet-mediated waste plastic conversion to diacids4Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  3. Recent Progress in the Chemical Upcycling of Plastic Wastes

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  4. Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes

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  5. Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution

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  8. Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis

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  15. Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes

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  17. Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR

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  19. Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts

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  20. Upcycling of polyethylenes by catalysis

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