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RESEARCH PAPER · ACS Catalysis · 2021

Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts

Pavel A. Kots, Sibao Liu, Brandon C. Vance, Cong Wang, James D. Sheehan, Dionisios G. Vlachos

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Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 CatalystsOriginalEffects of Temperature and Time on Supercritical Methanol Co-Liquefaction of Rice Straw and Linear Low-Density Polyethylene0Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts82Towards low-temperature catalysts for sustainable fuel from plastic: A review20Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst42Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Sub/supercritical CO2-induced benign fabrication of magnetic hybrid using waste halogenated plastics and its performance for Cr(Ⅵ) stabilization2Catalytic cascade vapor-phase hydrotreatment of plastic waste into fuels and its sustainability assessment18Catalytic conversion of SPW and products upgrading9Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Polyethylene Upcycling to Fuels: Narrowing the Carbon Number Distribution in N-Alkanes by Tandem Hydropyrolysis/Hydrocracking56Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution22The reductive catalytic upcycling of polyolefin plastic waste17How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics Recycling398From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Catalytic carbon and hydrogen cycles in plastics chemistry78Upgrading waste plastic derived pyrolysis gas via chemical looping cracking–gasification using Ni–Fe–Al redox catalysts70Epilogue: Sorting, Depolymerizing, and Recycling Polymers: The Long Road to a Circular Plastics Economy2A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling32A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling0Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Plasma boosted the conversion of waste plastics into liquid fuel by a peroxymonosulfate-hydrothermal process8Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling32Unleashing the Power of Knowledge Extraction from Scientific Literature in Catalysis27Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of Polyolefins49Current Prospects for Plastic Waste Treatment163Processive Depolymerization Catalysts: A Population Balance Model for Chemistry’s “While” Loop19Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts143Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Processing Poly (ethylene terephthalate) Waste into Functional Carbon Materials by Mechanochemical Extrusion11Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Recycling and Upgrading Utilization of Polymer Plastics †34RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Conformations of polyolefins on platinum catalysts control product distribution in plastics recycling29Highly effective ruthenium-doped mesoporous Ti 1− x Ru x O 2− y crystals for photocatalytic tetracycline degradation8Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Impact modification of wood flour reinforced PP composites: Problems, analysis, solution19Turning Polyethylene Waste to Hydrocarbons Using a Sustainable Acidic Carbocatalyst5Role of solvent in plasma-assisted peroxymonosulfate-hydrothermal process for plastic conversion4Polyethylene Valorization by Combined Chemical Catalysis with Bioconversion by Plastic-Enriched Microbial Consortia26Chemical Upcycling of Waste Plastics to High Value‐Added Products via Pyrolysis: Current Trends, Future Perspectives, and Techno‐Feasibility Analysis33Strategic use of thermo-chemical processes for plastic waste valorization23Carbon nanotubes production from catalytic pyrolysis of polyethylene over nickel-based catalysts: The influence of support materials34Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways31The Key to Solving Plastic Packaging Wastes: Design for Recycling and Recycling Technology105Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Techno-Economic and Life Cycle Analyses of Thermochemical Upcycling Technologies of Low-Density Polyethylene Waste116Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Zeolite Supported Pt for Depolymerization of Polyethylene by Induction Heating18Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR25A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113A two-stage strategy for upcycling chlorine-contaminated plastic waste141Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Catalytic approaches for the removal of microplastics from water: Recent advances and future opportunities73Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Ni-catalyzed carbon–carbon bonds cleavage of mixed polyolefin plastics waste42Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina23Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Conversion of polyethylene to gasoline: Influence of porosity and acidity of zeolites14Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism14Rapid Polyolefin Hydrogenolysis by a Single‐Site Organo‐Tantalum Catalyst on a Super‐Acidic Support: Structure and Mechanism5End-of-Life Plastics Management: A Review7Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture17Precise activation of C–C bonds for recycling and upcycling of plastics81Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins39Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Computational Insights into Catalysis: Evaluating Alternative Metal Potentials in Mgcl2-Supported Ziegler-Natta Catalysts0Direct amination of poly( p -phenylene oxide) to substituted anilines over bimetallic Pd–Ru catalysts13Structurally and surficially activated TiO 2 nanomaterials for photochemical reactions99Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Recycling waste polyethylene into fuels over Fe/USY catalyst: Evaluation on the catalytic activities of varied iron states23Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Probing Interactions between Adsorbed Polymers and γ-Al2O3 Using Solid-State NMR5Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Research Progress in Fuel Oil Production by Catalytic Pyrolysis Technologies of Waste Plastics29Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Recycling Valuable Alkylbenzenes from Polystyrene through Methanol‐Assisted Depolymerization40Recycling Valuable Alkylbenzenes from Polystyrene through Methanol‐Assisted Depolymerization3Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166Hydrogenolysis of Poly(Ethylene‐co‐Vinyl Alcohol) and Related Polymer Blends over Ruthenium Heterogeneous Catalysts7Effect of reaction media on hydrogenolysis of polyethylene plastic waste: Polymer-surface interactions in small alkane/polymer blends35Predicting hydrogenolysis reaction barriers of large hydrocarbons on metal surfaces using machine learning: Implications for polymer deconstruction15Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Radicals mediated polypropylene waste plastics oxidation into ketone fuel12A review on liquid fuel produced from microwave-assisted pyrolysis of plastic waste48Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Catalytic Deconstruction of Ethylene Vinyl Acetate Copolymer and Polyethylene Mixtures via Hydroconversion: Challenges and Solutions8Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Catalytic chemical recycling and upcycling of polyolefin plastics27Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Managing Waste by Generation of Lubricants from Waste Oils2Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Recycling polyolefin plastic waste at short contact times via rapid joule heating93Economically attractive production of commercial-grade gasoline from waste plastics1High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Upvaluing chlorinated plastic wastes18Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12A review on catalytic pyrolysis of textile waste to high-value products: Catalytic mechanisms, products application and perspectives36Assessment of transport phenomena in catalyst effectiveness for chemical polyolefin recycling45

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  5. Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst

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  6. Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study

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  7. Sub/supercritical CO2-induced benign fabrication of magnetic hybrid using waste halogenated plastics and its performance for Cr(Ⅵ) stabilization

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  12. Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor

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  13. Polyethylene Upcycling to Fuels: Narrowing the Carbon Number Distribution in N-Alkanes by Tandem Hydropyrolysis/Hydrocracking

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  14. Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution

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  15. The reductive catalytic upcycling of polyolefin plastic waste

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  31. Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of Polyolefins

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  32. Current Prospects for Plastic Waste Treatment

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  33. Processive Depolymerization Catalysts: A Population Balance Model for Chemistry’s “While” Loop

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  34. Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

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  35. Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts

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  36. Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene

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  37. Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts

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  38. Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts

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  39. Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst

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  40. Processing Poly (ethylene terephthalate) Waste into Functional Carbon Materials by Mechanochemical Extrusion

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  41. Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics

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  42. Recycling and Upgrading Utilization of Polymer Plastics †

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  43. RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts

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  44. Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons

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  45. Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism

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  46. Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy

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  47. Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst

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    Alexander H. Mason, Alessandro Motta, Anusheela Das, Qing Ma, Michael J. Bedzyk, Yosi Kratish, Tobin Jay Marks

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  48. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

    Catalysis Science & Technology · 2022-12-14

    Junde Wei, Jieyi Liu, Weihao Zeng, Zichen Dong, Jingkuo Song, Sibao Liu, Guozhu Liu

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