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RESEARCH PAPER · Nature Catalysis · 2021

Chemical and biological catalysis for plastics recycling and upcycling

Lucas D. Ellis, Nicholas A. Rorrer, Kevin P. Sullivan, Maike Otto, J.E. McGeehan, Yuriy Román‐Leshkov, Nick J. P. Wierckx, Gregg T. Beckham

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Chemical and biological catalysis for plastics recycling and upcyclingOriginalTandem chemical deconstruction and biological upcycling of poly(ethylene terephthalate) to β-ketoadipic acid by Pseudomonas putida KT2440206Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288High-value products from ex-situ catalytic pyrolysis of polypropylene waste using iron-based catalysts: the influence of support materials76Design principles for intrinsically circular polymers with tunable properties217Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Valorization of sugar beet pulp to value-added products: A review135The metabolic potential of plastics as biotechnological carbon sources – Review and targets for the future152Sustainability of Synthetic Plastics: Considerations in Materials Life-Cycle Management92A general electrochemical strategy for upcycling polyester plastics into added-value chemicals by a CuCo 2 O 4 catalyst164Catalytic Conversion of Model Compounds of Plastic Pyrolysis Oil Over Zsm-587Chemical recycling of bioplastics: technical opportunities to preserve chemical functionality as path towards a circular economy88Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Life cycle assessment of enzymatic poly(ethylene terephthalate) recycling156Optimisation of PET glycolysis by applying recyclable heterogeneous organocatalysts112From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Mechanism-Based Design of Efficient PET Hydrolases283Influence of substrate crystallinity and glass transition temperature on enzymatic degradation of polyethylene terephthalate (PET)181Redesigned Hybrid Nylons with Optical Clarity and Chemical Recyclability127The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114High-yield H2 production from polypropylene through pyrolysis-catalytic reforming over activated carbon based nickel catalyst93Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework116Critical advances and future opportunities in upcycling commodity polymers1324Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Rational Design of Chemical Catalysis for Plastic Recycling391NbOx-Based Catalysts for the Activation of C–O and C–C Bonds in the Valorization of Waste Carbon Resources80Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Quantification and evaluation of plastic waste in the United States189Machine learning-aided engineering of hydrolases for PET depolymerization1181Biodegradation of polyethylene and polystyrene: From microbial deterioration to enzyme discovery369Closing the Carbon Loop in the Circular Plastics Economy115Sustainable polymers354Enzymatic Degradation of Polyethylene Terephthalate Plastics by Bacterial Curli Display PETase92Towards synthetic PETtrophy: Engineering Pseudomonas putida for concurrent polyethylene terephthalate (PET) monomer metabolism and PET hydrolase expression82Particle Size Reduction of Poly(ethylene terephthalate) Increases the Rate of Enzymatic Depolymerization But Does Not Increase the Overall Conversion Extent116Photoelectrochemical Catalysis of Waste Polyethylene Terephthalate Plastic to Coproduce Formic Acid and Hydrogen90Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Solar-driven catalytic plastic upcycling87Current Advances in Biodegradation of Polyolefins83Polyolefin Innovations toward Circularity and Sustainable Alternatives96Current Prospects for Plastic Waste Treatment163Coking-Resistant Polyethylene Upcycling Modulated by Zeolite Micropore Diffusion271Directed evolution of an efficient and thermostable PET depolymerase463Catalytic oxidation of polystyrene to aromatic oxygenates over a graphitic carbon nitride catalyst260Catalytic strategies for upvaluing plastic wastes209Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Synthetic biodegradable polyhydroxyalkanoates (PHAs): Recent advances and future challenges161Wax worm saliva and the enzymes therein are the key to polyethylene degradation by Galleria mellonella233Sustainable Design of Structural and Functional Polymers for a Circular Economy159Mixed plastics waste valorization through tandem chemical oxidation and biological funneling635Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Recent advances and challenges in the biotechnological upcycling of plastic wastes for constructing a circular bioeconomy91Mechanochemistry Milling of Waste Poly(Ethylene Terephthalate) into Metal–Organic Frameworks85Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Sustainable cycloaliphatic polyurethanes: from synthesis to applications170Catalytic Chemical Recycling of Post-Consumer Polyethylene188Sourcing thermotolerant poly(ethylene terephthalate) hydrolase scaffolds from natural diversity186Catalytic routes towards polystyrene recycling109Circularity in polymers: addressing performance and sustainability challenges using dynamic covalent chemistries112Electrocatalytic upcycling of plastic waste79From green to circular chemistry paved by biocatalysis92Recent advances in plastic recycling and upgrading under mild conditions147Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210Techno-economic analysis and life cycle assessment of mixed plastic waste gasification for production of methanol and hydrogen139Technical, Economic, and Environmental Comparison of Closed-Loop Recycling Technologies for Common Plastics425Boosting Degradation of Biodegradable Polymers95Concerted and Selective Electrooxidation of Polyethylene‐Terephthalate‐Derived Alcohol to Glycolic Acid at an Industry‐Level Current Density over a Pd−Ni(OH) 2 Catalyst295Review of polymer technologies for improving the recycling and upcycling efficiency of plastic waste271Microbial Enzyme Biotechnology to Reach Plastic Waste Circularity: Current Status, Problems and Perspectives104Upcycling plastic waste to carbon materials for electrochemical energy storage and conversion109Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Photoelectrochemical conversion of plastic waste into high-value chemicals coupling hydrogen production85Towards circular plastics within planetary boundaries392Enzymes’ Power for Plastics Degradation589Complete bio-degradation of poly(butylene adipate-co-terephthalate) via engineered cutinases203Chemical Recycling Processes of Waste Polyethylene Terephthalate Using Solid Catalysts197Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Chemically circular, mechanically tough, and melt-processable polyhydroxyalkanoates218Depolymerization of plastics by means of electrified spatiotemporal heating330Dynamic crosslinking compatibilizes immiscible mixed plastics245Depolymerization of polyesters by a binuclear catalyst for plastic recycling292Acetolysis of waste polyethylene terephthalate for upcycling and life-cycle assessment study205Upcycling chlorinated waste plastics87Mechanistic studies of a lipase unveil effect of pH on hydrolysis products of small PET modules97A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Chemical Recycling of Flexible Polyurethane Foams by Aminolysis to Recover High-Quality Polyols103Discovery and mechanism-guided engineering of BHET hydrolases for improved PET recycling and upcycling111Heterogeneous Photocatalytic Oxidative Cleavage of Polystyrene to Aromatics at Room Temperature76Circular Polyolefins: Advances toward a Sustainable Future76Highly Efficient Biomass Upgrading by a Ni−Cu Electrocatalyst Featuring Passivation of Water Oxidation Activity225Discovery and rational engineering of PET hydrolase with both mesophilic and thermophilic PET hydrolase properties134Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers94Selective electrocatalytic reforming of PET-derived ethylene glycol to formate with a Faraday efficiency of 93.2% at industrial-level current densities98Insights into the Enhancement of the Poly(ethylene terephthalate) Degradation by FAST-PETase from Computational Modeling90Sources, Degradation, Ingestion and Effects of Microplastics on Humans: A Review87Pyrolysis–catalysis upcycling of waste plastic using a multilayer stainless-steel catalyst toward a circular economy99From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Solar-driven photocatalysis for recycling and upcycling plastics122Recent advances in the biodegradation of polyethylene terephthalate with cutinase-like enzymes77Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Energy-saving and product-oriented hydrogen peroxide electrosynthesis enabled by electrochemistry pairing and product engineering146Co-upcycling of polyvinyl chloride and polyesters199Recent advances in polyvinyl chloride ( PVC ) recycling91Significance of poly(ethylene terephthalate) (PET) substrate crystallinity on enzymatic degradation142Catalytic depolymerization of polyester plastics toward closed-loop recycling and upcycling127Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Recent advances in polyhydroxyalkanoates degradation and chemical recycling88Characterization of polymer properties and identification of additives in commercially available research plastics112Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Heterogeneous catalysis for the environment92Recent advances in microbial and enzymatic engineering for the biodegradation of micro- and nanoplastics108Recent advances in oxidative degradation of plastics227Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Solar reforming as an emerging technology for circular chemical industries182Designing a circular carbon and plastics economy for a sustainable future489Natural diversity screening, assay development, and characterization of nylon-6 enzymatic depolymerization100Assessment of PET Depolymerization Processes for Circular Economy. 1. Thermodynamics, Chemistry, Purification, and Process Design77Tandem Chemical Depolymerization and Photoreforming of Waste PET Plastic to High-Value-Added Chemicals148Plastic pretreatment: The key for efficient enzymatic and biodegradation processes81Computational redesign of a hydrolase for nearly complete PET depolymerization at industrially relevant high-solids loading197Depolymerization within a Circular Plastics System387Ring-Opening Polymerization of Lactones to Prepare Closed-Loop Recyclable Polyesters116Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Depolymerization and Re/Upcycling of Biodegradable PLA Plastics106Layered Double Hydroxide Derivatives for Polyolefin Upcycling103The future of bioplastics in food packaging: An industrial perspective198Inspiration of Bimetallic Peroxide for Controllable Electrooxidizing Ethylene Glycol Through Modulating Surficial Intermediates105Recycling and Degradation of Polyamides85Coupling Waste Plastic Upgrading and CO 2 Photoreduction to High-Value Chemicals by a Binuclear Re–Ru Heterogeneous Catalyst77The refinery of the future341From Plastic Waste to Green Hydrogen and Valuable Chemicals Using Sunlight and Water83Advancements and future directions in waste plastics recycling: From mechanical methods to innovative chemical processes136Bottlenecks in biobased approaches to plastic degradation114Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions102Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144Advances in Nonreactive Polymer Compatibilizers for Commodity Polyolefin Blends102Tandem Integration of Biological and Electrochemical Catalysis for Efficient Polyester Upcycling under Ambient Conditions82Interstitial Boron Atoms in Pd Aerogel Selectively Switch the Pathway for Glycolic Acid Synthesis from Waste Plastics122Recent trends in microbial and enzymatic plastic degradation: a solution for plastic pollution predicaments111Catalytic Upcycling of Polyolefins316Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Advanced Catalysts for the Chemical Recycling of Plastic Waste90Stereomicrostructure-regulated biodegradable adhesives104A systematic review of plastic recycling: technology, environmental impact and economic evaluation78Atom-level enzyme active site scaffolding using RFdiffusion2114

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