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RESEARCH PAPER · Applied Catalysis B: Environmental · 2020

Low-temperature catalytic upgrading of waste polyolefinic plastics into liquid fuels and waxes

Yosuke Nakaji, Masazumi Tamura, Shuhei Miyaoka, Shogo Kumagai, Mifumi Tanji, Yoshinao Nakagawa, Toshiaki Yoshioka, Keiichi Tomishige

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Low-temperature catalytic upgrading of waste polyolefinic plastics into liquid fuels and waxesOriginalNanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Probing β-alkyl elimination and selectivity in polyolefin hydrogenolysis through DFT17Catalytic carbon-carbon bond cleavage and carbon-element bond formation give new life for polyolefins as biodegradable surfactants81Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Recent Progress in the Chemical Upcycling of Plastic Wastes298Towards a greater olefin share in polypropylene cracking – Amorphous mesoporous aluminosilicate competes with zeolites48Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts262Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Recycling of Wastes Plastics and Tires from Automotive Industry32Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts82Microwave heating performances of low density polyethylene (LDPE) plastic particles38Towards low-temperature catalysts for sustainable fuel from plastic: A review20Polyolefins and Polyethylene Terephthalate Package Wastes: Recycling and Use in Composites55Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst42Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions44Conversion of Plastic Waste into Supports for Nanostructured Heterogeneous Catalysts: Application in Environmental Remediation15Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610Hydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13The reductive catalytic upcycling of polyolefin plastic waste17TOWARDS A CIRCULAR ECONOMY: LIQUID-FED FAST PYROLYSIS OF WASTE POLYOLEFIN PLASTICS1From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Highly efficient electrocatalytic hydrogen evolution coupled with upcycling of microplastics in seawater enabled via Ni3N/W5N4 janus nanostructures166Non-thermal plasma-assisted rapid hydrogenolysis of polystyrene to high yield ethylene76Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Transition metal chalcogenide bifunctional catalysts for chemical recycling by plastic hydrocracking: a single-source precursor approach30Catalytic carbon and hydrogen cycles in plastics chemistry78A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling32A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling0A structured catalyst of ZSM-5/SiC foam for chemical recycling of waste plastics via catalytic pyrolysis100Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Upgrading of polyethylene to hydrocarbon fuels over the Fe-modified Pt/Al2O3 catalysts at a mild condition without external H245Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Conversion of low-density polyethylene into monocyclic aromatic hydrocarbons by catalytic pyrolysis: Comparison of HZSM-5, Hβ, HY and MCM-41119Reactive Molecular Dynamics Simulations of the Depolymerization of Polyethylene Using Graphene-Oxide-Supported Platinum Nanoparticles12A new sustainable strategy for oil, CH4 and aluminum recovery from metallised food packaging plastics waste using catalytic pyrolysis over ZSM-5 zeolite catalyst28Combined Activated Carbon with Spent Fluid Catalytic Cracking Catalyst and MgO for the Catalytic Conversion of Waste Polyethylene Wax into Diesel-like Hydrocarbon Fuels20Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling32Emulsion templated porous funnel from polypropylene waste for efficient oil separation and spillage management16Catalytic Upcycling of Plastic Waste into High Value-added Chemicals0Unleashing the Power of Knowledge Extraction from Scientific Literature in Catalysis27Innovations Toward the Valorization of Plastics Waste65Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Sustainably Recycling and Upcycling of Single-Use Plastic Wastes through Heterogeneous Catalysis32Current Prospects for Plastic Waste Treatment163Physicochemical assessment of waxy products directly recovered from plastic waste pyrolysis: Review and synthesis of characterization techniques21Pyrolysis technology for plastic waste recycling: A state-of-the-art review481Catalytic oxidation of polystyrene to aromatic oxygenates over a graphitic carbon nitride catalyst260Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Enhanced photocatalytic performance by polarizing ferroelectric KNbO3 for degradation of plastic wastes under mild conditions60A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Electronic modulation of metal-support interactions improves polypropylene hydrogenolysis over ruthenium catalysts129Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst78Processing Poly (ethylene terephthalate) Waste into Functional Carbon Materials by Mechanochemical Extrusion11Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Recycling and Upgrading Utilization of Polymer Plastics †34RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Catalytical thermal conversion of waste fishing nets for a higher added value energy products generation and caprolactam recovery10Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes59Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42An efficient and recyclable Ni 2 P–Co 2 P/ZrO 2 /C nanofiber photocatalyst for the conversion of plastic waste into H 2 and valuable chemicals19Converting plastic waste to fuel and fine chemicals5Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90State of the art in the photochemical degradation of (micro)plastics: from fundamental principles to catalysts and applications112Water-assisted single-step catalytic hydrodeoxygenation of polyethylene terephthalate into gasoline- and jet fuel-range cycloalkanes over supported Ru catalysts in a biphasic system29Catalytic Upgrading of Plastic Waste of Electric and Electronic Equipment (WEEE) Pyrolysis Vapors over Si–Al Ash Pellets in a Two-Stage Reactor10Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Catalytic degradation of microplastics21Polyethylene Valorization by Combined Chemical Catalysis with Bioconversion by Plastic-Enriched Microbial Consortia26Ultrasmall amorphous zirconia nanoparticles catalyse polyolefin hydrogenolysis176Photoredox-Catalyzed Plastic Waste Conversion: Nonselective Degradation versus Selective Synthesis110Strategic use of thermo-chemical processes for plastic waste valorization23Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways31Boosted Photoreforming of Plastic Waste via Defect-Rich NiPS 3 Nanosheets245Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment86Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment29Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals61Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Investigation of Optimal Temperature for Thermal Catalytic Conversion of Marine Biomass for Recovery of Higher-Added-Value Energy Products8Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47Chemical recycling of plastic waste to monomers: Effect of catalyst contact time, acidity and pore size on olefin recovery in ex-situ catalytic pyrolysis of polyolefin waste93Recent Advances in the Photoreforming of Plastic Waste: Principles, Challenges, and Perspectives40Plastic Recycling: A Review on Life Cycle, Methods, Misconceptions, and Techno‐Economic Analysis60Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide4A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58A new strategy to achieve the recycling of plastic waste by catalysis under mild conditions10Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Ni-catalyzed carbon–carbon bonds cleavage of mixed polyolefin plastics waste42Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Catalytic microwave-assisted pyrolysis of plastic waste to produce naphtha for a circular economy35Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23In Situ Construction of an Intramolecular Donor–Acceptor Conjugated Copolymer via Terephthalic Acid Derived from Plastic Waste for Photocatalysis of Plastic to Hydrogen Peroxide43Enhancing Kerosene Selectivity of Fischer-Tropsch Synthesis by Periodical Pore Drainage Via Hydrogenolysis4Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Transition Metal Catalysts for Depolymerization0Magnetic induction assisted pyrolysis of plastic waste to liquid hydrocarbons on carbon catalyst21Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26Simultaneous hydrogen production and conversion of plastic wastes into valued chemicals over a Z-scheme photocatalyst40End-of-Life Plastics Management: A Review7Influence of Pore Length on Hydrogenolysis of Polyethylene within a Mesoporous Support Architecture17Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Isoreticular Metal–Organic Frameworks Confined Mononuclear Ru-Hydrides Enable Highly Efficient Shape-Selective Hydrogenolysis of Polyolefins39Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles2Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Consumer Grade Polyethylene Recycling via Hydrogenolysis on Ultrafine Supported Ruthenium Nanoparticles38A Concise Review of Plastic Pyrolysis and Upgrading Pyrolysis Oil1Catalytic pyrolysis of polypropylene waste for liquid fuels production using Ni/Al-MOF-derived catalysts14Direct amination of poly( p -phenylene oxide) to substituted anilines over bimetallic Pd–Ru catalysts13Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions15Opportunities and challenges for plastic depolymerization by biomimetic catalysis36Recycling tendencies in plastic waste management for environmental sustainability1Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Visible light-induced PET degradation using red CdxZn1−xSeyS1−y quantum dots capped with two different ligands under varying pH conditions2Acid-modified MXenes, Ti3C2, as catalysts for up-cycling polyethylene terephthalate1Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Selective Hydrocracking of Waste Polyolefins toward Gasoline-Range Liquid Fuels via Tandem Catalysis over a Cerium-Promoted Pt/HY Catalyst37Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Catalytic aquathermolysis of contaminated polyolefin plastic waste over an in situ iron hydroxide/oxide nanocatalyst derived from an oil-soluble iron precursor16A Comparative Study on the Migration of Substances from Microwavable Plastic Food Containers into Food by Microwave and Conventional Heating9

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  48. Innovations Toward the Valorization of Plastics Waste

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  49. Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies

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  50. Sustainably Recycling and Upcycling of Single-Use Plastic Wastes through Heterogeneous Catalysis

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