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RESEARCH PAPER · Nature Catalysis · 2020

Catalytic upcycling of high-density polyethylene via a processive mechanism

Akalanka Tennakoon, Xun Wei Wu, Alexander L. Paterson, Smita Patnaik, Yuchen Pei, Anne M. LaPointe, Salai Cheettu Ammal, Ryan A. Hackler, Andreas Heyden, Igor I. Slowing, Geoffrey W. Coates, Massimiliano Delferro, Baron Peters, Wenyu Huang, Aaron David Sadow, Frédéric A. Perras

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Catalytic upcycling of high-density polyethylene via a processive mechanismOriginal100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers280Strong metal–support interaction between palladium and gallium oxide within monodisperse nanoparticles: self-supported catalysts for propyne semi-hydrogenation50Direct synthesis of a jet fuel range dicycloalkane by the aqueous phase hydrodeoxygenation of polycarbonate48Microbial synthesis of vanillin from waste poly(ethylene terephthalate)232Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Catalytic processing of plastic waste on the rise613H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen127Chemical upcycling of waste polyolefinic plastics to low-carbon synthetic naphtha for closing the plastic use loop48Catalytic carbon-carbon bond cleavage and carbon-element bond formation give new life for polyolefins as biodegradable surfactants81Near-complete depolymerization of polyesters with nano-dispersed enzymes298Plastic waste to fuels by hydrocracking at mild conditions577Deconstruction of high-density polyethylene into liquid hydrocarbon fuels and lubricants by hydrogenolysis over Ru catalyst208Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Polypropylene Plastic Waste Conversion to Lubricants over Ru/TiO 2 Catalysts262Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Toward polymer upcycling—adding value and tackling circularity719Conversion of Polyethylene Waste into Gaseous Hydrocarbons via Integrated Tandem Chemical–Photo/Electrocatalytic Processes167Recent Advancements in Photocatalytic Valorization of Plastic Waste to Chemicals and Fuels60Chemical and biological catalysis for plastics recycling and upcycling1198Upcycling and catalytic degradation of plastic wastes332Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Pyrolysis-catalysis for waste polyolefin conversion into low aromatic naphtha86Why is Recycling of Postconsumer Plastics so Challenging?381Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts82Catalytic Amination of Polylactic Acid to Alanine208Chemical Upcycling of Polyethylene to Value-Added α,ω-Divinyl-Functionalized Oligomers92Fluorescence-activated droplet sorting of PET degrading microorganisms73Design principles for intrinsically circular polymers with tunable properties217Sustainable Bioplastic Made from Biomass DNA and Ionomers103From plastic waste to wealth using chemical recycling: A review300Polyolefin plastic waste hydroconversion to fuels, lubricants, and waxes: a comparative study145Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality101Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality449A sustainable approach for the synthesis of recyclable cyclic CO 2 -based polycarbonates56Effect of reaction conditions on the hydrogenolysis of polypropylene and polyethylene into gas and liquid alkanes133Expanding plastics recycling technologies: chemical aspects, technology status and challenges610From trash to treasure: Chemical recycling and upcycling of commodity plastic waste to fuels, high-valued chemicals and advanced materials269Non-thermal plasma-assisted rapid hydrogenolysis of polystyrene to high yield ethylene76Size-Controlled Nanoparticles Embedded in a Mesoporous Architecture Leading to Efficient and Selective Hydrogenolysis of Polyolefins168Catalytic carbon and hydrogen cycles in plastics chemistry78The Critical Role of Process Analysis in Chemical Recycling and Upcycling of Waste Plastics114Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis127Disordered, Sub-Nanometer Ru Structures on CeO2 are Highly Efficient and Selective Catalysts in Polymer Upcycling by Hydrogenolysis213Rational Design of Chemical Catalysis for Plastic Recycling391Current Trends in Waste Plastics’ Liquefaction into Fuel Fraction: A Review61Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Biodegradation of polyethylene and polystyrene: From microbial deterioration to enzyme discovery369Converting waste PET plastics into automobile fuels and antifreeze components260Sustainable polymers354Integrated strategy for the synthesis of aromatic building blocks via upcycling of real-life plastic wastes142Bridging Plastic Recycling and Organic Catalysis: Photocatalytic Deconstruction of Polystyrene via a C–H Oxidation Pathway211End-of-Life Management Options for Agricultural Mulch Films in the United States—A Review72Catalytic Pyrolysis of Waste Polyethylene Using Combined CaO and Ga/ZSM-5 Catalysts for High Value-Added Aromatics Production96Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Polyolefin Innovations toward Circularity and Sustainable Alternatives96Coking-Resistant Polyethylene Upcycling Modulated by Zeolite Micropore Diffusion271Environmental toxicity and decomposition of polyethylene286Pyrolysis technology for plastic waste recycling: A state-of-the-art review481Microwave-initiated MAX Ti3AlC2-catalyzed upcycling of polyolefin plastic wastes: Selective conversion to hydrogen and carbon nanofibers for sodium-ion battery68A unified view on catalytic conversion of biomass and waste plastics584Cascade degradation and upcycling of polystyrene waste to high-value chemicals113Catalytic oxidation of polystyrene to aromatic oxygenates over a graphitic carbon nitride catalyst260Breaking C─C Bonds and Preserving C─O Bonds in Aromatic Plastics and Lignin via a Reversing Bond Energy Cleavage Strategy49Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts143Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts139Grave-to-cradle upcycling of Ni from electroplating wastewater to photothermal CO2 catalysis97Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Chemical Recycling of Polyethylene by Tandem Catalytic Conversion to Propylene259RETRACTED: Hydrogenolysis of Polyethylene and Polypropylene into Propane over Cobalt-Based Catalysts72Trash to Treasure: Photoreforming of Plastic Waste into Commodity Chemicals and Hydrogen over MoS 2 -Tipped CdS Nanorods271Microplastic materials in the environment: Problem and strategical solutions201Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Ni/SiO2 catalysts for polyolefin deconstruction via the divergent hydrogenolysis mechanism121Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117A state-of-the-art review on waste plastics-derived aviation fuel: Unveiling the heterogeneous catalytic systems and techno-economy feasibility of catalytic pyrolysis78Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Degradation of low density polyethylene by Bacillus species85Thermocatalytic CO 2 conversion by siliceous matter: a review48In-situ exsolution of Fe-Ni alloy catalysts for H2 and carbon nanotube production from microwave plasma-initiated decomposition of plastic wastes49Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Catalytic Chemical Recycling of Post-Consumer Polyethylene188Photochemical aerobic upcycling of polystyrene plastics to commodity chemicals using anthraquinone as the photocatalyst117Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Transport limitations in polyolefin cracking at the single catalyst particle level66Converting Plastic Wastes to Naphtha for Closing the Plastic Loop187Ultrasmall amorphous zirconia nanoparticles catalyse polyolefin hydrogenolysis176Catalytic Amounts of an Antibacterial Monomer Enable the Upcycling of Poly(Ethylene Terephthalate) Waste59Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment86Metal-catalyzed plastic depolymerization79Recent Advances in Catalytic Chemical Recycling of Polyolefins104Rational design of photo− /electro−catalytic systems for the transformation of plastic wastes51Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance63Micro/nano-plastic removal from wastewater using cellulose membrane: Performance and life cycle assessment48Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process73Bifunctional tandem catalytic upcycling of polyethylene to surfactant-range alkylaromatics101Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Chemical recycling of polyolefins: a closed-loop cycle of waste to olefins126Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Hydroformylation of pyrolysis oils to aldehydes and alcohols from polyolefin waste195Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering55Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Catalytic depolymerization of polyester plastics toward closed-loop recycling and upcycling127Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Rational design principles of single-atom catalysts for hydrogen production and hydrogenation58Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Solar reforming as an emerging technology for circular chemical industries182Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Synthesis and Deconstruction of Polyethylene-type Materials194A state-of-the-art review of multilayer packaging recycling: Challenges, alternatives, and outlook150Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104CO2-facilitated upcycling of polyolefin plastics to aromatics at low temperature56Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166Coupled conversion of polyethylene and carbon dioxide catalyzed by a zeolite–metal oxide system50Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Microwave‐Assisted Pyrolysis‐A New Way for the Sustainable Recycling and Upgrading of Plastic and Biomass: A Review46Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Catalytic Upcycling of Polyolefins316Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Rapid Generation of Microplastics and Plastic-Derived Dissolved Organic Matter from Food Packaging Films under Simulated Aging Conditions54Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Advanced Catalysts for the Chemical Recycling of Plastic Waste90Photocatalytic Reforming Raw Plastic in Seawater by Atomically‐Engineered GeS/ZnIn 2 S 452Highly selective upcycling of plastic mixture waste by microwave-assisted catalysis over Zn/b-ZnO68Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47External acidity as performance descriptor in polyolefin cracking using zeolite-based materials60In-line NMR guided orthogonal transformation of real-life plastics63High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65Prospects of Nanoscience with Nanocrystals: 2025 Edition58

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