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RESEARCH PAPER · ChemSusChem · 2020

The Use of Heterogeneous Catalysis in the Chemical Valorization of Plastic Waste

Lesli O. Mark, Melissa C. Cendejas, Ive Hermans

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The Use of Heterogeneous Catalysis in the Chemical Valorization of Plastic WasteOriginalLow-temperature catalytic upgrading of waste polyolefinic plastics into liquid fuels and waxes328Simultaneous pretreatment and catalytic conversion of polyolefins into hydrocarbon fuels over acidic zeolite catalysts20100th Anniversary of Macromolecular Science Viewpoint: Redefining Sustainable Polymers280Catalytic Hydrogenolysis of Polyolefins into Alkanes46Direct synthesis of a jet fuel range dicycloalkane by the aqueous phase hydrodeoxygenation of polycarbonate48Nanocatalyzed Upcycling of the Plastic Wastes for a Circular Economy123Solar fuels and feedstocks: the quest for renewable black gold33Catalytic processing of plastic waste on the rise613Modeling Metal-Catalyzed Polyethylene Depolymerization: [(Phen)Pd(X)]+ (X = H and CH3) Catalyze the Decomposition of Hexane into a Mixture of Alkenes via a Complex Reaction Network14Waste Refinery: The Valorization of Waste Plastics and End-of-Life Tires in Refinery Units. A Review211H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen127Ultrafast microwave assisted recycling of PET to a family of functional precursors and materials53Synthetic Lubricants Derived from Plastic Waste and their Tribological Performance53Conversion of HDPE into Value Products by Fast Pyrolysis Using FCC Spent Catalysts in a Fountain Confined Conical Spouted Bed Reactor63Single pot catalyst strategy to branched products via adhesive isomerization and hydrocracking of polyethylene over platinum tungstated zirconia176Recent Advancements in Photocatalytic Valorization of Plastic Waste to Chemicals and Fuels60Hydrogenolysis of Polypropylene and Mixed Polyolefin Plastic Waste over Ru/C to Produce Liquid Alkanes288Thermochemical Recycling of Waste Plastics by Pyrolysis: A Review241Kombucha SCOBY Waste as a Catalyst Support5Why is Recycling of Postconsumer Plastics so Challenging?381Polyethylene Hydrogenolysis at Mild Conditions over Ruthenium on Tungstated Zirconia292Maximizing light olefins and aromatics as high value base chemicals via single step catalytic conversion of plastic waste131Chemical recycling of plastic waste via thermocatalytic routes157Boron-Modified Mesoporous ZSM-5 for the Conversion of Pyrolysis Vapors from LDPE and Mixed Polyolefins: Maximizing the C 2 –C 4 Olefin Yield with Minimal Carbon Footprint59A review of the plastic value chain from a circular economy perspective279Upgrading spent battery separator into syngas and hydrocarbons through CO2-Assisted thermochemical platform6A Review of Recent Research on Catalytic Biomass Pyrolysis and Low-Pressure Hydropyrolysis65Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes301Efficient upgrading of polyolefin plastics into C 5 –C 12 gasoline alkanes over a Pt/W/Beta catalyst42From plastic waste to wealth using chemical recycling: A review300Recent Trends in the Pyrolysis of Non‐Degradable Waste Plastics189Controlling Nucleation Pathways in Zeolite Crystallization: Seeding Conceptual Methodologies for Advanced Materials Design155Approaches for the Synthesis of High-Melting Waxes: A Review11Catalytic Conversion of Model Compounds of Plastic Pyrolysis Oil Over Zsm-587Catalytic conversion of SPW and products upgrading9Development of porous solid acid catalysts for lignocellulose and plastic upcycling.0Marine waste upcycling—recovery of nylon monomers from fishing net waste using seashell waste-derived catalysts in a CO 2 -mediated thermocatalytic process64Solid Base Assisted Dual‐Promoted Heterogeneous Conversion of PVC to Metal‐Free Porous Carbon Catalyst25Highly selective conversion of mixed polyolefins to valuable base chemicals using phosphorus-modified and steam-treated mesoporous HZSM-5 zeolite with minimal carbon footprint105The Frontier of Plastics Recycling: Rethinking Waste as a Resource for High‐Value Applications68Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Upgrading of polyethylene to hydrocarbon fuels over the Fe-modified Pt/Al2O3 catalysts at a mild condition without external H245Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Catalytic pyrolysis of single-use waste polyethylene for the production of liquid hydrocarbon using modified bentonite catalyst2Effect of Zeolite Catalyst on the Pyrolysis Kinetics of Multi-Layered Plastic Food Packaging21Innovations Toward the Valorization of Plastics Waste65Modelling Compression Strength of Waste PET and SCM Blended Cementitious Grout Using Hybrid of LSSVM Models10Current Prospects for Plastic Waste Treatment163First-Generation Organic Reaction Intermediates in Zeolite Chemistry and Catalysis107CO2-mediated thermal treatment of disposable plastic food containers24Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene44Upcycling of abandoned banner via thermocatalytic process over a MnFeCoNiCu high-entropy alloy catalyst48Towards high-quality petrochemical feedstocks from mixed plastic packaging waste via advanced recycling: The past, present and future110Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Nachhaltiges Design von Struktur‐ und Funktionspolymeren für die Kreislaufwirtschaft6Sustainable Design of Structural and Functional Polymers for a Circular Economy159Microplastic materials in the environment: Problem and strategical solutions201Upcycling plastic waste into high value-added chemicals under mild conditions1Role of Bifunctional Ru/Acid Catalysts in the Selective Hydrocracking of Polyethylene and Polypropylene Waste to Liquid Hydrocarbons172Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Grand challenges present great opportunities in environmental catalysis0Plastic and Waste Tire Pyrolysis Focused on Hydrogen Production—A Review18Enhanced Production of Liquid Alkanes from Waste Polyethylene via the Electronic Effect‐Favored Csecondary−Csecondary Bond Cleavage42Catalytic Pyrolysis of Plastic Waste and Molecular Symmetry Effects: A Review47Catalytic conversion of polyethylene into aromatics with Pt/ZSM-5: insights into reaction pathways and rate-controlling step regulation53Catalytic routes towards polystyrene recycling109Chemo-Biological Upcycling of Mixed Plastic Wastes into Medium-Chain Α,Ω-Diacids0Cobalt catalysts (Co–N–C) for C–O bond cleavage in lignin-derived aryl ethers and lignin11Converting plastic waste to fuel and fine chemicals5Functionalization of polyethylene with hydrolytically-stable ester groups6Leveraging Chemolysis to Confront the Raise of Emerging Polyester Waste: A Sustainable Strategy Alongside Biological Degradation0Tandem oxidative and thermal cracking of polypropylene at low temperatures21Techno-economic analysis and life cycle assessment for catalytic fast pyrolysis of mixed plastic waste210Upcycling of waste plastics to carbon nanomaterials3Conversion of toxic chemicals into flammable gases through the thermolysis of polyurethane foam using CO213Catalytic degradation of microplastics21Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation309Environmentally Friendly Polymer Concrete: Polymer Treatment, Processing, and Investigating Carbon Footprint with Climate Change24Strategic use of thermo-chemical processes for plastic waste valorization23Plastic waste as pyrolysis feedstock for plastic oil production: A review300Chemical Recycling Processes of Waste Polyethylene Terephthalate Using Solid Catalysts197Machine Learning and Informatics Based Elucidation of Reaction Pathways for Upcycling Model Polyolefin to Aromatics11Recent Advances in Catalytic Chemical Recycling of Polyolefins104Estimating the efficiency of catalysts for catalytic pyrolysis of polyethylene1The role of porosity and acidity in the catalytic upcycling of polyethylene8Sustainable catalytic strategies for the transformation of plastic wastes into valued products53HBpin/MoO2Cl2(H2O)2 as an efficient catalytic system for the reduction of esters, lactones and polyester plastic waste16Selective recovery of caprolactam from the thermo-catalytic conversion of textile waste over γ-Al2O3 supported metal catalysts26Intrinsic Millisecond Kinetics of Polyethylene Pyrolysis via Pulse-Heated Analysis of Solid Reactions37Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process7Highly Selective Catalytic Oxi‐upcycling of Polyethylene to Aliphatic Dicarboxylic Acid under a Mild Hydrogen‐Free Process73Metal-organic framework-based nanostructured catalysts: Applications in efficient organic transformations41Investigation into the Reaction Pathways and Catalyst Deactivation for Polyethylene Hydrogenolysis over Silica-Supported Cobalt Catalysts58Continuous flow synthesis of Ag-PEDOT-COF nanocomposite for sustainable photoreforming of plastic waste and chromium remediation in visible light29Hierarchical zeolites TNU-9 and IM-5 as the catalysts for cracking processes29Rapid chemical recycling of waste polyester plastics catalyzed by recyclable catalyst30Controlling PET oligomers vs monomers via microwave-induced heating and swelling49Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Heterogenous electromediated depolymerization of highly crystalline polyoxymethylene43Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Bead Mill-driven Acceleration of Catalytic Methanolysis of Poly(ethylene terephthalate) under Mild Reaction Conditions6Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23Depolymerization of Polyester and Polycarbonate Waste using HBpin and Cheap Zinc Catalysts21Sustainable ethylene production: Recovery from plastic waste via thermochemical processes35Efficient Depolymerization of Polyester and Polycarbonate Plastic Waste Catalyzed by Commercially Available Homogeneous and Heterogeneous Manganese Catalysts28Hydrocracking of polyethylene to hydrocarbon fuels over Pt/USY catalysts: Assessment of the hydrogen donors28Solar-driven photocatalysis for recycling and upcycling plastics122Low‐Temperature Upcycling of Polypropylene Waste into H2 Fuel via a Novel Tandem Hydrothermal Process7Modeling and simulation of microwave assisted catalytic pyrolysis system of waste plastics polymer for fuel production14Investigation into the shape selectivity of zeolites for conversion of polyolefin plastic pyrolysis oil model compound36An Overview of Management Status and Recycling Strategies for Plastic Packaging Waste in China14Tailoring the Near-Surface Environment of Rh Single-Atom Catalysts for Selective CO 2 Hydrogenation28Assessment of the Efficiency of Catalysts for the Catalytic Pyrolysis of Polyethylene7Optimisation of polyethylene catalytic pyrolysis in the presence of zeolites0Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Catalytic and biocatalytic degradation of microplastics73Synthesis of straight-chain C49H100 alkane using a modular splicing strategy2Co-production of hydrogen and carbon nanotubes via catalytic pyrolysis of polyethylene over Fe/ZSM-5 catalysts: Effect of Fe loading on the catalytic activity50Maximizing light olefin production via one-pot catalytic cracking of crude waste plastic pyrolysis oil29Waste to energy: Trending key challenges and current technologies in waste plastic management148Advances in catalytic chemical recycling of synthetic textiles43Catalytic recycling of PET waste bottles into a value-added amide monomer using a heterogeneous niobium pentoxide nanocatalyst12ChemPren: a new and economical technology for conversion of waste plastics to light olefins0Identification of coke species on Fe/USY catalysts used for recycling polyethylene into fuels18Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0Recycling tendencies in plastic waste management for environmental sustainability1Recycling waste polyethylene into fuels over Fe/USY catalyst: Evaluation on the catalytic activities of varied iron states23Thermochemical Valorization of Waste Plastic for Production of Synthetic Fuels, Fine Chemicals, and Carbon Nanotubes39Influence of Natural Zeolites on the Thermal Decomposition of Multi-layered Plastic Waste1Development stages of a number of electromechanical systems to establish a green additive remanufacturing ecosystem2Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50A new circulation in glycolysis of polyethylene terephthalate using MOF-based catalysts for environmental sustainability of plastic28Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Mg(OTf)2 as an Excellent Catalyst for the Reductive Depolymerization and Methanolysis of Polyesters and Polycarbonates17Unravelling the structure-performance relationship of zeolite Beta in the catalytic cracking of low-density polyethylene by proposing gasoline factor as the descriptor11Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst12Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35An Overview of the Sustainable Depolymerization/Degradation of Polypropylene Microplastics by Advanced Oxidation Technologies33Syngas production through CO2-mediated pyrolysis of polyoxymethylene9A critical examination of advanced approaches in green chemistry: microbial bioremediation strategies for sustainable mitigation of plastic pollution18Thermochemical recovery of propylene from plastic waste: A review17Methanolysis of Plastic Waste with Manganese Compounds10Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Bimetal-carbon engineering for polypropylene conversion into hydrocarbons and ketones in a Fenton-like system10

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  37. Marine waste upcycling—recovery of nylon monomers from fishing net waste using seashell waste-derived catalysts in a CO 2 -mediated thermocatalytic process

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  44. Catalytic pyrolysis of single-use waste polyethylene for the production of liquid hydrocarbon using modified bentonite catalyst

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  45. Effect of Zeolite Catalyst on the Pyrolysis Kinetics of Multi-Layered Plastic Food Packaging

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  46. Innovations Toward the Valorization of Plastics Waste

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  47. Modelling Compression Strength of Waste PET and SCM Blended Cementitious Grout Using Hybrid of LSSVM Models

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  48. Current Prospects for Plastic Waste Treatment

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  49. First-Generation Organic Reaction Intermediates in Zeolite Chemistry and Catalysis

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  50. CO2-mediated thermal treatment of disposable plastic food containers

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    Sungyup Jung, Yiu Fai Tsang, Dohee Kwon, Dongho Choi, Wei‐Hsin Chen, Yong‐Hyun Kim, Deok Hyun Moon, Eilhann E. Kwon

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