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RESEARCH PAPER · Angewandte Chemie · 2020

Die nächste Generation des Recyclings – neues Leben für Kunststoffmüll

Ina Vollmer, Michael J. F. Jenks, Mark C. P. Roelands, Robin J. White, Toon van Harmelen, Paul J. de Wild, Gerard P. van der Laan, Florian Meirer, Jos T. F. Keurentjes, Bert Marc Weckhuysen

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Die nächste Generation des Recyclings – neues Leben für KunststoffmüllOriginalHighly Efficient Solid‐State Hydrolysis of Waste Polyethylene Terephthalate by Mechanochemical Milling and Vapor‐Assisted Aging137The Use of Heterogeneous Catalysis in the Chemical Valorization of Plastic Waste220Towards the Circular Economy: Converting Aromatic Plastic Waste Back to Arenes over a Ru/Nb2O5 Catalyst74Towards the Circular Economy: Converting Aromatic Plastic Waste Back to Arenes over a Ru/Nb2O5 Catalyst397Selective Chemical Upcycling of Mixed Plastics Guided by a Thermally Stable Organocatalyst242Selective Chemical Upcycling of Mixed Plastics Guided by a Thermally Stable Organocatalyst27Exploring the synergetic effects of the major components of biomass additives in the pyrolysis of polylactic acid47Biocatalysis in the Recycling Landscape for Synthetic Polymers and Plastics towards Circular Textiles116H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen127Reductive Depolymerization of Plastic Waste Catalyzed by Zn(OAc) 2 ⋅ 2H 2 O72The Chemical Recycling of Polyesters for a Circular Plastics Economy: Challenges and Emerging Opportunities425Plastic Waste Conversion over a Refinery Waste Catalyst173Plastic Waste Conversion over a Refinery Waste Catalyst12Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future320Recent Progress in the Chemical Upcycling of Plastic Wastes298Current Developments in the Chemical Upcycling of Waste Plastics Using Alternative Energy Sources86Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities174Catalytic Reductive Alcohol Etherifications with Carbonyl‐Based Compounds or CO2 and Related Transformations for the Synthesis of Ether Derivatives45Computational Approach for Rapidly Predicting Temperature‐Dependent Polymer Solubilities Using Molecular‐Scale Models45State‐Of‐The‐Art Quantification of Polymer Solution Viscosity for Plastic Waste Recycling61Reducing Antisolvent Use in the STRAP Process by Enabling a Temperature‐Controlled Polymer Dissolution and Precipitation for the Recycling of Multilayer Plastic Films105Zinc‐Catalyzed Depolymerization of the End‐of‐Life Poly(ethylene 2,5‐furandicarboxylate)19Fabricating a Repairable, Recyclable, Imine‐based Dynamic Covalent Thermosetting Resin with Excellent Water Resistance by Introducing Dynamic Covalent Oxime Bonds16Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts82Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis100Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis15Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality101Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality449Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer Reactions63Chemical recovery of thermosetting unsaturated polyester resins73Solid Base Assisted Dual‐Promoted Heterogeneous Conversion of PVC to Metal‐Free Porous Carbon Catalyst25A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling32A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling0Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks172Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework116Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework27Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis112Multilayer Packaging in a Circular Economy98“Like Recycles Like”: Selective Ring‐Closing Depolymerization of Poly(L‐Lactic Acid) to L‐Lactide101“Like Recycles Like”: Selective Ring‐Closing Depolymerization of Poly(L‐Lactic Acid) to L‐Lactide15A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry135A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry16Sustainable recycling technologies for thermoplastic polymers and their composites: A review of the state of the art162State‐of‐the‐art and future challenges of polymer recycling in the context of circular economy2Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources130Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources18A Highly Dynamic Covalent Polymer Network without Creep: Mission Impossible?183A Highly Dynamic Covalent Polymer Network without Creep: Mission Impossible?6Nachhaltiges Design von Struktur‐ und Funktionspolymeren für die Kreislaufwirtschaft6Sustainable Design of Structural and Functional Polymers for a Circular Economy159Accelerated Polyethylene Terephthalate (PET) Enzymatic Degradation by Room Temperature Alkali Pre‐treatment for Reduced Polymer Crystallinity62Selective Lanthanide‐Organic Catalyzed Depolymerization of Nylon‐6 to ϵ‐Caprolactam6Selective Lanthanide‐Organic Catalyzed Depolymerization of Nylon‐6 to ϵ‐Caprolactam99Biodegradable High‐Density Polyethylene‐like Material105Biodegradable High‐Density Polyethylene‐like Material26Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes59Open Loop Recycling – Guanidine Iron(II) Polymerization Catalyst for the Depolymerization of Polylactide36Electroreforming injects a new life into solid waste39Ionic Liquids for the Chemical Recycling of Polymeric Materials and Control of Their Solubility16Recent Advances in Catalytic Chemical Recycling of Polyolefins104Influence of Molecular Characteristics and Size Effects in Polystyrene Pyrolysis7Systemized and Effective Methodologies of Converting Worn Naphtha Plastic into Combustible Fuels0Using Yield and Entropy-Based Characteristics for Circular Economy9Open‐ and Closed‐Loop Recycling: Highly Active Zinc Bisguanidine Polymerization Catalyst for the Depolymerization of Polyesters20Circular Economy and Chemical Conversion for Polyester Wastes23Electrochemical Deconstruction of Waste Polyvinylidene Chloride (PVDC) to Value‐Added Products in Batch and Flow16Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling21Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation7Transitioning of the Chemical Industry Toward a Net‐Zero Carbon Dioxide Emission Path0Unveiling the Electrochemical Reactivity of Urethane Toward Different Bond Formations and Application to Polyurethane Deconstruction via C─N Bond Formation0Natural Sunlight‐Driven Synthesis of Conjugated Microporous Polymers via Electron Donor‐Acceptor Complexes for Highly Efficient Catalytic Upcycling of Real‐World Plastic Waste0Enhanced Formation of Dicarboxylic Acids in the Catalytic Oxidation of Polyethylene With O 2 and NO x0Attractive Ni … O Interactions Enable Non‐Alternating Ethylene‐Carbon Monoxide Copolymerization0Selective Sequential Depolymerization of Mixed Plastics Mediated by Photothermal Conversion1Room‐Temperature Depolymerization of Waste Polycarbonate and Polyester Enabled by an Electrochemically Generated Local Alkaline Microenvironment0Titanium‐Catalyzed Defluorination of Poly(Vinyl Fluoride) and Poly(Vinylidene Fluoride) Under Friedel–Crafts Conditions0

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  1. Highly Efficient Solid‐State Hydrolysis of Waste Polyethylene Terephthalate by Mechanochemical Milling and Vapor‐Assisted Aging

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  2. The Use of Heterogeneous Catalysis in the Chemical Valorization of Plastic Waste

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  3. Towards the Circular Economy: Converting Aromatic Plastic Waste Back to Arenes over a Ru/Nb2O5 Catalyst

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  4. Towards the Circular Economy: Converting Aromatic Plastic Waste Back to Arenes over a Ru/Nb2O5 Catalyst

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  5. Selective Chemical Upcycling of Mixed Plastics Guided by a Thermally Stable Organocatalyst

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  6. Selective Chemical Upcycling of Mixed Plastics Guided by a Thermally Stable Organocatalyst

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  7. Exploring the synergetic effects of the major components of biomass additives in the pyrolysis of polylactic acid

    Green Chemistry · 2021-01-01

    Ce Sun, Xiaojian Chen, Dingyuan Zheng, Wenrui Yao, Haiyan Tan, Yanhua Zhang, Song Liu

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  8. Biocatalysis in the Recycling Landscape for Synthetic Polymers and Plastics towards Circular Textiles

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  9. H 2 ‐free Plastic Conversion: Converting PET back to BTX by Unlocking Hidden Hydrogen

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  10. Reductive Depolymerization of Plastic Waste Catalyzed by Zn(OAc) 2 ⋅ 2H 2 O

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  11. The Chemical Recycling of Polyesters for a Circular Plastics Economy: Challenges and Emerging Opportunities

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  12. Plastic Waste Conversion over a Refinery Waste Catalyst

    Angewandte Chemie International Edition · 2021-05-11

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  13. Plastic Waste Conversion over a Refinery Waste Catalyst

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    Ina Vollmer, Michael J. F. Jenks, Rafael Mayorga González, Florian Meirer, Bert Marc Weckhuysen

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  14. Waste to Wealth: Chemical Recycling and Chemical Upcycling of Waste Plastics for a Great Future

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  15. Recent Progress in the Chemical Upcycling of Plastic Wastes

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  16. Current Developments in the Chemical Upcycling of Waste Plastics Using Alternative Energy Sources

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  17. Strategic Approach Towards Plastic Waste Valorization: Challenges and Promising Chemical Upcycling Possibilities

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  18. Catalytic Reductive Alcohol Etherifications with Carbonyl‐Based Compounds or CO2 and Related Transformations for the Synthesis of Ether Derivatives

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  19. Computational Approach for Rapidly Predicting Temperature‐Dependent Polymer Solubilities Using Molecular‐Scale Models

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  20. State‐Of‐The‐Art Quantification of Polymer Solution Viscosity for Plastic Waste Recycling

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  21. Reducing Antisolvent Use in the STRAP Process by Enabling a Temperature‐Controlled Polymer Dissolution and Precipitation for the Recycling of Multilayer Plastic Films

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    Kevin L. Sánchez‐Rivera, Panzheng Zhou, Min Soo Kim, Leonardo D. González Chávez, Steve Grey, Kevin Nelson, Shao‐Chun Wang, Ive Hermans, Ví­ctor M. Zavala, Reid C. Van Lehn, George W. Huber

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  22. Zinc‐Catalyzed Depolymerization of the End‐of‐Life Poly(ethylene 2,5‐furandicarboxylate)

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  23. Fabricating a Repairable, Recyclable, Imine‐based Dynamic Covalent Thermosetting Resin with Excellent Water Resistance by Introducing Dynamic Covalent Oxime Bonds

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  24. Direct Conversion of Polypropylene into Liquid Hydrocarbons on Carbon‐Supported Platinum Catalysts

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  25. Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis

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  26. Efficient Polyester Hydrogenolytic Deconstruction via Tandem Catalysis

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  27. Green Carbon Science: Efficient Carbon Resource Processing, Utilization, and Recycling towards Carbon Neutrality

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  29. Electrochemical Activation of C−C Bonds through Mediated Hydrogen Atom Transfer Reactions

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  30. Chemical recovery of thermosetting unsaturated polyester resins

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  31. Solid Base Assisted Dual‐Promoted Heterogeneous Conversion of PVC to Metal‐Free Porous Carbon Catalyst

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  32. A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling

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  33. A High‐Throughput Approach to Repurposing Olefin Polymerization Catalysts for Polymer Upcycling

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  34. Thermochemical Conversion of Plastic Waste into Fuels, Chemicals, and Value‐Added Materials: A Critical Review and Outlooks

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  35. Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework

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  36. Catalytic Degradation of Polyethylene Terephthalate Using a Phase‐Transitional Zirconium‐Based Metal–Organic Framework

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  37. Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis

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  38. Multilayer Packaging in a Circular Economy

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  39. “Like Recycles Like”: Selective Ring‐Closing Depolymerization of Poly(L‐Lactic Acid) to L‐Lactide

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  40. “Like Recycles Like”: Selective Ring‐Closing Depolymerization of Poly(L‐Lactic Acid) to L‐Lactide

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  41. A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry

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  42. A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry

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  43. Sustainable recycling technologies for thermoplastic polymers and their composites: A review of the state of the art

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  44. State‐of‐the‐art and future challenges of polymer recycling in the context of circular economy

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  45. Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources

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  46. Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources

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  47. A Highly Dynamic Covalent Polymer Network without Creep: Mission Impossible?

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  48. A Highly Dynamic Covalent Polymer Network without Creep: Mission Impossible?

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  49. Nachhaltiges Design von Struktur‐ und Funktionspolymeren für die Kreislaufwirtschaft

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  50. Sustainable Design of Structural and Functional Polymers for a Circular Economy

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