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RESEARCH PAPER · SusMat · 2022

Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysis

Mingyu Chu, Weilin Tu, Shuangqiao Yang, Congyang Zhang, Qingye Li, Qiao Zhang, Jinxing Chen

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Sustainable chemical upcycling of waste polyolefins by heterogeneous catalysisOriginalPopulation balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution22A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Upcycling of waste artificial turf for high‐performance wood‐plastic composites4Photo-plasma catalytic degradation of high concentration volatile organic compounds18Photocatalytic Oxidative Dehydrogenation of Propane for Selective Propene Production with TiO225Multilevel reconstruction of g-C3N4 nanorings via natural pollen for remarkable photocatalysis10Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Two-dimensional nanomaterials: synthesis and applications in photothermal catalysis50“Functional upcycling” of polymer waste towards the design of new materials226Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Visible-light-driven photoreforming of poly(ethylene terephthalate) plastics via carbon nitride porous microtubes45Thiol–ene Click Chemistry Incorporates Hydroxyl Functionality on Polycyclooctene to Tune Properties30Strategic use of thermo-chemical processes for plastic waste valorization23The greener side of polymers in the light of d-block metal complexes as precatalysts18Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Recyclable thermally conductive poly(butylene adipate‐co‐terephthalate) composites prepared via forced infiltration49Catalyst-free upcycling of crosslinked polyethylene foams for CO2 capture13Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Highly efficient photothermal catalytic upcycling of polyethylene terephthalate via boosted localized heating60Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Chemical Upcycling of Polyolefins through C−H Functionalization50Direct Regeneration of NCM Cathode Material with Aluminum Scraps7Direct recycling of spent Li-ion batteries: Challenges and opportunities toward practical applications114Transition Metal Catalysts for Depolymerization0Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Polyolefin Ionomer Synthesis Enabled by C–H Thioheteroarylation18Excavating the Potential of Photo‐ and Electroupcycling Platforms Toward a Sustainable Future for Waste Plastics11Precise activation of C–C bonds for recycling and upcycling of plastics81Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts19A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters15Heterogeneous catalysis for the environment92Mild aqueous metal catalyzed oxidative conversion of low-density polyethylene to low molecular weight aliphatic carboxylic acids15Water Resistance, Mechanical Properties and Water-Induced Shape Memory Properties of Poly(vinyl Alcohol) Materials Modified by Waste Polyester Depolymerization Monomer3Solar‐Driven Hydrogen Evolution from Value‐Added Waste Treatment29Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Upgrading waste plastics to value-added aromatics30Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Upcycling of Plastic Waste Using Photo-, Electro-, and Photoelectrocatalytic Approaches: A Way toward Circular Economy159Synergism of solar-driven interfacial evaporation and photo-Fenton Cr(VI) reduction by sustainable Bi-MOF-based evaporator from waste polyester78Photothermal Mineralization of Polyolefin Microplastics via TiO2 Hierarchical Porous Layer‐Based Semiwetting Air‐Plastic‐Solid Interfaces30Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19From sustainable macro debris chemical recycling to microplastic reclamation: Overview, research challenges, and outlook9Innovative carbon nanotubes-bridging strategy valorizes plastic waste into high-quality H2-rich syngas while suppressing CO2 emissions21Mechanistic Insight into Heteroatom Removal from Vacuum Gas Oil Blended with PMMA or PET Waste4Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Green Catalytic Ionic Liquids Containing Organophosphorus for Efficient Glycolysis of Waste PET Bottle Flakes14Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Photocatalytic upcycling of plastics containing aliphatic C–C bonds into versatile chemicals9Advances in Nonreactive Polymer Compatibilizers for Commodity Polyolefin Blends102Quantifying microplastics in sediments of Jinzhou Bay, China: Characterization and ecological risk with a focus on small sizes16Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Catalytic Upcycling of Polyolefins316Interfacial solar‐driven steam and electricity co‐generation using Hydrangea‐like graphene by salt‐assisted carbonization of waste polylactic acid94Preparation and Performance of PBAT/PLA/CaCO3 Composites via Solid-State Shear Milling Technology19Applications of nickel-containing structured microfibrous catalysts for the process of propane hydrogenolysis0Fabrication of high performance polypropylene based blends from ethylene vinyl acetate-based sole waste via solid-state shear Co-milling6Cr6+ Loaded Lewis Acidic Sn‐Beta Zeolites as Reusable Catalysts for Selective Production of Light Olefins via Polyolefin Cracking2Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Photothermal Upcycling of Waste Polyvinyl Chloride Plastics27Plastic‐to‐Treasure: Innovative advances in photo/electro‐catalytic upcycling technologies for commodity chemicals and fuels15Polarization-Induced Internal Electric Field-Dominated S-Scheme KNbO3–CuO Heterojunction for Photoreduction of CO2 with High CH4 Selectivity9Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Enhancing Polypropylene/Polyethylene Blend Performance Through Compatibilization for A Sustainable Future: A Mini Review Focusing on Establishing Bio‐Derived Filler Based Hybrid Compatibilizer System31Turning Waste into Valuable Products: Sunlight-Driven Hydrogen from Polystyrene via Porous Tungsten Oxide Photoanodes2Upgrading polyethylene plastic waste into a biodegradable polymer: Harnessing a hybrid chemical oxidation–biological conversion approach18Mechanochemical Recycling of Acid Anhydride-Cured Epoxy Resin for Functional Applications16Enhanced catalytic aminolysis of polyethylene terephthalate plastic wastes via zeolite acid–base site regulation6MODIFICATION OF A POLYETHYLENE AND POLYPROPYLENE BLEND WITH UREA-FUNCTIONALIZED PHENOL-FORMALDEHYDE CO-OLIGOMER1Microwave-assisted pyrolysis of waste LDPE: Unveiling the role of induced gas-solid thermal gradients on pyrolysis oil product distribution20Upcycling wind turbine blades into durable Super-Hydrophobic coating for High-Efficiency Anti-Icing application49Advances in chemical recycling of polyethylene terephthalate (PET) via hydrolysis: A comprehensive review121Barrier properties of polylactic acid to binary aqueous solution systems2Using Nickel-Containing Structured Microfiber Catalysts in the Hydrogenolysis of Propane0Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling21Fabrication of poly(vinyl alcohol)/sulfonated itaconic starch blend film with enhanced antibacterial performance and soil absorption capacity for environment-friendly packaging12Tailored synthesis of circular polyolefins27Electronic Configuration‐Modulated Dual‐Active Nanocomposite NiAlOx for Promoting Plastic‐To‐Green Hydrogen9Hydrocarbon Deposition during Polyolefin Upcycling: Irreversible Adsorption and Surface Reactions of Polyethylene and Ethylene Oligomers on Silica Supports2Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Construction of Multistep Charge Transfer Pathways in Bi 0 @Bi 3+ ‐KNbO 3 for Significantly Accelerated Photoconversion of Waste Plastics13Construction of Multistep Charge Transfer Pathways in Bi 0 @Bi 3+ ‐KNbO 3 for Significantly Accelerated Photoconversion of Waste Plastics2Rheological and thermal investigation of blends of ionically cross-linked and un-modified polypropylene and preparation of carbon black-based electromagnetic wave shielding composites0Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth5Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth2Simple but efficient preparation of high-strength, heat-resistant, and high-barrier PLA/TOBC plastic packaging containers via pickering emulsion5Synergistic Catalysis for Recycling and Upcycling of Plastics35Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3From Waste Plastics to Carbon/Graphene Quantum Dots: A Journey Towards Value-Added Carbon Nanostructures for Various Applications5Enhancing polypropylene/high-density polyethylene blend performance through the incorporation of microcrystalline cellulose-based core-shell particles at the interface9Morphology‐Controlled Rheological and Non‐Isothermal Crystallization Behaviors in Immiscible Polypropylene/High Density Polyethylene Blends1A Review on Sustainable Upcycling of Plastic Waste Through Depolymerization into High-Value Monomer38High-Temperature Size Exclusion Chromatography for Advanced Recycling: Systematic Errors in Analysis of Polyethylene─Alkane Mixtures0Tensile and Structural Properties of Antioxidant- and CaCO3-Modified Polyethylene Films6Study on co-pyrolysis of waste rapeseed oil and low-density polyethylene: Kinetic study and microwave-assisted process optimization5Tandem catalytic cracking of LDPE to C2-C4 olefins over interconnected NZ@Al-meso-SiO2: Role of hierarchical porosity and acidity4Catalytic Depolymerization of Plastics to Valuable Products7Phosphorus-nitrogen synergistic flame retardant system for high-performance polypropylene composites reinforced with recycled wind turbine blade powder10Recent advances in chemical upcycling of plastic waste: microwave-assisted heating and heterogeneous catalysis11One‐Pot Upcycling of Heterogeneous Polyester Waste to Biodegradable Thermoplastics: A Cost‐Effective Solution for a Circular Economy6Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Catalytic Oxidation of Commodity Plastics: Advances in Polyethylene and Polystyrene Valorization5Entropy Engineering for the Efficient Hydrogenolysis of Waste Polyolefins1Upcycling Waste Polyethylene and Polypropylene into Carbon Oxides and Hydrocarbons via a Mechanochemistry-Photocatalysis Combined Technology under Mild Conditions1Beyond mechanical recycling: artificial photosynthesis enables polyester plastic upcycling into valuable chemicals5Carbon-modified TiO 2 catalysts for oxidative upcycling of waste polyethylene to dicarboxylic acids1Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Selective catalytic chlorination: key strategic pathways for renewable resources functionalization to transition away from fossil fuels0Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling0Photothermal catalysis for plastic upcycling: a review on material design and reaction mechanisms2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Innovative Interfacial Compatibilization and Blowing Strategies for Advancing PLA/PBAT Blown Films: Enhancing Film Blowing Stability, Mechanical Properties, and Barrier Properties1Catalyst Control of Alkylbenzene Molecular Architecture in Tandem Catalytic Hydrogenolysis-Aromatization of Polyethylene0Photogenerated hole-mediated oxi-upcycling of polyethylene to dicarboxylic acids over a waste plastic-derived MIL-101(Cr)0

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  1. Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution

    Journal of Materials Chemistry A · 2022-01-01

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  2. A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium

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  3. Upcycling of waste artificial turf for high‐performance wood‐plastic composites

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  4. Photo-plasma catalytic degradation of high concentration volatile organic compounds

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  5. Photocatalytic Oxidative Dehydrogenation of Propane for Selective Propene Production with TiO2

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  6. Multilevel reconstruction of g-C3N4 nanorings via natural pollen for remarkable photocatalysis

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  7. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

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  8. Two-dimensional nanomaterials: synthesis and applications in photothermal catalysis

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  9. “Functional upcycling” of polymer waste towards the design of new materials

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  10. Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production

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  11. Visible-light-driven photoreforming of poly(ethylene terephthalate) plastics via carbon nitride porous microtubes

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  12. Thiol–ene Click Chemistry Incorporates Hydroxyl Functionality on Polycyclooctene to Tune Properties

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  13. Strategic use of thermo-chemical processes for plastic waste valorization

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  14. The greener side of polymers in the light of d-block metal complexes as precatalysts

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  15. Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes

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  17. Catalyst-free upcycling of crosslinked polyethylene foams for CO2 capture

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  18. Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste

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  19. Highly efficient photothermal catalytic upcycling of polyethylene terephthalate via boosted localized heating

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  20. Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites

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  21. Upcycling of polyethylenes by catalysis

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  22. SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

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  23. Chemical Upcycling of Polyolefins through C−H Functionalization

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  24. Direct Regeneration of NCM Cathode Material with Aluminum Scraps

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  27. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

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  28. Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling

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  29. Polyolefin Ionomer Synthesis Enabled by C–H Thioheteroarylation

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  32. Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts

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  33. A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds

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  34. Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters

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  35. Heterogeneous catalysis for the environment

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  36. Mild aqueous metal catalyzed oxidative conversion of low-density polyethylene to low molecular weight aliphatic carboxylic acids

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  40. Upgrading waste plastics to value-added aromatics

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  41. Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling

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  42. Upcycling of Plastic Waste Using Photo-, Electro-, and Photoelectrocatalytic Approaches: A Way toward Circular Economy

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  43. Synergism of solar-driven interfacial evaporation and photo-Fenton Cr(VI) reduction by sustainable Bi-MOF-based evaporator from waste polyester

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  44. Photothermal Mineralization of Polyolefin Microplastics via TiO2 Hierarchical Porous Layer‐Based Semiwetting Air‐Plastic‐Solid Interfaces

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  45. Layered Double Hydroxide Derivatives for Polyolefin Upcycling

    Journal of the American Chemical Society · 2024-04-02

    Mingyu Chu, Xianpeng Wang, Xuchun Wang, Panpan Xu, Zhang Lin, Shengming Li, Kun Feng, Jun Bo Zhong, Lu Wang, Youyong Li, Le He, Muhan Cao, Qiao Zhang, Lifeng Chi, Jinxing Chen

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  46. Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization

    ACS Nano · 2024-04-16

    Qingyun Kang, Xiaofang Zhang, Qianyue Feng, Lin Zhang, Mingyu Chu, Chaoran Li, Panpan Xu, Muhan Cao, Le He, Qiao Zhang, Jinxing Chen

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  47. From sustainable macro debris chemical recycling to microplastic reclamation: Overview, research challenges, and outlook

    Journal of Cleaner Production · 2024-04-22

    Xiang Zhao, Fengqi You

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  48. Innovative carbon nanotubes-bridging strategy valorizes plastic waste into high-quality H2-rich syngas while suppressing CO2 emissions

    One Earth · 2024-05-01

    Xuesong Zhang, Xuesong Zhang, Ge Kong, Yuan Jiang, Linling Zhou, Kejie Wang, Xin Zhang, Xin Zhang, Guanya Ji, Lujia Han

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  49. Mechanistic Insight into Heteroatom Removal from Vacuum Gas Oil Blended with PMMA or PET Waste

    ChemSusChem · 2024-05-15

    Naydu Zambrano, David Trueba, Idoia Hita, Roberto Palos, Josune Azkoiti, Alazne Gutiérrez, Pedro Castaño

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  50. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

    JACS Au · 2024-06-04

    Simin Sun, Wenyu Huang

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