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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Converting Plastic Wastes to Naphtha for Closing the Plastic Loop

Lin Li, Hu Luo, Zilong Shao, Haozhi Zhou, Junwen Lu, Junjun Chen, Chaojie Huang, Shunan Zhang, Xiaofang Liu, Lin Xia, Jiong Li, Hui Wang, Yuhan Sun

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Converting Plastic Wastes to Naphtha for Closing the Plastic LoopOriginalAdvancements in catalysis for plastic resource utilization21Transport limitations in polyolefin cracking at the single catalyst particle level66Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Upcycling Waste Polycarbonate to Poly(carbonate imine) Vitrimers with High Thermal Properties and Unprecedented Hydrolytic Stability42A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Production of C5-C12 olefins by catalytic pyrolysis of low-density polyethylene with MCM-41 in CO2/N223Upcycling of polyethylenes by catalysis0Chemical recycling of polyolefins: a closed-loop cycle of waste to olefins126Functionalizable and Recyclable Aliphatic Polycarbonates Derived from Biomass Feedstocks and CO26From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Mixed Plastics Wastes Upcycling with High-Stability Single-Atom Ru Catalyst188Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Low-temperature catalytic dechlorination of model plastic pyrolytic oil over zeolite catalysts5Self-assembly kieselguhr-based ZSM-5 for catalytic pyrolysis of mask waste to produce high value-added aromatics20Upcycling of Poly(lactic acid) Waste: A Valuable Strategy to Obtain Ionic Liquids10PPAF: A Plastics Production and Accumulation Forecast Model Based on Entropy Weighting for Reducing Global Plastic Waste1Influence of temperatures and loadings on olefin diffusion in MFI-type zeolites in one- to three-dimensions6Rational design principles of single-atom catalysts for hydrogen production and hydrogenation58Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters21Production of Sustainable Aviation Fuel by Hydrocracking of n-Heptadecane Using Pt-Supported Y-Zeolite-Al2O3 Composite Catalysts5Solar‐Driven Hydrogen Evolution from Value‐Added Waste Treatment29Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Strengthening the Metal–Acid Interactions by Using CeO2 as Regulators of Precisely Placing Pt Species in ZSM‐5 for Furfural Hydrogenation35Perspectives on sustainable plastic treatment: A shift from linear to circular economy39High-efficiency Ce-modified ZSM-5 nanosheets for waste plastic upgrading43Selective Hydrocracking of Waste Polyolefins toward Gasoline-Range Liquid Fuels via Tandem Catalysis over a Cerium-Promoted Pt/HY Catalyst37Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Coupled conversion of polyethylene and carbon dioxide catalyzed by a zeolite–metal oxide system50Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6Technical evaluation of low-carbon fuels as a decarbonization pathway of the light-duty transport sector14Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Poisoning effect of polyvinyl chloride on the catalytic pyrolysis of mixed plastics over zeolites31Use of Zero-Valent Iron Nanoparticles (nZVIs) from Environmentally Friendly Synthesis for the Removal of Dyes from Water—A Review48Catalytic chemical recycling and upcycling of polyolefin plastics27Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Stapler Strategies for Upcycling Mixed Plastics49Recycling polyolefin plastic waste at short contact times via rapid joule heating93Insights into the development of greener mild zeolite dealumination routes applied to the hydrocracking of waste plastics29Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking24Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Catalytic Upcycling of Polyolefins316Recent advancement in microplastic removal process from wastewater - A critical review65Catalyst Accessibility and Acidity in the Hydrocracking of HDPE: A Comparative Study of H-USY, H-ZSM-5, and MCM-41 Modified with Ga and Al11Unlocking the structure-activity relationship of hierarchical MFI zeolites towards the hydrocracking of HDPE14Catalytic recycling of plastics into value-added products28Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Solvents and Green Solvents in Polymers and Industry—Devil or Savior?0Machine Learning-Aided 3D Dynamic SERS Strategy for Physiological Mapping: Biotoxicity of Environmentally Dimensional Aged Nanoplastics and Corresponding Protein Corona Complexes10Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Efficient Hydrocracking of Waste Polyethylene into Branched Liquid Fuels over Low Pt‐loaded Nb2O5 Catalyst5Polypropylene Decomposition in Hydrocarbon Solvents: Zeolite-Catalyzed Chemical Recycling5Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Research progress on chemical upcycling of waste polyethylene terephthalate2Transparent Materials Top-Down Constructed by Using Animal Skins for Light Management Application13Accurately tuning the pore size and acidity of mesoporous zeolites for enhancing the catalytic hydrocracking of polypropylene24Synergistic toughening of polylactide by layer structure and network structure3Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes12Catalytic amounts of sodium-sulfonate–naphthol enable mechanically robust, ultra-transparent, super-fire-resistant and easily recyclable polycarbonate8Economical 550 V energy harvesting from plastic and electronic waste using human motions9Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Selective production of a jet fuel fraction through hydrocracking of n -heptadecane using Pt-supported β-zeolite-Al 2 O 3 composite catalysts4Upgrading of waste polyolefins with non-noble metal catalysts21Advanced Catalysts for the Chemical Recycling of Plastic Waste90Catalytic and engineering strategies for enhanced hydrogenation reactions: A review of heterogeneous catalysts and process optimization15Production of low-aromatic oil from catalytic pyrolysis of waste plastics-derived wax16Microwave-assisted pyrolysis of waste LDPE: Unveiling the role of induced gas-solid thermal gradients on pyrolysis oil product distribution20Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8A “polymer-to-polymer” recycling of PET by the dissolution-precipitation strategy20Sequential hydrogenation enhanced by bidirectional hydrogen spillover over cascade catalyst2Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Boosting Degradation of Polyethylene at Room Temperature4Efficient photoreforming of organic solvents into CH4 over 2D donor-π-acceptor conjugated polymers with tunable symmetry8Emerging Biochemical Conversion for Plastic Waste Management: A Review8Enhancing sustainability with lignin-based green adhesives for bamboo bioplastics11Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Upcycling of Waste Plastics into Value-Added Chemicals6Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Zeolites in the epoch of catalytic recycling plastic waste: Toward circular economy and sustainability20Advances in catalytic transformations of waste plastic resources with zeolites0Engineering porous Beta zeolite-encapsulated nickel catalyst for waste polyolefins upcycling26Silicalite-1 zeolite encapsulated Pt nanoparticles via ligand-protected in-situ construction for boosting auto-exhaust carbon particle oxidation3Co-recycling of plastics and other waste materials70Synergistic Catalysis for Recycling and Upcycling of Plastics35Harnessing Synergistic Cooperation of Neighboring Active Motifs in Heterogeneous Catalysts for Enhanced Catalytic Performance26Coordinating cracking and hydrogenation of polyethylene waste via acid-metal site isolation for selective hydrocarbon production10Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics7Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics0Millisecond dwell time enables closed-loop recycling of polypropylene waste plastics: effects of pyrolysis parameters on low-carbon olefin and carbon nanosphere formation9Ambient solar thermal catalysis for polyolefin upcycling using copper encapsulated in silicon nanosheets and chloroaluminate ionic liquid32A Minimalist Design for a Dual-Catalyst System for High-Efficiency Conversion of Waste Plastics into Liquid Fuel Products27Proposal for a Circular Recycling of Hydrocarbon Plastics1Plasma-catalytic cracking of polyethylene over Ni/Hβ zeolites to light hydrocarbon fuels and hydrogen without external heating5Rational design of zeolite-based composite catalysts in catalytic cracking of polyethylene6Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Decoupling the catalytic features of an Fe2O3/USY catalyst in polyethylene pyrolysis using machine learning2Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Synergistic Catalysis Driven by Solvent Effect: Efficient Glycolysis of Polyethylene Terephthalate (PET) by the Zn(OAc) 2 /DBU-DMSO System15Noble Metal‐Free Low‐Temperature Aromatization of Polyethylene Waste for High‐Quality Fuel Production8Noble Metal‐Free Low‐Temperature Aromatization of Polyethylene Waste for High‐Quality Fuel Production3Production of Polymer Monomers through Integrated Catalytic Approaches3High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites65Recyclable Inorganic Subnanowire Plastics8Assessment of thermochemical pathways for sustainable production of high-value chemicals from agroforestry wastes and plastics biorefineries1Upgrading Natural Ores for Efficient Photothermal Polyester Recycling21Tandem catalytic cracking of LDPE to C2-C4 olefins over interconnected NZ@Al-meso-SiO2: Role of hierarchical porosity and acidity4Catalytic Depolymerization of Plastics to Valuable Products7Upgrading waste LiMn2O4 cathode for efficient photothermal polyester recycling20Desalination of MSWI fly ash washing wastewater coupled with in-plant flue gas waste heat: Techno-economic analysis and carbon emission accounting4Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Optimizing the use of pyrolysis waste oil as a feedstock for the naphtha cracking process by hydrotreating and hydrocracking4An Extraordinary Stable and Ultramicroporous Y-MOF for Propylene/Ethylene Separation and Knoevenagel Condensation5Polypropylene Decomposition in Petroleum-based Solvents over Beta Zeolite toward Chemical Recycling0Degradation of Polyvinyl Chloride Microplastics via Hydrothermal Catalysis Using CoMn 2 O 4 Nanofibers3Facile catalytic conversion of spent mulching films to light oil via Fe-modified Al2O31Solvent swelling-induced microstructural modulation of polypropylene for targeted pyrolysis: Product distribution and pyrolysis mechanisms explored through experimental and DFT investigations2A review of recent advances in thermal-catalytic cracking of plastic waste8Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes0Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Transparent materials derived from sheepskin for light conversion application14Upcycling Polyethylene into Separable Aromatics Through Tandem Catalysis with CO2 at Atmospheric Pressure2Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling4Biosourced, Performance‐Tunable, Monomer‐Recyclable Semi‐Aromatic Polyamides: Synthesis and Properties0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Dual advantages of rapid zeolite channel diffusion and Ni sites: 1Ni/L-DAl zeolite enables efficient polyolefin hydrocracking to liquid fuel1Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Zeolite-encapsulated metal catalysts for alkane conversion2Ice template steam-assisted synthesis of multistage porous ZSM-5 boosts catalytic reforming of plastics to produce aromatics2Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Photothermal Oxidative Upcycling of Polyethylene to Aliphatic Dicarboxylic Acids over a Pt/TiO 2 Catalyst10Microwave-driven molecular activation enables efficient hydrogen recovery via low-carbon plastic recycling0Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1

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    Tianyu Wei, Pengcheng Zhou, Wenxian Liu, Xijun Liu, Tairong Kuang

    Read original paper ↗ ·
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