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RESEARCH PAPER · ChemCatChem · 2023

Recent Advances in Catalytic Chemical Recycling of Polyolefins

Kirill Faust, Peter Denifl, Marko Hapke

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Recent Advances in Catalytic Chemical Recycling of PolyolefinsOriginalSynthesis, Characterization and Application of Biobased Unsaturated Polyester Resin Reinforced with Unmodified/Modified Biosilica Nanoparticles33Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Upcycling of Polypropylene Wastes via Catalytically C−H Modification with Polar Olefins12Catalytic and non-catalytic low-pressure hydrothermal liquefaction of pinewood sawdust, polyolefin plastics and their mixtures34Chemical upcycling of PVC-containing plastic wastes by thermal degradation and catalysis in a chlorine-rich environment33Waste to energy: Trending key challenges and current technologies in waste plastic management148A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12Effect of thermal-oxidative and mechanical degradation of recycled LDPE on foaming3Electrochemical recycling of polymeric materials56Fuel Production from Waste Plastics Over Copper/Zeolites2Photochemical upcycling and recycling of plastics: achievements and future opportunities56Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)12Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Tar conversion and recombination in steam gasification of biogenic residues: The influence of a countercurrent flow column in pilot- and demonstration-scale7The catalytic pyrolysis of waste polyolefins by zeolite-based catalysts: A critical review on the structure-acidity synergies of catalysts47Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Perspectives on sustainable plastic treatment: A shift from linear to circular economy39Thermochemical transformation of CO2 into high-value products34Light-driven polymer recycling to monomers and small molecules112Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38A Microkinetic Model for Isomerizing Ethenolysis8Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35References0Upcycling of polyethylene terephthalate (PET) plastic wastes into carbon-based nanomaterials: Current status and future perspectives51Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts5Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Tailoring Olefin Contents Formation during Waste Plastic Pyrolysis12Catalytic Upcycling of Polyolefins316Oxidative degradation and upcycling of polyethylene wastes40Upcycling of recycled polyethylene for rotomolding applications via dicumyl peroxide crosslinking14Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Cross-Linked Polyolefins: Opportunities for Fostering Circularity Throughout the Materials Lifecycle28Chemo‐Enzymatic Depolymerization of Functionalized Low‐Molecular‐Weight Polyethylene46Chemo‐Enzymatische Depolymerisation von funktionalisiertem niedermolekularem Polyethylen1Aquathermolysis of polyolefin plastic wastes over a MOF-derived TiO2 anatase catalyst: Enhancing C–N bond cleavage and coke suppression6Selective catalytic conversion of model olefin and diolefin compounds of waste plastic pyrolysis oil: Insights for light olefin production and coke minimization25Plastic‐to‐Treasure: Innovative advances in photo/electro‐catalytic upcycling technologies for commodity chemicals and fuels15Highly Selective, Catalyst‐Free, and Low Temperature Depolymerizable Styrene Copolymer With Incorporated α‐Methylstyrene Structural Units3Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Chemical bio-manufacture from diverse C-rich waste polymeric feedstocks using engineered microorganisms7Circular plastic economy for sustainable development: current advances and future perspectives49Heterogeneous Fenton-type oxidative degradation of low-density polyethylene to valuable acid products using a nanostructured Fe–CeO 2 solid solution catalyst5Impact of nanofillers on vitrimerization and recycling strategies: a review20Innovative recycling strategies for non-recycled plastics: advancing the circular economy for a sustainable future22Melamine-Doped Plastic-Derived Adsorbents for Carbon Capture: The Influence of Plastic Type on Textural Properties and Co2 Uptake0Melamine-Doped Plastic-Derived Adsorbents for Carbon Capture: The Influence of Plastic Type on Textural Properties and Co2 Uptake0Recycling of HDPE-giant reed composites: Processability and performance3Sustainability in Polyolefins0Tuning solvent strength can fractionate PVC into ultra-low molecular weight material with low dispersity6Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27A Mini-review on Development for the Direct Catalytic Hydroconversion of Polypropylene to Liquid and Gaseous Hydrocarbons for Fuels and Chemicals1Recyclable polyolefin-like materials with weakened all-carbon backbones1Research roadmap for sustainable polymeric materials in Korea9Melt spinning of sustainable high-quality polypropylene from post-consumer waste for monofilaments5Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upcycling depolymerized PET waste into polyhydroxyalkanoates and triacylglycerols by a newly isolated Rhodococcus sp. strain9Upcycling of Waste Plastics into Value-Added Chemicals6Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Hydrothermal Synthesis of AlV‐Rich Nonporous Amorphous Silica‐Alumina for Stable Cracking of Plastics Waste into Light Olefins2Advancements in Catalytic Depolymerization Technologies10Harnessing Biofilm-Mediated Plastic Biodegradation: Innovating Smart Material Design18Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Recent progress in upcycling of plastic-derived intermediates into value-added chemicals via electrocatalytic strategies – A review1Mitigating Extrusion Instabilities and Enhancing Mechanical Performance of Post‐Consumer Recycled Polyolefins via Layer Multiplying Elements7Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Recent advances in chemical upcycling of plastic waste: microwave-assisted heating and heterogeneous catalysis11Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2In Situ Catalytic Pyrolysis of Spent Mulching Film over Fe/Ni/Co-Doped α-Al 2 O 3 for Light Oil and High-Value Aromatics1One step closer to circularity: recycling post-consumer PE-HD into shampoo bottles1A chemically recyclable thermosetting elastomer via ring-opening metathesis polymerization0Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Model-based optimization of properties of post-consumer recycled PP/PE blends via compatibilization3Pincer iridium( iii ) carboxylate catalysts for polyolefin dehydrogenation0Mechanistic Pathways and Product Selectivity in Pyrolysis of PE, PP and PVC: A Foundation for Applied Chemistry in Europe12Varying the Oxidative Functionalization of Polypropylene Films under Quiescent Conditions2Tuning Feedstock-to-Catalyst Ratio for Efficient Coproduction of Hydrogen and Nanocarbon from Polyolefin Waste Pyrolysis1Unexpected Ductility Enhancement in Crystalline–Crystalline Polyolefin Diblock Copolymers without Introducing Soft Segments0Oxidative Extrusion of Polypropylene Melts: Impact of Chain-End and In-Chain Functionalization on Thermal Properties, Crystal Structure, and Crystallization Kinetics1Direct Polymer-on-Polymer Grafting of Polyolefins under Visible Light2Upcycling Waste Polyethylene Into Ultra‐High Thermal Conductivity Composites Through Interface Engineering and Shear‐Induced Orientation1Co-Pyrolysis of Polyolefins and Silicone Rubber: Effects on Mass Balancing, Product Distribution, and Potential Siloxane Recovery2Effect of Radical Initiators on Polypropylene Thermal Deconstruction0Degradation of Polyethylene in the Presence of Nickel(II) 2-Ethylhexanoate0Rheological Modeling in Recycled Polyolefin Systems: A Systematic Review of Model Classification, Applicability, and Limitations for Eco-Composite Design0Recent advances in the directed degradation of polyolefins into oligomers0Design of a Chitinase-Responsive, Depolymerizable Petroleum-Derived Polymer for Circular and Antifouling Materials0Reactive compatibilization strategies for mixed polyolefin waste toward food packaging applications0Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production1Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production0Upgrading Polyolefin Plastics Into Ethanol Using an Integrated Hydrothermal‐Photoelectrocatalytic Strategy0Upcycling of Polycaprolactone via Nonthermal Plasma‐Enhanced Catalytic In Situ Hydrogenolysis at Ambient Pressure0Upcycling of Polycaprolactone via Nonthermal Plasma‐Enhanced Catalytic In Situ Hydrogenolysis at Ambient Pressure0Integrated Retrosynthesis and Large Language Modeling for Chemistry-Informed Circular Chemical Reaction Networks0Biodegradability of Chromium-Free Finished Leather Through ISO 14855-1:2012 and ISO 20136:2020: A Multi-Faceted Analytical Approach0

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  3. Upcycling of Polypropylene Wastes via Catalytically C−H Modification with Polar Olefins

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  4. Catalytic and non-catalytic low-pressure hydrothermal liquefaction of pinewood sawdust, polyolefin plastics and their mixtures

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  5. Chemical upcycling of PVC-containing plastic wastes by thermal degradation and catalysis in a chlorine-rich environment

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  10. Fuel Production from Waste Plastics Over Copper/Zeolites

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  17. Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity

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  18. Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes

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  23. Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels

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  34. Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals

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