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RESEARCH PAPER · ACS Catalysis · 2022

Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review

Zhongwen Dong, Wenjun Chen, Keqing Xu, Yue Liu, Jing Wu, Fan Zhang

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Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical ReviewOriginalCatalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Catalytic conversion of polyethylene into aromatics with Pt/ZSM-5: insights into reaction pathways and rate-controlling step regulation53From waste plastics to layered porous nitrogen-doped carbon materials with excellent HER performance26Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Structure-property relationship of zeolite-Y/cubic ZnS nanohybrid material and its utilization for gaseous phase mercury removal20Tailoring ZSM-5 zeolite through metal incorporation: Toward enhanced light olefins production via catalytic cracking: A minireview49Design of a bifunctional catalyst by alloying Ni with Ru-supported H-beta for selective hydrodeoxygenation of bisphenol A and polycarbonate plastic waste94Coking Reduction of Cr‐loaded Beta Zeolite during Polymer Cracking: Hydrocracking of Aromatics by Synergistic Effect of Cr6+ and Zeolitic Acid Sites8Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Catalytic cracking of low-density polyethylene dissolved in various solvents: product distribution and coking behavior9Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Dendritic copolymers from P-, N- and Si-based monomer and melamine phosphate generate thermal deformation toughening and a rapid charring flame retardant effect in polypropylene60Conversion of low-density polyethylene into monocyclic aromatic hydrocarbons through continuous microwave pyrolysis with ex-situ dual-catalyst beds40Catalytic conversion of n-Dodecane to lower olefins hydrogen carriers over bran-shaped modified MCM-22 zeolite catalyst: SiO2/Al2O3 ratio effects5Review of the Preparation and Application of Porous Materials for Typical Coal-Based Solid Waste27Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants349Conversion of polyethylene to gasoline: Influence of porosity and acidity of zeolites14Encapsulation of carbon-nanodots into metal-organic frameworks for boosting photocatalytic upcycling of polyvinyl chloride plastic80Utilization of Deposited Coke on Zeolites During the Catalytic Cracking of Nitrogen‐Containing Polymer for the Oxygen Reduction Reaction1Experimental Evidence for the Relationship between Al Site Distribution and Catalytic Performance in Methanol-to-Olefins Reaction over ZSM-5 Zeolite33D-printed monolithic ZSM-5@nano-ZSM-5: Hierarchical core-shell structured catalysts for enhanced cracking of polyethylene-derived pyrolysis oils11Accelerated Synthesis of Nanolayered MWW Zeolite by Interzeolite Transformation10Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Chemocatalytic production of sorbitol from cellulose via sustainable chemistry – a tutorial review48Chemical recycling of plastic wastes via homogeneous catalysis: A review78Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Catalyst for lactose hydrolysis based on zeolite Y modified with Fe species by ultrasound treatment7Catalytic upcycling of waste polyethylene to fuels over a nanosized beta zeolite under mild conditions6Enhanced efficiency in plastic waste upcycling: the role of mesoporosity and acidity in zeolites31Fuel Production from Waste Plastics Over Copper/Zeolites2Identification of coke species on Fe/USY catalysts used for recycling polyethylene into fuels18Machine learning thermodynamic perturbation theory offers accurate activation free energies at the RPA level for alkene isomerization in zeolites9Nanoconfinement-Induced Shift in Photooxidative Degradation Pathway of Polystyrene4Selective recovery of light olefins from polyolefin catalyzed by Lewis acidic Sn-Beta zeolites without Brønsted acidity15Population Balance Equations for Reactive Separation in Polymer Upcycling20Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Regulating framework aluminum location towards boosted light olefins generation in ex-situ catalytic pyrolysis of low-density polyethylene18The catalytic pyrolysis of waste polyolefins by zeolite-based catalysts: A critical review on the structure-acidity synergies of catalysts47Upgrading waste plastics to value-added aromatics30Catalytic upcycling plastics with CO2: A novel strategy for carbon waste valorization0Mechanism investigation of acid-tailored USY zeolites via ion exchange in polypropylene cracking7High-efficiency Ce-modified ZSM-5 nanosheets for waste plastic upgrading43Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Effect of Feed Mass, Reactor Temperature, and Time on the Yield of Waste Polypropylene Pyrolysis Oil Produced via a Fixed-Bed Reactor16Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Poisoning effect of polyvinyl chloride on the catalytic pyrolysis of mixed plastics over zeolites31Pioneering Aromatic Generation from Plastic Waste via Catalytic Thermolysis: A Minireview38Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Assessing the Binding of Plastics Additives at Brønsted Acid Sites of Zeolites4Selective and Controllable Cracking of Polyethylene Waste by Beta Zeolites with Different Mesoporosity and Crystallinity33Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking24High Molecular Weight Product Formation in Polyolefin Chemical Recycling: A Comprehensive Review on Primary and Secondary Products18Fast Pyrolysis Product Analysis of Commercial Polyethylenes17Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks38Pyrolytic Depolymerization of Polyolefins Catalysed by Zirconium‐based UiO‐66 Metal–Organic Frameworks10Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Recycling Valuable Phenol from Polycarbonate Plastic Waste Via Direct Depolymerization and Csp2−Csp3 Bond Cleavage Under Mild Conditions8Catalytic Upcycling of Polyolefins316The Support and Bimetallic Synergy Effects in Cu‐Ni/SiO 2 Catalysts for Hydrogenation of Furfural4The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Analysis of catalytic sites in FeY zeolite prepared by sono-assisted exchange of iron (II) ions14Unlocking the structure-activity relationship of hierarchical MFI zeolites towards the hydrocracking of HDPE14Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Review on recent development in catalytic cracking of waste polyolefins: Effect of zeolite-based catalysts and reaction parameters33Silica gel supported Cu nanoparticles for selective reductive etherification of furfural into isopropyl furfuryl ether5Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Highly Efficient Depolymerization of Polycarbonate Enabled by Dispersions of Ultrasmall ZnO Nanoparticles4Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Role of Bifunctional Metal-Promoted Zeolitic Catalyst in Microwave-Assisted Pyrolysis of Polyethylene to Monocyclic Aromatics21Selective catalytic conversion of model olefin and diolefin compounds of waste plastic pyrolysis oil: Insights for light olefin production and coke minimization25Exploring the Morphological Effect of Zeolite Beta on Catalytic Cracking of Polyethylene10Efficient flame retardancy of polypropylene by cobalt ions doped phytate melamine synergized with expandable graphite23Hydroconversion of waste polyethylene plastics under mild conditions using mechanically mixed bifunctional catalysts: Impact of metal-acid balance and proximity9Catalytic Aromatization of Rapid Pyrolysis Gas of Low-density Polyethylene Using a Tandem Reactor0The new developments of the design and application of novel propane dehydrogenation catalysts0Cr6+ Loaded Lewis Acidic Sn‐Beta Zeolites as Reusable Catalysts for Selective Production of Light Olefins via Polyolefin Cracking2Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Shaped zeolites Y for polypropylene cracking22Deciphering Faujasite Zeolite Dealumination at the Atomic Scale13Accurately tuning the pore size and acidity of mesoporous zeolites for enhancing the catalytic hydrocracking of polypropylene24Recent Progress for Designing of Catalysts for Photothermal Conversion of Plastic Wastes48Acid Catalysis Mediated by Aqueous Hydronium Ions Formed by Contacting Zeolite Crystals with Liquid Water18Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy59Upcycling of waste plastics: strategies, status-quo, and prospects3Boosting SAPO-34 catalyst longevity and activity in MTO processes via indium oxide doping: an experimental and theoretical study10Bridging plastic recycling and clean energy production: hydrogen-free catalytic pyrolysis of polyethylene over CuMgAlO x for high-yield diesel fuel generation13Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Exploring the influence of morphological variations in M/CeO 2 catalysts for enhanced CO 2 hydrogenation to C1 products9Exposing active sites in zeolites with fluoropyridines as NMR probe molecules1Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Hydrogen spillover boosts PET upcycling to aviation fuel additives over Co–ReO x catalysts5Influence of functional additives, fillers, and pigments on thermal and catalytic pyrolysis of polyethylene for waste plastic upcycling61Maximizing light olefin production in the cracking of polyethylene using hierarchical acidic–basic zeolites5Mechanistic insights into coke suppression in the methanol-to-olefins process via CeO 2 doping to SAPO-3413Mechano-catalytic conversion of polypropylene over zeolite-based materials6Pyrolysis of municipal solid waste for bio-oil production0Synergetic Effects of P-Toluenesulfonic Acid and Acetatic Acid on the Catalytic Depolymerization of Bisphenol a Polycarbonate Waste into Valuable Chemicals0Synthesis of acidic–basic Y zeolite from kaolin: catalytic and mechanism study in the cracking of polyethylene4Valorization of Waste Plastic Mixtures by Pyrolysis and In-Line Catalytic Cracking on a Hy Zeolite0Zeolite-catalytic pyrolysis of waste plastics: Machine learning prediction, interpretation, and optimization50Catalytic conversion of polyolefins to aromatics by ultra-thin b-axis oriented ZSM-5 zeolite1Recovery of chemicals and energy through thermo-chemical processing of plastic waste33Hydrocracking of polyethylene to high quality liquid fuels over bimetallic catalyst PdAg/HZSM-58Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Discovery of ketene/acetyl as a potential receptor for hydrogen-transfer reactions in zeolites9Photothermocatalytic Wet Reforming of Waste Plastics to Syngas45Cold plasma-assisted co-conversion of polyolefin wastes and CO2 into aromatics over hierarchical Ga/ZSM-5 catalyst24Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Jet Fuel Range Products Produced from Catalytic Pyrolysis of Low-Density Polyethylene with a Bimetallic Mg–Mo/Biochar Catalyst18External acidity as performance descriptor in polyolefin cracking using zeolite-based materials60Upcycling of Waste Plastics into Value-Added Chemicals6Comparison of the Synthesis Method of Zeolite Catalysts Based on Pozzolan, Pumice, and Ignimbrite Applied to the Sustainable Pyrolysis of Polymers2Atomic-Precision Engineering of Single-Atom Alloy Materials for Green Catalysis and Energy Conversion7Zeolites in the epoch of catalytic recycling plastic waste: Toward circular economy and sustainability20Unveiling the Dichotomy Between Cobalt(II)-Exchanged X and Y Faujasite Zeolites via Oxidative Carboxylation of Alkene to Cyclic Carbonate2Advances in catalytic transformations of waste plastic resources with zeolites0Mechanistic insights into coke suppression and enhanced olefin selectivity in mixed metal oxide-modified SAPO-34 for high-performance methanol-to-olefins catalysis21Surface potential charge modulation and sequential etching strategies for optimizing SAPO-34 catalysts in the MTO process: Mechanistic insights into catalytic performance21Exploring novel strategies and integrated systems for photothermal catalytic hydrogen production14Machine learning-driven product prediction and process optimization for catalytic pyrolysis of polyolefin plastics16Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth5Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth2MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Microwave-Assisted Catalytic Upcycling of Plastic Wastes over Heterojunction-Structured Layered Triple Oxides8Synergetic effects of p-toluenesulfonic acid and acetic acid on the catalytic depolymerization of bisphenol A polycarbonate waste into valuable chemicals2Synergistic Catalysis for Recycling and Upcycling of Plastics35Conversion of polypropylene into valued-added gasoline range hydrocarbons by catalytic pyrolysis at atmospheric pressure: different composite catalysts of HZSM-5, HY and MCM-411A review of multi-contaminant risks in textile dyeing sludge pyrolysis: Transformation mechanisms and mitigation strategies12Effect of Silicon Sources on the Synthesis of Nanosized Beta Zeolite Aggregates as Catalysts for Conversion of Lactic Acid to Lactide4Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics7Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics0Revealing the Crucial Roles of Pore Interconnectivity between Zeolitic and Nonzeolitic Components in Enhancing Diffusion and Catalytic Efficiency of Industrial Zeolite-Based Catalysts36Catalytic pyrolysis of low-density polyethylene to produce sustainable aviation fuel fractions: Improving isomerized alkane selectivity via magnetic metal-modified HY zeolites6Selective Upcycling of Aromatic Polymer Waste into Light C6C9 Aromatics Over Ru‐Supported Catalysts6Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Hydrothermal Synthesis of AlV‐Rich Nonporous Amorphous Silica‐Alumina for Stable Cracking of Plastics Waste into Light Olefins2Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Zeolite-based catalysis for plastic waste recycling: Sustainable solutions from laboratory testing to industrial applications24Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Increasing para-Xylene Selectivity during Polyolefins to Aromatics via an Olefin Intermediate Tandem Catalysis Process1

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