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RESEARCH PAPER · ChemSusChem · 2022

Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous Catalysis

Tian Tan, Wei Wang, Kai Zhang, Zixiang Zhan, Weiping Deng, Qinghong Zhang, Ye Wang

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Upcycling Plastic Wastes into Value‐Added Products by Heterogeneous CatalysisOriginalHighly Efficient Removal of Aromatic Diamines from the Polyurethane Bio-Hydrolysate by Mil-53 Series Mofs23First-Generation Organic Reaction Intermediates in Zeolite Chemistry and Catalysis107Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Circular Upcycling of Bottlebrush Thermosets14Circular Upcycling of Bottlebrush Thermosets3Boosting 3-Acetamido-5-Acetylfuran Production from N-Acetyl-D-Glucosamine in Γ-Valerolactone by a Dissolution-Catalytic Effect0Functionalization of polyethylene with hydrolytically-stable ester groups6MXene-cellulose nanofiber composites: toward green, multi-functional, flexible, and highly efficient electromagnetic interference shielding materials26An Integrated Plasma–Photocatalytic System for Upcycling of Polyolefin Plastics63Metal Oxides‐Based Nano/Microstructures for Photodegradation of Microplastics51Catalytic Cracking of Polylactic Acid to Acrylic Acid19Preparing Fuel-Range Chemicals via the Direct and Selective Pyrolysis of Disposable Mask Waste for Sustainable Environment4HBpin/MoO2Cl2(H2O)2 as an efficient catalytic system for the reduction of esters, lactones and polyester plastic waste16Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66PET Waste Recycling into BTX Fraction Using In Situ Obtained Nickel Phosphide18Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Novel catalysts in catalytic upcycling of common polymer wastes262023 Highlights in Interface Science and Engineering: A Collection of Virtual Special Issues4Bead Mill-driven Acceleration of Catalytic Methanolysis of Poly(ethylene terephthalate) under Mild Reaction Conditions6Solar-driven reforming of waste polyester plastics into hydrogen over CdS/NiS catalyst54Depolymerization of Polyester and Polycarbonate Waste using HBpin and Cheap Zinc Catalysts21Efficient Depolymerization of Polyester and Polycarbonate Plastic Waste Catalyzed by Commercially Available Homogeneous and Heterogeneous Manganese Catalysts28Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Coupling electrochemical CO 2 reduction with value-added anodic oxidation reactions: progress and challenges23Boosting 3-acetamido-5-acetylfuran production from N-acetyl-D-glucosamine in γ-valerolactone by a dissolution-dehydration effect24Catalytic depolymerization of polyester plastics toward closed-loop recycling and upcycling127Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Production of carbon nanotubes via catalytic pyrolysis of waste plastics over Ni/Al2O3 catalyst: The influence of plastic types54Co-production of hydrogen and carbon nanotubes via catalytic pyrolysis of polyethylene over Fe/ZSM-5 catalysts: Effect of Fe loading on the catalytic activity50Valorization of Plastic Wastes for the Development of Adsorbent Designed for the Removal of Emerging Contaminants in Wastewater2Advances in catalytic chemical recycling of synthetic textiles43Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters15Potential strategies for bioremediation of microplastic contaminated soil65Solvent-free chemical upcycling of poly(bisphenol A carbonate) and poly(lactic acid) plastic waste using SBA-15-functionalized basic ionic liquids48Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Zeolite‐Based Catalysts for Conversion of Oxygenated Polymer Waste by Positron Annihilation9Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Hybrid Oxidation of Microplastics with Fenton and Hydrothermal Reactions17Emerging green approaches for valorization of plastics with saturated carbon backbones42Recent advances in nanotechnology-based modifications of micro/nano PET plastics for green energy applications26Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Conversion of Waste Plastics into Value‐added Materials: A Global Perspective7Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38A Microkinetic Model for Isomerizing Ethenolysis8Enhanced catalytic hydrogenolysis of natural rubber to natural gas over Ru/ZrO2 via phase control strategy15A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy60Production of liquid hydrocarbon fuels through catalytic cracking of high and low-density polyethylene medical wastes using fly ash as a catalyst22Mg(OTf)2 as an Excellent Catalyst for the Reductive Depolymerization and Methanolysis of Polyesters and Polycarbonates17Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Methanolysis of Plastic Waste with Manganese Compounds10Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Highly Efficient Recycling Waste Plastic into Hydrogen and Carbon Nanotubes through a Double Layer Microwave‐Assisted Pyrolysis Method9Insight into the Competitive Adsorption Behavior of Polymer Chains in Silica Nanopores by Small-Angle Neutron Scattering3Catalytic Upcycling of Polyolefins316The application of spent catalysts from catalytic pyrolysis of plastic waste as solid functional materials5Hydroborative Depolymerization of Polyesters and Polycarbonates to Diols Catalyzed by Heterogeneous Lanthanum Materials La(CH2C6H4NMe2-o)3@SBA-155Functionalization and Repurposing of Polypropylene to a Thermoset Polyurethane13Upcycling of monomers derived from waste polyester plastics via electrocatalysis38Circular Economy and Chemical Conversion for Polyester Wastes23Introduction of Environmental Materials and Relevant Technologies0Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Aerobic oxidation of alkylarenes and polystyrene waste to benzoic acids via a copper-based catalyst28Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy59Current methods for plastic waste recycling: Challenges and opportunities64Induction Heating for the Electrification of Catalytic Processes51Electrothermal upcycling of plastic waste18Enhanced catalytic aminolysis of polyethylene terephthalate plastic wastes via zeolite acid–base site regulation6Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Morphology-tuned MnO x /TiO 2 nanocatalysts for recycling PET plastic waste using biomass-derived ethylene glycol15PET-derived heteroatom-doped carbon quantum dots as color-modulated solid-state fluorescent materials13Structural and electronic tuning of hybrid metal thiocyanate N -oxides0Hydrocracking of polyethylene to high quality liquid fuels over bimetallic catalyst PdAg/HZSM-58Photocatalytic upcycling of polylactic acid to alanine by sulfur vacancy-rich cadmium sulfide103A Mini-review on Development for the Direct Catalytic Hydroconversion of Polypropylene to Liquid and Gaseous Hydrocarbons for Fuels and Chemicals1CO2-mediated pyrolysis for syngas generation from wood-plastic composite waste6Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling21Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Comparison of the Synthesis Method of Zeolite Catalysts Based on Pozzolan, Pumice, and Ignimbrite Applied to the Sustainable Pyrolysis of Polymers2Advances in catalytic transformations of waste plastic resources with zeolites0Plastic pollutants: From wastes to fuels and high-value chemicals8Recycling Methods of Plastic Materials for Circular and Sustainable Production Design: A Review1Comparison of In Situ Formed Metal (Mo, W) Phosphides and Oxides in the Hydroprocessing of Used PET Bottles4Upcycling of waste PET via reprocessable thermoset-like covalent adaptable networks12Atomic Cu–O–Zr Sites for Highly Selective Production of p ‐xylene from Tandem Upcycling of PET and CO 216Atomic Cu–O–Zr Sites for Highly Selective Production of p ‐xylene from Tandem Upcycling of PET and CO 20Reductive depolymerization of polycarbonates and polyesters using alkaline earth catalysts6Synergistic torrefaction of plastic polymers and biomass8Solar-driven plastic waste conversion: A mini-review on photoreforming for Co-producing hydrogen and chemical feedstocks7Waste plastic-derived carbon materials for supercapacitors and rechargeable batteries27From waste to value: Synthesis of diols from polyester and polycarbonate plastics using commercial iron catalysts0Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Experimental investigation and lumped kinetic modeling studies for upcycling of polyolefins1Dynamics of inverse metal oxides on metal catalysts using spectro-kinetics: reversible Brønsted acid site formation and irreversible reduction2An anthraquinone-based covalent organic framework for sustainable photocatalytic oxidative degradation of polystyrene3Circular economy in polystyrene photodegradation to valuable chemicals0Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Primary Treatment of Synthetic Plastic Waste Materials0Photothermal Oxidative Upcycling of Polyethylene to Aliphatic Dicarboxylic Acids over a Pt/TiO 2 Catalyst10Polyurethane Recycling: Sustainable Development Perspectives and Innovative Approaches4Highly Selective Gasoline Production by Polyethylene Hydrogenolysis Using Ternary RuNiPt Nanoalloy Catalyst1Single-Atom Nickel Dispersed on Mo 2 TiC 2 T x MXene for Upcycling of Polyolefins via Catalytic Hydropyrolysis for Fuels and Lubricants0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Engineering Zeolite Synthesis for the Green Energy Transformation1Ambient-pressure conversion of plastic waste to jet fuel cycloalkanes by tandem hydropyrolysis and vapour-phase hydrogenation2Advances in Electrocatalytic Upcycling of Polyethylene Terephthalate to Value‐Added Chemicals1Toward Full-Range Recycling of Disposable Diapers0Valorization of Textile Waste: Enzymatic Upcycling of Terephthalic Acid Toward a Sustainable PET Value Chain0

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  1. Highly Efficient Removal of Aromatic Diamines from the Polyurethane Bio-Hydrolysate by Mil-53 Series Mofs

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  3. Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review

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  12. Catalytic Cracking of Polylactic Acid to Acrylic Acid

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  14. HBpin/MoO2Cl2(H2O)2 as an efficient catalytic system for the reduction of esters, lactones and polyester plastic waste

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  15. Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes

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  16. PET Waste Recycling into BTX Fraction Using In Situ Obtained Nickel Phosphide

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  17. Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste

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  20. Bead Mill-driven Acceleration of Catalytic Methanolysis of Poly(ethylene terephthalate) under Mild Reaction Conditions

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  21. Solar-driven reforming of waste polyester plastics into hydrogen over CdS/NiS catalyst

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  22. Depolymerization of Polyester and Polycarbonate Waste using HBpin and Cheap Zinc Catalysts

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  49. Production of liquid hydrocarbon fuels through catalytic cracking of high and low-density polyethylene medical wastes using fly ash as a catalyst

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  50. Mg(OTf)2 as an Excellent Catalyst for the Reductive Depolymerization and Methanolysis of Polyesters and Polycarbonates

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