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RESEARCH PAPER · Applied Catalysis B: Environmental · 2022

A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium

Cong Wang, Kewei Yu, Boris Sheludko, Tianjun Xie, Pavel A. Kots, Brandon C. Vance, Pawan Kumar, Eric A. Stach, Weiqing Zheng, Dionisios G. Vlachos

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A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over rutheniumOriginalHydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Polyethylene Valorization by Combined Chemical Catalysis with Bioconversion by Plastic-Enriched Microbial Consortia26Recent Advances in Catalytic Chemical Recycling of Polyolefins104Techno-Economic and Life Cycle Analyses of Thermochemical Upcycling Technologies of Low-Density Polyethylene Waste116Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Mechanistic Understanding of Ring-Opening of Tetrahydrofurfuryl Alcohol over WOx-Modified Pt Model Surfaces and Powder Catalysts16Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Comparison study of the effects of different synthesis methods towards Ag 2 O / TiO 2 nanowires’ morphology and catalytic activity on the 4-nitrophenol reduction reaction4Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey4Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions15Superstructure optimization for management of low-density polyethylene plastic waste24Controlling Product Distribution of Polyethylene Hydrogenolysis Using Bimetallic RuM3 (M = Fe, Co, Ni) Catalysts28Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Suppression of methane formation as catalytic converting light hydrocarbons into H2 and carbon nanotubes2Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24The Role of Mo Single Atoms and Clusters in Enhancing Pt Catalyst for Benzene Hydrogenation: Distinguishing Between Benzene Spillover and Electronic Effect30Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Hydrogenolysis of Poly(Ethylene‐co‐Vinyl Alcohol) and Related Polymer Blends over Ruthenium Heterogeneous Catalysts7Effect of reaction media on hydrogenolysis of polyethylene plastic waste: Polymer-surface interactions in small alkane/polymer blends35Predicting hydrogenolysis reaction barriers of large hydrocarbons on metal surfaces using machine learning: Implications for polymer deconstruction15Pt enhanced C–H bond activation for efficient and low-methane-selectivity hydrogenolysis of polyethylene over alloyed RuPt/ZrO264Selective Upcycling of Polyethylene over Ru/H‐ZSM‐5 Bifunctional Catalyst into High‐Quality Liquid Fuel at Mild Conditions31Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Effect of CeO2 morphology and Ru impregnation method on CH4 selectivity reduction in polyethylene waste conversion to liquid fuels and lubricants15Towards circularity of plastics: A materials informatics perspective15Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Upcycling of Plastic Waste0Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Efficient upgrading of polystyrene plastics to nitriles through a catalytic oxidative amination process9Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Recent developments in recycling of post-consumer polyethylene waste33Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Design of the Transition for Sustainable Plastic Waste Management under Carbon Policies in the United States11Effective Methane Suppression in Upcycling of Polyethylene into Fuels via Alloying Platinum with Ruthenium Supported on ZSM-5 Zeolite17Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Upcycling of Waste Plastics into Value-Added Chemicals6Catalytic Upgrading of Plastic Wastes into High-Value Carbon Nanomaterials: Synthesis and Applications59Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Predicting a generalized mechanism of branched alkane hydrogenolysis on Ru, Ir, and Pt surfaces relevant to polymer upcycling applications3Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20The silent partner in catalysis: How support architectures dictate efficiency in polyolefin hydrogenolysis1Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Selective hydrocracking of polystyrene waste over Pt- and Ru-supported zeolite catalysts into high yield LPG and ethylbenzene4Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Carbon–carbon bond cleavage for lignin and plastics deconstruction0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Techno-Economic and Life Cycle Assessment of Chemical Recycling and Upcycling of Mixed Plastics Waste Containing Poly-vinyl-chloride7Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Highly Selective Gasoline Production by Polyethylene Hydrogenolysis Using Ternary RuNiPt Nanoalloy Catalyst1Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Design and analysis of a new Ru-Cu/ZSM-5 bimetallic catalyst for hydrogenolysis of polyolefin waste0Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0Highly active and selective heterogeneous Ru/La2O3-CeO2 catalyst for hydrogenolysis of LDPE to valuable chemicals0

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