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RESEARCH PAPER · Angewandte Chemie International Edition · 2023

Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide

Qimin Zhou, Deliang Wang, Qingyue Wang, Kailin He, Khak Ho Lim, Xuan Yang, Wenjun Wang, Bo‐Geng Li, Pingwei Liu

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Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten TrioxideOriginalHeterogeneous catalysis for the environment92Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters21Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Chemical Upcycling of Polylactic Acid Plastic Waste into Alanine over Ru/CeO 2 with Decoration of Indium20Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Constructing the Al deficiency in Si-O(H)-Al units based on Pt/ZSM-5 for enhanced hydrocracking of polyethylene into high-quality liquid fuel20Catalytic Upcycling of Polyolefins316Chemical recycling of polyolefin waste: from the perspective of efficient pyrolysis reactors13Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Enhancing oil shale pyrolysis using metal-doped carbon quantum dot catalysts: A comprehensive behavioral, kinetic, and mechanistic analysis18Oxidative Upcycling of Polyolefin Wastes into the Dynamically Cross-Linked Elastomer25Efficient Hydrocracking of Waste Polyethylene into Branched Liquid Fuels over Low Pt‐loaded Nb2O5 Catalyst5Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst27Production of Branched Alkanes by Upcycling of Waste Polyethylene over Controlled Acid Sites of SO 4 /ZrO 2 ‐Al 2 O 3 Catalyst6Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Upcycling of Polyethylene Wastes to Valuable Chemicals over Group VIII Metal‐decorated WO 3 Nanosheets6Enhanced Pyrolysis of Low to Medium Maturity Oil Shale with Lanthanide and Nitrogen Co-doped Carbon Quantum Dot Catalysts: Mechanistic Insights and Kinetic Implications0Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Co-recycling of plastics and other waste materials70Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels4Synergistic Catalysis for Recycling and Upcycling of Plastics35Current developments in multifunctional technology for waste plastic chemical recycling and case studies0Fully exposed Ptn cluster catalysts enable cascade oxidation of polyol to dicarboxylic acid20Production of Polymer Monomers through Integrated Catalytic Approaches3CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20Efficient Decarbonylation of Fatty Acids to Long-Chain Alkenes by Ordered Mesoporous N-Doped Carbon-Supported Co Single-Atom Catalysts3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Anion Shielding in Nb‐WO 3 /WS 2 Heterostructures: A Strategy for Efficient and Corrosion‐Resistant Seawater Electrolysis15Solar-Driven Upcycling of Polylactic Acid to Alanine over Pt/CdS–TiO 2 Heterojunction Single-Atom Photocatalyst35Bayesian Optimization of Hierarchical ZSM-5 for High-Efficiency Polyolefin Waste Recycling to Light Olefins7Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes0Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Single-Atom Ni on Tungsten Oxides Drives Hydrogen Spillover for Efficient Plastic Waste Upcycling13Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Direct upcycling of mixed plastic waste into liquid alkanes3Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis6Engineering Microporous Zn-Functionalized Carbon Catalysts for Controllable Chain Cracking and Aromatization in Polyethylene Upcycling1Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts6Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Adaptive Brønsted Acidity From Heterolytic Dihydrogen Activation Enables Polyethylene Hydrogenolysis Over Pd‐Encapsulated Na‐Zeolites2Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Bifunctional RhRu Dual-Atom Catalyst Drives the Tandem Degradation of Polystyrene for Highly Selective Production of Toluene0Confined Isomerization Enables Solar-Thermal Upcycling of Polyolefins into High-Octane Gasoline0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0

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