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RESEARCH PAPER · ACS Catalysis · 2022

Rational Design of Chemical Catalysis for Plastic Recycling

Mingyu Chu, Yu Liu, Xiangxi Lou, Qiao Zhang, Jinxing Chen

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Rational Design of Chemical Catalysis for Plastic RecyclingOriginalCatalytic cascade vapor-phase hydrotreatment of plastic waste into fuels and its sustainability assessment18La( iii )-Catalysed degradation of polyesters to monomers via transesterifications38Population balance models for polymer upcycling: signatures of the mechanism in the molecular weight evolution22Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling32Catalytic Upcycling of Plastic Waste into High Value-added Chemicals0Plastic Waste Valorization by Leveraging Multidisciplinary Catalytic Technologies169Solar-driven catalytic plastic upcycling87A general strategy and a consolidated mechanism for low-methane hydrogenolysis of polyethylene over ruthenium107Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics49Catalytic deconstruction of waste polyethylene with ethylene to form propylene419Upcycling disposable face masks into fuel range iso-alkanes through hydropyrolysis coupled with vapor-phase hydrocracking13Photothermal Catalytic Polyester Upcycling over Cobalt Single‐Site Catalyst129Biologically bound nickel accelerated de-polymerization of polyethylene to high value hydrocarbons and hydrogen12Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Upcycling Waste Poly(ethylene terephthalate) into a Porous Carbon Cuboid through a MOF-Derived Carbonization Strategy for Interfacial Solar-Driven Water–Thermoelectricity Cogeneration90Mechanochemistry Milling of Waste Poly(Ethylene Terephthalate) into Metal–Organic Frameworks85Recent progress in photoelectrocatalysis beyond water oxidation46Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Advancements in catalysis for plastic resource utilization21Catalytic conversion of polyethylene into aromatics with Pt/ZSM-5: insights into reaction pathways and rate-controlling step regulation53Efficient depolymerization of PET over Ti-doped SBA-15 with abundant Lewis acid sites via glycolysis35Hydrolytic depolymerisation of polyesters over heterogeneous ZnO catalyst26Metal-free recycling of waste polyethylene terephthalate mediated by TBD protic ionic salts: the crucial role of anionic ligands23Selective deconstruction of mixed plastics by a tailored organocatalyst70Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90State of the art in the photochemical degradation of (micro)plastics: from fundamental principles to catalysts and applications112Ti–Fe2O3/Ni(OH) as an efficient and durable photoanode for the photoelectrochemical catalysis of PET plastic to formic acid64Concerted and Selective Electrooxidation of Polyethylene‐Terephthalate‐Derived Alcohol to Glycolic Acid at an Industry‐Level Current Density over a Pd−Ni(OH) 2 Catalyst17Concerted and Selective Electrooxidation of Polyethylene‐Terephthalate‐Derived Alcohol to Glycolic Acid at an Industry‐Level Current Density over a Pd−Ni(OH) 2 Catalyst295Acidic deep eutectic solvent assisted mechanochemical delignification of lignocellulosic biomass at room temperature77Microbial Enzyme Biotechnology to Reach Plastic Waste Circularity: Current Status, Problems and Perspectives104Depolymerization of Polyesters by Transesterification with Ethanol Using (Cyclopentadienyl)titanium Trichlorides19Upcycling plastic waste to carbon materials for electrochemical energy storage and conversion109Diverse Alkyl–Silyl Cross-Coupling via Homolysis of Unactivated C(sp 3 )–O Bonds with the Cooperation of Gold Nanoparticles and Amphoteric Zirconium Oxides50Analysis of the Scale of Global Human Needs and Opportunities for Sustainable Catalytic Technologies42Oxygen Vacancy Promoted Generation of Monatomic Oxygen Anion over Ni 2+ ‐Doped MgO for Efficient Glycolysis of Waste PET**14Trends in Polyester Upcycling for Diversifying a Problematic Waste Stream50Enzymes’ Power for Plastics Degradation589Enantioselectivity and origin of enhanced efficiency in polyethylene terephthalate hydrolases catalyzed depolymerization11Metal-catalyzed plastic depolymerization79Rational design of photo− /electro−catalytic systems for the transformation of plastic wastes51Biodegradation in Composting Conditions of PBEAS Monofilaments for the Sustainable End‐Use of Fishing Nets14Preparation of monocyclic aromatic hydrocarbons from chlorine-containing mixed waste plastics via tandem catalysis coupled with hydrothermal pretreatment27Catalyst Design to Address Nylon Plastics Recycling4Reconstruction of new high-performance epoxy thermoset based on the full utilization of the degradation products of waste epoxy thermoset26Mass transfer in catalytic depolymerization: External effectiveness factors and serendipitous processivity in stagnant and stirred melts31Accurate Layer Spacing Matching of Polyoxometalate (POM) Anion‐based Ionic Liquids (ILs) to Promote PET Alcoholysis12Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Zeolite Supported Pt for Depolymerization of Polyethylene by Induction Heating18Net Zero Transition: Possible Implications for Catalysis36Highly efficient photothermal catalytic upcycling of polyethylene terephthalate via boosted localized heating60A comprehensive review of separation technologies for waste plastics in urban mine70A focused review on recycling and hydrolysis techniques of polyethylene terephthalate205Novel catalysts in catalytic upcycling of common polymer wastes26Systemically Understanding Aqueous Photocatalytic Upgrading of Microplastic to Fuels11Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Upcycling of polyvinyl chloride to hydrocarbon waxes via dechlorination and catalytic hydrogenation50Catalytic Fabric Recycling: Glycolysis of Blended PET with Carbon Dioxide and Ammonia59Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Polymer composites of biobased aliphatic polyesters with natural abundant fibers that improve the mechanical properties7Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers94Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers14Mechanistic Insights Enable Divergent Product Selectivity in Catalyst-Controlled Photooxidative Degradation of Polystyrene90Direct Regeneration of NCM Cathode Material with Aluminum Scraps7Bead Mill-driven Acceleration of Catalytic Methanolysis of Poly(ethylene terephthalate) under Mild Reaction Conditions6Direct recycling of spent Li-ion batteries: Challenges and opportunities toward practical applications114Chemical Upcycling of PET into a Morpholine Amide as a Versatile Synthetic Building Block27Green recycling of waste PET plastic monomers by banana peel extract32Highly Efficient Depolymerization of Waste Polyesters Enabled by Transesterification/Hydrogenation Relay Under Mild Conditions4Highly Efficient Depolymerization of Waste Polyesters Enabled by Transesterification/Hydrogenation Relay Under Mild Conditions87From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Homogeneous Catalysis in Plastic Waste Upcycling: A DFT Study on the Role of Imperfections in Polymer Chains15Magnetic induction assisted pyrolysis of plastic waste to liquid hydrocarbons on carbon catalyst21Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling72Entropy Confinement Promotes Hydrogenolysis Activity for Polyethylene Upcycling8Catalyst metal-ligand design for rapid, selective, and solventless depolymerization of Nylon-6 plastics70Thermodynamic and Kinetic Insights into Hydrogen Adsorption and Dissociation on the Ru (0001) Surface under STM and Catalytic Conditions11Upcycling of waste PET into high-performance and multifunctional materials27Precise activation of C–C bonds for recycling and upcycling of plastics81Enhancing coking resistance of ZSM-5 in the conversion of pine sawdust into oxygen-free bio-aromatic hydrocarbons through tandem catalytic hydropyrolysis/vapor-phase hydrotreatment13Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Highly selective pressure-dependent (transfer) hydrogenative depolymerization of polybutylene succinate9Monomer recycling of polyethylene terephthalate, polycarbonate and polyethers: Scalable processes to achieve high carbon circularity62Waste to energy: Trending key challenges and current technologies in waste plastic management148A review on microplastics degradation with MOF: Mechanism and action32Advances in catalytic chemical recycling of synthetic textiles43Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters15Catalytic function of ionic liquids in polyethylene terephthalate glycolysis by molecular dynamics simulations4Complete Conversion of Waste Pet into Dimethyl Terephthalate and Ethylene Carbonate0Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Heterogeneous catalysis for the environment92Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis0On the metal- and bio-catalyzed solvolysis of polyesters and polyurethanes wastes7Photoreforming of Poly(Ethylene-Terephthalate) Plastics into Valuable Chemicals and Hydrogen Over Bivo4/Moox: Synergistic Promotion of Oxidation and Reduction Processes0Rational design principles of single-atom catalysts for hydrogen production and hydrogenation58Recent advances in oxidative degradation of plastics227Research Progress in Depolymerization of Polyethylene Terephthalate into High Value-Added Chemicals2Solvent-free chemical upcycling of poly(bisphenol A carbonate) and poly(lactic acid) plastic waste using SBA-15-functionalized basic ionic liquids48Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Synthesis of α-methylene-δ-valerolactone and its selective polymerization from a product mixture for concurrent separation and polymer production6Alcoholysis of oxyphenylene-based super engineering plastics mediated by readily available bases11Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst5Solvent-Promoted Catalyst-Free Recycling of Waste Polyester and Polycarbonate Materials39Photo- and electrochemical processes to convert plastic waste into fuels and high-value chemicals45Population Balance Equations for Reactive Separation in Polymer Upcycling20Synthesis of Polyesters Containing Long Aliphatic Methylene Units by ADMET Polymerization and Synthesis of ABA-Triblock Copolymers by One-Pot End Modification and Subsequent Living Ring-Opening Polymerization10Tandem catalysis enables chlorine-containing waste as chlorination reagents48Polymeric Carbon Nitride Nanosheets as a Metal‐Free Heterogeneous Catalyst for Highly Efficient Methanolysis of Polycarbonates14Upcycling of waste poly(lactic acid) into crumped carbon nanosheet towards high-performance interfacial solar-driven evaporation15Industrialized fine physical regeneration process and economic benefit assessment for recycling waste HDPE containers13Depolymerization of Polyester Fibers with Dimethyl Carbonate-Aided Methanolysis52Upcycling of Plastic Waste Using Photo-, Electro-, and Photoelectrocatalytic Approaches: A Way toward Circular Economy159Cu Promoted the Dynamic Evolution of Ni-Based Catalysts for Polyethylene Terephthalate Plastic Upcycling140Grave-to-cradle photothermal upcycling of waste polyesters over spent LiCoO2111Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Catalytic aquathermolysis of contaminated polyolefin plastic waste over an in situ iron hydroxide/oxide nanocatalyst derived from an oil-soluble iron precursor16Coupling Waste Plastic Upgrading and CO 2 Photoreduction to High-Value Chemicals by a Binuclear Re–Ru Heterogeneous Catalyst77Emerging Photoreforming Process to Hydrogen Production: A Future Energy106From Polyester Plastics to Diverse Monomers via Low‐Energy Upcycling65Full valorisation of waste PET into dimethyl terephthalate and cyclic arylboronic esters61Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes into Cycloalkanes and Aromatics11Coupling pyrolysis and catalytic reforming of waste plastics for syngas production over confined Ni within silicalite-1 catalysts5CO2-enhanced PET depolymerization by catalyst free methanolysis13Extended producer responsibility practices and prospects for waste management in Japan15Iron‐Catalyzed Oxidative Deconstruction of Polyethylene Terephthalate to Terephthalic Acid under O223Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Poisoning effect of polyvinyl chloride on the catalytic pyrolysis of mixed plastics over zeolites31Regioselective enzymatic depolymerization of aromatic-aliphatic polyester revealed by computational modelling7Optimization of polyethylene terephthalate biodegradation using a self-assembled multi-enzyme cascade strategy25Sustainable upcycling of waste polyethylene terephthalate into hierarchically porous carbon nanosheet for interfacial solar steam and hydroelectricity generation17Hydrogenation of the benzene rings in PET degraded chemicals over meso-HZSM-5 supported Ru catalyst32Photocatalytic Cracking of non‐Biodegradable Plastics to Chemicals and Fuels1Photocatalytic Cracking of non‐Biodegradable Plastics to Chemicals and Fuels16Photoreforming of poly(ethylene-terephthalate) plastic into valuable chemicals and hydrogen over BiVO4/MoOx: Synergistic promotion of oxidation and reduction processes71Hydrolase-Catalyzed Depolymerization Mechanism toward Crystalline and Amorphous Polyethylene Terephthalate19Chemical upcycling of polyolefins into liquid refinery feedstock from the circularity and chemical engineering aspects11Assessing the Binding of Plastics Additives at Brønsted Acid Sites of Zeolites4Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction22High value-added conversion and functional recycling of waste polyethylene terephthalate (PET) plastics: A comprehensive review52Plastic upgrading via catalytic pyrolysis with combined metal-modified gallium-based HZSM-5 and MCM-4110Enhancement of terephthalic acid recovered from PET waste using a combination of citric acid and dimethyl sulfoxide extraction7Utilization of Poly(Ethylene Terephthalate) Waste Bottle into Disodium Terephthalate: A Sustainable Electrolyte for Visible to Near‐Infrared Broadband Electrochromic Modulation2Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26

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  4. Multiscale modeling of hydrogenolysis of ethane and propane on Ru(0001): Implications for plastics recycling

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  47. Accurate Layer Spacing Matching of Polyoxometalate (POM) Anion‐based Ionic Liquids (ILs) to Promote PET Alcoholysis

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  49. Zeolite Supported Pt for Depolymerization of Polyethylene by Induction Heating

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