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RESEARCH PAPER · ACS Sustainable Chemistry & Engineering · 2023

Tuning High-Density Polyethylene Hydrocracking through Mordenite Zeolite Crystal Engineering

Pavel A. Kots, Panagiota A. Doika, Brandon C. Vance, Sean Najmi, Dionisios G. Vlachos

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Tuning High-Density Polyethylene Hydrocracking through Mordenite Zeolite Crystal EngineeringOriginalQuantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling12Toward Intrinsic Catalytic Rates and Selectivities of Zeolites in the Presence of Limiting Diffusion and Deactivation50Solar-driven photocatalysis for recycling and upcycling plastics122Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions15Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Co-cracking of atmospheric residue and plastic waste4Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts59Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking24Catalytic Upcycling of Polyolefins316Catalyst Accessibility and Acidity in the Hydrocracking of HDPE: A Comparative Study of H-USY, H-ZSM-5, and MCM-41 Modified with Ga and Al11Unlocking the structure-activity relationship of hierarchical MFI zeolites towards the hydrocracking of HDPE14Hydrocracking of Plastic Pyrolysis Oil (PPO) Blended with Vacuum Gas Oil (VGO) over Pt–Pd Catalysts Supported on USY–ASA–Al 2 O 3 Composites9Isolating Al Surface Sites in Amorphous Silica–Alumina by Homogeneous Deposition of Al3+ on SiO2 Nanoparticles21Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Chain-length-controllable upcycling of polyolefins to sulfate detergents41Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Synergistic Catalysis for Recycling and Upcycling of Plastics35N-Containing Compound-Assisted Morphological Engineering of Anisotropic Growth of MFI Crystals5Synergistic and antagonistic effects of ZnO/Zn2+ species and Brønsted/Lewis acid sites variations on the catalytic conversion of polyethylene to aromatics7Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Synergy between acidity and Pt in Pt/HY zeolite for boosting the hydrocracking of polyethylene to C5-C7 liquid fuels0Performance comparison and sustainability assessment of mesoporous FAU zeolites for the plastic upcycling4Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins6Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Recycling of Plastic Waste: How the Conditions of Thermal Cracking and the Composition of Plastic Mixtures Affect Product Yield0Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Dissolution–recrystallization of zeolites: From chemical nature to structure reconstruction and functional engineering1Tailored Ga-modified zeolites for efficient chemical recycling of polyolefins into aromatics0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Self‐Pillared Pentasil Zeolite Microspheres as Self‐Supported Catalysts With Enhanced Molecular Diffusion for Waste Plastic Upcycling0Self‐Pillared Pentasil Zeolite Microspheres as Self‐Supported Catalysts With Enhanced Molecular Diffusion for Waste Plastic Upcycling0

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  1. Quantifying synergy for mixed end-scission and random-scission catalysts in polymer upcycling

    Reaction Chemistry & Engineering · 2023-09-26

    Ziqiu Chen, Emmanuel Ejiogu, Baron Peters

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  2. Toward Intrinsic Catalytic Rates and Selectivities of Zeolites in the Presence of Limiting Diffusion and Deactivation

    ACS Catalysis · 2023-09-26

    Cole W. Hullfish, Jun Zhi Tan, Hayat I. Adawi, Michele L. Sarazen

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  3. Solar-driven photocatalysis for recycling and upcycling plastics

    Applied Catalysis B: Environmental · 2023-09-30

    Ruochen Cao, Dequan Xiao, Meng Wang, Gao Y, Ding Ma

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  4. Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions

    Catalysis Science & Technology · 2024-01-01

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  5. Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste

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    Shaodan Xu, Junhong Tang, Li Fu

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  6. Co-cracking of atmospheric residue and plastic waste

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    Nikita S. Sergeyev, Nikita N. Sviridenko, Khoshim Kh. Urazov

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  7. Unlocking naphtha from polyolefins using Ni-based hydrocracking catalysts

    Chemical Engineering Journal · 2024-03-15

    Brandon C. Vance, Zhifei Yuliu, Sean Najmi, Esun Selvam, Jack E. Granite, Kewei Yu, Marianthi Ierapetritou, Dionisios G. Vlachos

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  8. Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels

    ACS Sustainable Chemistry & Engineering · 2024-04-03

    Xinru Zhou, Xinlei Han, Zhengyan Qu, Jiuxuan Zhang, Feng Zeng, Zhenchen Tang, Rizhi Chen

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  9. Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking

    Catalysts · 2024-07-12

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  10. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  11. Catalyst Accessibility and Acidity in the Hydrocracking of HDPE: A Comparative Study of H-USY, H-ZSM-5, and MCM-41 Modified with Ga and Al

    Molecules · 2024-09-07

    Cátia S. Costa, M. Rosário Ribeiro, João Miguel Silva

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  12. Unlocking the structure-activity relationship of hierarchical MFI zeolites towards the hydrocracking of HDPE

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  13. Hydrocracking of Plastic Pyrolysis Oil (PPO) Blended with Vacuum Gas Oil (VGO) over Pt–Pd Catalysts Supported on USY–ASA–Al 2 O 3 Composites

    Energy & Fuels · 2024-09-11

    Roberto Palos, Iratxe Crespo, David Trueba, О. В. Климов, Maxim O. Kazakov, Javier Bilbao, Alazne Gutiérrez

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  14. Isolating Al Surface Sites in Amorphous Silica–Alumina by Homogeneous Deposition of Al3+ on SiO2 Nanoparticles

    ACS Applied Nano Materials · 2024-10-31

    Ferdy J. A. G. Coumans, Brahim Mezari, Norwin Zuidema, Jason M. J. J. Heinrichs, Emiel J. M. Hensen

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  15. Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions

    Fuel · 2024-11-17

    Xinlei Han, Jiuxuan Zhang, Zhengyan Qu, Tuo Ji, Feng Zeng, Hong Li Jiang, Jun Huang, Zhenchen Tang, Weihong Xing, Rizhi Chen

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  16. Chain-length-controllable upcycling of polyolefins to sulfate detergents

    Nature Sustainability · 2024-11-18

    Nuwayo Eric Munyaneza, Ruiyang Ji, Adrian DiMarco, Joel Miscall, Lisa Stanley, Nicholas A. Rorrer, Rui Qiao, Guoliang Liu

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  17. Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters

    Polymer Degradation and Stability · 2025-01-27

    Thangaraj Baskaran, Yong-Kul Lee

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  18. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  19. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  20. Synergistic Catalysis for Recycling and Upcycling of Plastics

    ACS Catalysis · 2025-05-07

    Hongshun Ran, Xinyang Sun, Mengying Zheng, Yaxuan Jing

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  21. N-Containing Compound-Assisted Morphological Engineering of Anisotropic Growth of MFI Crystals

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  22. Synergistic and antagonistic effects of ZnO/Zn2+ species and Brønsted/Lewis acid sites variations on the catalytic conversion of polyethylene to aromatics

    Journal of Environmental Management · 2025-07-19

    Ruizhe Chen, Leilei Cheng, Wenbo Zhang, Jing Gu, Haoran Yuan, Yong Chen

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  23. Methods for Carbon Mass Closure in Polyolefin Hydrocracking

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    Anna E. Brenner, Griffin Drake, Gregg T. Beckham, Yuriy Román‐Leshkov

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  24. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

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  25. Advances of rare earth-based catalysts for recycling CO 2 and plastic waste

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  26. Synergy between acidity and Pt in Pt/HY zeolite for boosting the hydrocracking of polyethylene to C5-C7 liquid fuels

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  28. Contaminant-Tolerant Conversion of Polyethylene Waste to α-Olefins

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  29. Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control

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  30. Recycling of Plastic Waste: How the Conditions of Thermal Cracking and the Composition of Plastic Mixtures Affect Product Yield

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  31. Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels

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  32. Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene

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  33. Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations

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  34. Dissolution–recrystallization of zeolites: From chemical nature to structure reconstruction and functional engineering

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  35. Tailored Ga-modified zeolites for efficient chemical recycling of polyolefins into aromatics

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  36. Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products

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  37. Self‐Pillared Pentasil Zeolite Microspheres as Self‐Supported Catalysts With Enhanced Molecular Diffusion for Waste Plastic Upcycling

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