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RESEARCH PAPER · Applied Catalysis B: Environmental · 2022

Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalysts

Masazumi Tamura, Shuhei Miyaoka, Yosuke Nakaji, Mifumi Tanji, Shogo Kumagai, Yoshinao Nakagawa, Toshiaki Yoshioka, Keiichi Tomishige

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Structure-activity relationship in hydrogenolysis of polyolefins over Ru/support catalystsOriginalHydrogenolysis of N-Eicosane Over Ru-Based Catalysts in a Continuous Flow Reactor13Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Plastic Waste Upcycling: A Sustainable Solution for Waste Management, Product Development, and Circular Economy117Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Synthesis and advantages of spinel-type composites37Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways31Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment86Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment29Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals61Artificial photosynthesis bringing new vigor into plastic wastes63Recent Advances in Catalytic Chemical Recycling of Polyolefins104Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Investigating the influence of Ru structures and supports on hydrogenolysis of polyethylene plastic waste41Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Chemical enrichment of conjugated linoleic acid in cottonseed oil using ruthenium nanoparticle immobilized on chemically modified multiwalled carbon nanotube as heterogeneous nanocatalyst2Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Thermodynamic and Kinetic Insights into Hydrogen Adsorption and Dissociation on the Ru (0001) Surface under STM and Catalytic Conditions11Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Enhanced ruthenium selectivity for the conversion of FAMEs to diesel-range alkanes by surface decoration of FeOx species23Direct amination of poly( p -phenylene oxide) to substituted anilines over bimetallic Pd–Ru catalysts13Heterogeneous oxidative upcycling of polystyrene plastics to benzoic acid under air conditions15Novel ordered β-ketoimine-palladium( ii ) multilayers supported on a silicon wafer fabricated using layer-by-layer self-assembly for catalyzing Suzuki cross-coupling reactions1Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Sustainable high-density polyethylene via chemical recycling: From modification to polymerization methods45Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Catalytic aquathermolysis of contaminated polyolefin plastic waste over an in situ iron hydroxide/oxide nanocatalyst derived from an oil-soluble iron precursor16Complete hydrogenolysis of mixed plastic wastes101Catalytic Deconstruction of Ethylene Vinyl Acetate Copolymer and Polyethylene Mixtures via Hydroconversion: Challenges and Solutions8Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts35Low‐Temperature Hydrogenation of Carboxylic Acids to Alcohols over Heterogeneous FeOx‐Modified Ru Catalyst4Synthesis of biosurfactants from polyethylene waste via an integrated chemical and biological process3Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation15Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation8Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Catalytic recycling of plastics into value-added products28Effect of CeO2 morphology and Ru impregnation method on CH4 selectivity reduction in polyethylene waste conversion to liquid fuels and lubricants15Transformation of Polyolefinic Plastics to Chemicals by Catalytic Decomposition0Efficient polycarbonate plastic upcycling into jet fuel cycloalkanes over a bifunctional MoCo/NiC hetero-catalyst12Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Efficient Hydrogenolysis of Consumer-Grade High-Density Polyethylene Wastes over MgAl-Layered Double Oxide-Supported Ru Catalysts11Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Reaction engineering of the hydrogenolysis of liquid n-Alkanes: Comparison of flow and batch reaction systems2Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes12Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Computational insights into hydrogen interaction with the Ru (1011) and Ru (1010) surfaces: implications for alkane and polyolefin hydrogenolysis1Effective production of liquid/wax fuels from polyethylene plastics using Ru/Al 2 O 3 catalysts10Highly energy-efficient hydrogenolysis of high-density polyethylene via hydrogen nonthermal plasma reaction engineering4Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Surface-confined growth of Ru amorphous sub-nanoclusters on reductive Mn 3 O 4 : a strongly coupled interface engineering for efficient neutral hydrogen production62Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis2Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis27Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Efficient Degradation and Optimization of Waste Polyisocyanurate by La-Ni Perovskite Catalysts0Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Upcycling polyolefins to methane-free liquid fuel by a Ru1-ZrO2 catalyst47Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Ru-Catalyzed Polyethylene Hydrogenolysis under Quasi-Supercritical Conditions25Synergistic Catalysis for Recycling and Upcycling of Plastics35Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Hydrocracking of Polypropylene to Light Alkanes over HMFI Zeolite Catalysts under H 27In-line NMR guided orthogonal transformation of real-life plastics63Plastic-waste hydrogenolysis over two-dimensional MXene-supported ruthenium catalysts with tunable interlayer spacing3Methods for Carbon Mass Closure in Polyolefin Hydrocracking6Poisoning effects of impurities on hydrogenolysis of polyethylenes over supported Ru catalysts3Tuning Catalytic Reactivity via Wetting Control through Oxygen Vacancies: Ru Clusters on Anatase TiO2 and CeO2 Supports22Unraveling support effects in Ru-based catalysts for efficient conversion of marine biomass to sugar alcohols1Acidic Site-Controlled ZSM-5 Catalysts for Fast Molten-Phase Pyrolysis of Plastic Waste with Tunable Product Distribution4Chemical recycling of polyethylenes with low gas products by catalytic hydrogenolysis with heterogeneous CeO2-supported Cu-doped Ru catalyst5Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Advances of rare earth-based catalysts for recycling CO 2 and plastic waste17Selective Hydrocracking of Polyethylene to Gasoline Over Bi‐Functional Ir/HBEA Catalysts Under Mild Condition2Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Research progress in metal-zeolite bifunctional systems for upcycling of waste polyolefins3Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking11Carbon–carbon bond cleavage for lignin and plastics deconstruction0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Electronegativity-driven d-band center shifts in Ru–Ni alloys for low methane hydrogenolysis of polyolefin plastics2Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Enhancing selectivity and yield in polyethylene hydrogenolysis using goal-aware Bayesian algorithm execution0Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Selective Conversion of Polyolefin Waste to Branched Alkanes via Methane‐Free Tandem Hydrocracking–Isomerization2Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3One-pot co-upcycling of mixed polyolefin waste6Tailoring the polyolefin hydrogenolysis performance of Ru/TiO2 through TiO2 support facet engineering1Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts6Techno-economic analysis and life cycle assessment for the catalytic hydrogenolysis and hydrocracking of polyethylene6Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Depolymerization of Nylon-6 over a Supported Ruthenium Catalyst to ε-Caprolactam1Upcycling plastic waste into drop-in fuels using tandem decalin dehydrogenation and hydrocracking: Economic and environmental impact assessments7Confined Ruthenium Nanoclusters in Montmorillonite for Ethylene Hydroformylation to 3-Pentanone0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Co 1 /Ru Single‐Atom Alloy Catalyst for Sustainable Polypropylene Hydrogenolysis to Long‐Chain Liquid Products1A Mesopore-Confined and Graphene Oxide-Localized Ruthenium Catalyst Increases Rates of Mid-Chain Polyolefin Hydrogenolysis0Unlocking cost and carbon parity with polyethylene recycling0Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Reductive catalytic upcycling of polyethylene using 2-propanol as transfer hydrogen-donor source1Implementable and Sustainable Upcycling of Medical Plastic Waste to Liquid Highly Branched Alkanes via Tandem Catalytic Cracking-Hydrogenation Strategy0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Volcano Trend between the Size of Ru Nanocatalysts and Hydrogenation Activity for Levulinic Acid0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Internal transport modulates catalytic hydrogenolysis of polyolefins0Highly active and selective heterogeneous Ru/La2O3-CeO2 catalyst for hydrogenolysis of LDPE to valuable chemicals0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  2. Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

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  4. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

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  5. Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production

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  7. Identifying selective catalysts in polypropylene hydrogenolysis by decoupling scission pathways

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  9. Ruthenium/TiO2‐Catalyzed Hydrogenolysis of Polyethylene Terephthalate: Reaction Pathways Dominated by Coordination Environment

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  10. Waste PVC upcycling: Transferring unmanageable Cl species into value-added Cl-containing chemicals

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  15. Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity

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  16. Upcycling of polyethylenes by catalysis

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  17. SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

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  18. Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins

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  34. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

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  35. Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

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  37. Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect

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  39. Complete hydrogenolysis of mixed plastic wastes

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  41. Chemical Upcycling of Polyolefin Plastics Using Structurally Well-defined Catalysts

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  42. Low‐Temperature Hydrogenation of Carboxylic Acids to Alcohols over Heterogeneous FeOx‐Modified Ru Catalyst

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  43. Synthesis of biosurfactants from polyethylene waste via an integrated chemical and biological process

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  44. Polyethylene hydrogenolysis over bimetallic catalyst with suppression of methane formation

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  45. Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design

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  46. Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics

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  47. Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation

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  48. Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review

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  49. Catalytic Upcycling of Polyolefins

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    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  50. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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