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RESEARCH PAPER · Applied Catalysis B: Environmental · 2022

Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethylene

Doyoung Kim, Zachary R. Hinton, Peng Bai, LaShanda T. J. Korley, Thomas H. III Epps, Raúl F. Lobo

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Metathesis, molecular redistribution of alkanes, and the chemical upgrading of low-density polyethyleneOriginalCatalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Recent Advances in Catalytic Chemical Recycling of Polyolefins104Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Processing Plastic Wastes into Value-Added Carbon Adsorbents by Sulfur-Based Solvothermal Synthesis14Bulk depolymerization of poly(methyl methacrylate) via chain-end initiation for catalyst-free reversion to monomer142Mechanistic study of heterogeneous propene metathesis on WOx/SiO2 catalysts13Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Bulk Depolymerization of Methacrylate Polymers via Pendent Group Activation93Deconstruction of Polymers through Olefin Metathesis101Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Catalytic Upcycling of Polyolefins316Polyolefin waste to light olefins with ethylene and base-metal heterogeneous catalysts151Close-loop chemical recycling unlocked via waste polyolefins-ethylene co-metathesis2One-pot catalytic conversion of polyethylene wastes to gasoline through a dual-catalyst system41Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies6Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Effects of Pretreatment Conditions and Branched Alkanes on Mo/MCM-41 Catalysts in Tandem Alkane Cross-metathesis for Non-hydrogen Polyolefin Recycling3Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Optimization of low-temperature catalytic cracking of polyolefin waste in open-batch reactors using zeolite beta with controlled intrinsic properties20Upcycling of Waste Plastics into Value-Added Chemicals6Bulk Depolymerization of Polystyrene with Comonomer Radical Triggers19Synergistic Catalysis for Recycling and Upcycling of Plastics35The role of H2 donation in heterogeneous Mo-based olefin metathesis site creation0Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Carbon–carbon bond cleavage for lignin and plastics deconstruction0InCuZn alloy layer guiding oriented Zn 2+ deposition for highly stable and dendrite-free zinc anodes0Interfacial electronic coupling engineering in Pt/WO x –Al 2 O 3 for hydrogen-free polyolefin upcycling0Heterogeneous olefin metathesis promotion using molecular hydrogen0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3High-performance ethylene/2-butene cross-metathesis catalysis over tungsten species in or close to zeolite Y for propylene production: The multifunctional roles of zeolite0Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Catalytic solvothermal upcycling of mixed polyolefin waste into gasoline-range liquid fuels: Solvent-assisted selectivity and coke kinetics over zeolite-based catalysts0Selective upcycling of virgin and post-consumer polypropylene waste into aromatic-rich oil via solvothermal liquefaction in tetralin0Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air0Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air0Enhancing light olefin production by pre-cracking and acidity tuning over hierarchical La/ZSM-5@ASA composites0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0Bioproduction of α,ω-oxyfunctionalised alkanes0

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  1. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

    Catalysis Science & Technology · 2022-12-14

    Junde Wei, Jieyi Liu, Weihao Zeng, Zichen Dong, Jingkuo Song, Sibao Liu, Guozhu Liu

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  2. Recent Advances in Catalytic Chemical Recycling of Polyolefins

    ChemCatChem · 2023-03-29

    Kirill Faust, Peter Denifl, Marko Hapke

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  3. Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures

    Applied Catalysis B: Environmental · 2023-07-06

    Julia N. Hancock, Julie E. Rorrer

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  4. Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity

    JACS Au · 2023-07-14

    Brandon C. Vance, Sean Najmi, Pavel A. Kots, Cong Wang, Sungho Jeon, Eric A. Stach, Dmitri N. Zakharov, Nebojša Marinković, Steven N. Ehrlich, Lu Ma, Dionisios G. Vlachos

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  5. Processing Plastic Wastes into Value-Added Carbon Adsorbents by Sulfur-Based Solvothermal Synthesis

    ACS Sustainable Chemistry & Engineering · 2023-07-18

    Jiahua Zhao, Shu Yuan, Qiang Niu, Pengfei Zhang

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  6. Bulk depolymerization of poly(methyl methacrylate) via chain-end initiation for catalyst-free reversion to monomer

    Chem · 2023-08-07

    James B. Young, Rhys W. Hughes, Ariana M. Tamura, Laura S. Bailey, Kevin A. Stewart, Brent S. Sumerlin

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  7. Mechanistic study of heterogeneous propene metathesis on WOx/SiO2 catalysts

    Journal of Catalysis · 2023-09-09

    Anne V. Le, Biplab Rajbanshi, Raúl F. Lobo, Peng Bai

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  8. Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis

    Langmuir · 2024-02-15

    Huidong Lv, Fei Huang, Fan Zhang

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  9. Bulk Depolymerization of Methacrylate Polymers via Pendent Group Activation

    Journal of the American Chemical Society · 2024-02-21

    Rhys W. Hughes, Megan E. Lott, Isabella S. Zastrow, James B. Young, Tanmoy Maity, Brent S. Sumerlin

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  10. Deconstruction of Polymers through Olefin Metathesis

    Chemical Reviews · 2024-05-24

    Devavrat Sathe, Seiyoung Yoon, Zeyu Wang, Hanlin Chen, Junpeng Wang

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  11. Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design

    Cell Reports Physical Science · 2024-07-01

    Haokun Wang, Shik Chi Edman Tsang

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  12. Catalytic Upcycling of Polyolefins

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    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  13. Polyolefin waste to light olefins with ethylene and base-metal heterogeneous catalysts

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    Richard J. Conk, Jules F. Stahler, Jake X. Shi, Ji Yang, Natalie G. Lefton, John N. Brunn, Alexis T. Bell, John F. Hartwig

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  14. Close-loop chemical recycling unlocked via waste polyolefins-ethylene co-metathesis

    Chem Catalysis · 2024-11-01

    Pavel A. Kots

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  15. One-pot catalytic conversion of polyethylene wastes to gasoline through a dual-catalyst system

    Chem · 2024-11-06

    Wanying Han, Longfei Lin, Ziyu Cen, Yubin Ke, Qian Xu, Junfa Zhu, Xuelei Mei, Zhanghui Xia, Xinrui Zheng, Yaqin Wang, Yani Liu, Mingyuan He, Haihong Wu, Buxing Han

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  16. Kinetic Models for Polymer Upcycling by Tag-and-Cut Strategies

    Industrial & Engineering Chemistry Research · 2024-12-06

    Emmanuel Ejiogu, Baron Peters

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  17. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

    Chemical Communications · 2024-12-18

    Haokun Wang, Sijie Huang, Shik Chi Edman Tsang

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  18. Effects of Pretreatment Conditions and Branched Alkanes on Mo/MCM-41 Catalysts in Tandem Alkane Cross-metathesis for Non-hydrogen Polyolefin Recycling

    Korean Journal of Chemical Engineering · 2025-02-07

    Seung Ha Ryu, Hankyeul Kang, Jong Hun Kang

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  19. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie International Edition · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  20. Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis

    Angewandte Chemie · 2025-03-13

    Wei Zhang, Sung Min Kim, Michele L. Sarazen, Mingyuan He, Jingguang G. Chen, Johannes A. Lercher

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  21. The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction

    Journal of Catalysis · 2025-03-21

    Selena Moore, Andrew Tran, Andreas Palmateer, Jose Naranjo Mendez, Dimitri Gatzios, Peter A. Eschbach, Joel Miscall, Lucas D. Ellis

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  22. Optimization of low-temperature catalytic cracking of polyolefin waste in open-batch reactors using zeolite beta with controlled intrinsic properties

    Communications Engineering · 2025-03-24

    Hankyeul Kang, Junghwa Yoon, Dongwoo Jun, Ki Hyuk Kang, Insoo Ro, Soo-Hwa Jeong, Jong Hun Kang

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  23. Upcycling of Waste Plastics into Value-Added Chemicals

    Science for energy and environment. · 2025-03-26

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  24. Bulk Depolymerization of Polystyrene with Comonomer Radical Triggers

    ACS Macro Letters · 2025-04-23

    James B. Young, Jared I. Bowman, Megan E. Lott, Lily Diodati, Kaden C. Stevens, Rhys W. Hughes, Lauren E. Mann, Alex H. Balzer, LaShanda T. J. Korley, Brent S. Sumerlin

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  25. Synergistic Catalysis for Recycling and Upcycling of Plastics

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  26. The role of H2 donation in heterogeneous Mo-based olefin metathesis site creation

    Cell Reports Physical Science · 2025-07-01

    Dimitri Gatzios, Stephen Stockton, Avery F. Hill, Hannah Frankovic, M. M. Montemore, Lucas D. Ellis

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  27. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

    Korean Journal of Chemical Engineering · 2025-10-20

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  28. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

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    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  29. A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis

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    Chuanya Li, Qianfeng Zhou, Changhu Leng, Yongchao Wang, Chenyang Ma, Junlei Zhang, Zhijun Li

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  30. Carbon–carbon bond cleavage for lignin and plastics deconstruction

    Chemical Society Reviews · 2026-01-01

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  31. InCuZn alloy layer guiding oriented Zn 2+ deposition for highly stable and dendrite-free zinc anodes

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  32. Interfacial electronic coupling engineering in Pt/WO x –Al 2 O 3 for hydrogen-free polyolefin upcycling

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  33. Heterogeneous olefin metathesis promotion using molecular hydrogen

    Chem Catalysis · 2026-02-01

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  34. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

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  35. High-performance ethylene/2-butene cross-metathesis catalysis over tungsten species in or close to zeolite Y for propylene production: The multifunctional roles of zeolite

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  36. Impact of Small-Alkane Solvents on Polyolefin Hydrogenolysis over a Ruthenium Catalyst

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  37. Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications

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  38. Catalytic solvothermal upcycling of mixed polyolefin waste into gasoline-range liquid fuels: Solvent-assisted selectivity and coke kinetics over zeolite-based catalysts

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  39. Selective upcycling of virgin and post-consumer polypropylene waste into aromatic-rich oil via solvothermal liquefaction in tetralin

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  40. Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air

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  41. Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air

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  42. Enhancing light olefin production by pre-cracking and acidity tuning over hierarchical La/ZSM-5@ASA composites

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  43. Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock

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  44. Bioproduction of α,ω-oxyfunctionalised alkanes

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