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RESEARCH PAPER · Macromolecules · 2022

Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of Polyolefins

Ryan A. Hackler, Jessica V. Lamb, Ian L. Peczak, Robert M. Kennedy, Uddhav Kanbur, Anne M. LaPointe, Kenneth Reinhard Poeppelmeier, Aaron David Sadow, Massimiliano Delferro

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Effect of Macro- and Microstructures on Catalytic Hydrogenolysis of PolyolefinsOriginalDual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Microwave‐Assisted Synthesis of SrTiO3 Nanocuboids without TiCl46Design of Microstructure-Engineered Polymers for Energy and Environmental Conservation20Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR25A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina23Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts23A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8Precise activation of C–C bonds for recycling and upcycling of plastics81Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey4Characterization of polymer properties and identification of additives in commercially available research plastics112Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Sustainable Petrochemical Alternatives From Plastic Upcycling5Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure40Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex12Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex3Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO230Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review27Observing the Surface Termination of LaScO 3 Perovskite Using Solid-State Nuclear Magnetic Resonance6Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12A Mini-review on Development for the Direct Catalytic Hydroconversion of Polypropylene to Liquid and Gaseous Hydrocarbons for Fuels and Chemicals1Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Catalytic Strategies for the Production of Alkane‐Based Lubricant Base Oils from Biomass and Plastic Wastes11Synergistic Catalysis for Recycling and Upcycling of Plastics35High-Temperature Size Exclusion Chromatography for Advanced Recycling: Systematic Errors in Analysis of Polyethylene─Alkane Mixtures0Tuning Catalytic Reactivity via Wetting Control through Oxygen Vacancies: Ru Clusters on Anatase TiO2 and CeO2 Supports22Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering2Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Recent advances in catalytic hydrogenolysis of polycarbonate, polyurethane and polyurea0Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3One-pot co-upcycling of mixed polyolefin waste6Polymer Deconstruction and Redesign Strategies for Plastics Recycling0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Internal transport modulates catalytic hydrogenolysis of polyolefins0Molecular Insights into Competitive Adsorption in the Deconstruction of Mixed Polyolefin Waste0

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  1. Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

    Applied Catalysis B: Environmental · 2022-08-17

    Linxiao Chen, J. Moreira, Laura C. Meyer, Oliver Y. Gutiérrez, János Szanyi

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  2. Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste

    Journal of Materials Chemistry A · 2022-12-12

    Katherine E. McCullough, Ian L. Peczak, Robert M. Kennedy, Yiyu Wang, James Lin, Xun Wei Wu, Alexander L. Paterson, Frédéric A. Perras, Jacklyn N. Hall, Arthur Jeremy Kropf, Ryan A. Hackler, Young-Ho Shin, Jens Niklas, Oleg G. Poluektov, Jianguo Wen, Wenyu Huang, Aaron David Sadow, Kenneth Reinhard Poeppelmeier, Massimiliano Delferro, Magali S. Ferrandon

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  3. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

    Catalysis Science & Technology · 2022-12-14

    Junde Wei, Jieyi Liu, Weihao Zeng, Zichen Dong, Jingkuo Song, Sibao Liu, Guozhu Liu

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  4. Microwave‐Assisted Synthesis of SrTiO3 Nanocuboids without TiCl4

    Small Science · 2023-04-06

    Ian L. Peczak, Robert M. Kennedy, Aili M. Simpson, Massimiliano Delferro, Kenneth Reinhard Poeppelmeier

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  5. Design of Microstructure-Engineered Polymers for Energy and Environmental Conservation

    JACS Au · 2023-04-27

    Yazhen Xue, Mengxue Cao, Charles Chen, Mingjiang Zhong

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  6. Mechanistic Insights into Processive Polyethylene Hydrogenolysis throughIn SituNMR

    Macromolecules · 2023-05-30

    Yunpu Zhao, Max Meirow, Akalanka Tennakoon, Xun Wei Wu, Alexander L. Paterson, Long Hao Qi, Anne M. LaPointe, Jessica V. Lamb, Takeshi Kobayashi, Massimiliano Delferro, Aaron David Sadow, Wenyu Huang, Erik Luijten, Frédéric A. Perras

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  7. A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins

    Science Advances · 2023-06-21

    Zetian Qiu, Siyu Lin, Zhuo Chen, Anqi Chen, Yitian Zhou, Xudong Cao, Yu Wang, Bo‐Lin Lin

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  8. Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures

    Applied Catalysis B: Environmental · 2023-07-06

    Julia N. Hancock, Julie E. Rorrer

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  9. Polypropylene Degradation Catalyzed by Tantalum Hydrides Supported on Sulfated Alumina

    ACS Catalysis · 2023-08-01

    Jiaxin Gao, Lingchao Zhu, Matthew P. Conley

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  10. Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials

    Matter · 2023-08-08

    Ian L. Peczak, Robert M. Kennedy, Ryan A. Hackler, Byeongdu Lee, Max Meirow, Erik Luijten, Kenneth Reinhard Poeppelmeier, Massimiliano Delferro

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  11. Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures

    ACS Sustainable Chemistry & Engineering · 2023-08-17

    Makenna L. Pennel, Anjani K. Maurya, Amani M. Ebrahim, Christopher J. Tassone, Matteo Cargnello

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  12. Enhanced production and control of liquid alkanes in the hydrogenolysis of polypropylene over shaped Ru/CeO2 catalysts

    Applied Catalysis A General · 2023-09-01

    Ajay Tomer, Mazharul M. Islam, Mounib Bahri, Donald R. Inns, Troy D. Manning, John B. Claridge, Nigel D. Browning, C. Richard A. Catlow, Alberto Roldán, Alexandros P. Katsoulidis, Matthew J. Rosseinsky

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  13. A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene

    Journal of the American Chemical Society · 2023-11-03

    Kavyasripriya K. Samudrala, Matthew P. Conley

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  14. Precise activation of C–C bonds for recycling and upcycling of plastics

    Chemical Science · 2023-12-07

    Hongshun Ran, Shuo Zhang, Wenyi Ni, Yaxuan Jing

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  15. Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey

    CHIMIA International Journal for Chemistry · 2023-12-20

    Christopher Hunston, Wei‐Tse Lee, Antoine P. van Muyden, Félix D. Bobbink

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  16. Characterization of polymer properties and identification of additives in commercially available research plastics

    Green Chemistry · 2024-01-01

    Amy A. Cuthbertson, Clarissa L. Lincoln, Joel Miscall, Lisa M. Stanley, Anjani K. Maurya, Arun S. Asundi, Christopher J. Tassone, Nicholas A. Rorrer, Gregg T. Beckham

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  17. Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production

    Chemical Communications · 2024-01-01

    Arjun K. Manal, Atal Shivhare, Sharad V. Lande, Rajendra Srivastava

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  18. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

    Energy & Fuels · 2024-01-22

    Abdulrahman Musa, E. A. Jaseer, Samir Barman, Néstor Garcı́a

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  19. Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation

    ACS Catalysis · 2024-01-24

    Yi‐Yu Wang, Akalanka Tennakoon, Xun Wei Wu, Chinmay Sahasrabudhe, Long Hao Qi, Baron Peters, Aaron David Sadow, Wenyu Huang

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  20. Sustainable Petrochemical Alternatives From Plastic Upcycling

    Unknown journal · 2024-01-26

    Ryan A. Hackler, Robert M. Kennedy

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  21. Catalytic conversion of mixed polyolefins under mild atmospheric pressure

    The Innovation · 2024-02-03

    Binzhi Zhao, Hui Tan, Jie Yang, Xiaohui Zhang, Zidi Yu, Han‐Li Sun, Jialiang Wei, Xinyi Zhao, Yufeng Zhang, Lili Chen, Dali Yang, Jin Deng, Yao Fu, Zheng Huang, Ning Jiao

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  22. Size and Structure Effects of Carbon-Supported Ruthenium Nanoparticles on Waste Polypropylene Hydrogenolysis Activity, Selectivity, and Product Microstructure

    ACS Catalysis · 2024-02-15

    Jessie A. Sun, Pavel A. Kots, Zachary R. Hinton, Nebojša Marinković, Lu Ma, Steven N. Ehrlich, Weiqing Zheng, Thomas H. III Epps, LaShanda T. J. Korley, Dionisios G. Vlachos

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  23. Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex

    Angewandte Chemie International Edition · 2024-02-19

    Andrey V. Pichugov, Léon Escomel, Sébastien Lassalle, Julien Petit, Ribal Jabbour, David Gajan, Laurent Veyre, Emiliano Fonda, Anne S. J. Lesage, Chloé Thieuleux, Clément Camp

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  24. Highly Selective and Efficient Perdeuteration of n‐Pentane via H/D Exchange Catalyzed by a Silica‐Supported Hafnium‐Iridium Bimetallic Complex

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  25. Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity

    ACS Applied Materials & Interfaces · 2024-02-23

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  26. Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components

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  27. Polystyrene Hydrogenolysis to High-Quality Lubricants Using Ni/SiO2

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  28. Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity

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  29. Catalytic Approaches to Tackle Mixed Plastic Waste Challenges: A Review

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  30. Observing the Surface Termination of LaScO 3 Perovskite Using Solid-State Nuclear Magnetic Resonance

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  31. Catalytic Upcycling of Polyolefins

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    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  32. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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  33. A Mini-review on Development for the Direct Catalytic Hydroconversion of Polypropylene to Liquid and Gaseous Hydrocarbons for Fuels and Chemicals

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  34. Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management

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  35. Catalytic Strategies for the Production of Alkane‐Based Lubricant Base Oils from Biomass and Plastic Wastes

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  36. Synergistic Catalysis for Recycling and Upcycling of Plastics

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  37. High-Temperature Size Exclusion Chromatography for Advanced Recycling: Systematic Errors in Analysis of Polyethylene─Alkane Mixtures

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  38. Tuning Catalytic Reactivity via Wetting Control through Oxygen Vacancies: Ru Clusters on Anatase TiO2 and CeO2 Supports

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  39. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

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  40. Molar-Mass-Dependent Partitioning of Polyethylene in Nanopores of Model Catalyst Supports from Small-Angle Neutron Scattering

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  41. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

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  42. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

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  43. Recent advances in catalytic hydrogenolysis of polycarbonate, polyurethane and polyurea

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  44. Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production

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  45. One-pot co-upcycling of mixed polyolefin waste

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  47. Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking

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  48. Internal transport modulates catalytic hydrogenolysis of polyolefins

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  49. Molecular Insights into Competitive Adsorption in the Deconstruction of Mixed Polyolefin Waste

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