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RESEARCH PAPER · Environmental Pollution · 2022

Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalyst

Zhigang Zhao, Zheng Li, Xiangkun Zhang, Tan Li, Yuqing Li, Xingkun Chen, Kaige Wang

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Catalytic hydrogenolysis of plastic to liquid hydrocarbons over a nickel-based catalystOriginalCatalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Recent Advances in Catalytic Chemical Recycling of Polyolefins104Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste47A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity61Upcycling of polyethylenes by catalysis0Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling45Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins62Development of reusable Ni/γ-Al2O3 catalyst for catalytic hydrolysis of waste PET bottles into terephthalic acid20Clarifying European terminology in plastics recycling58Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components18Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6Synthesis of sustainable aviation biofuels via catalytic hydropyrolysis of lignin38Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Catalytic Upcycling of Polyolefins316The role of size and structure of catalytic active sites in polyolefin hydrogenolysis12Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts16Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Synthesis of aviation biofuel precursors from biomass-derived ketones: Substrate adsorption configuration-catalytic activity7Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes12Hydrogenolysis and hydrocracking of biomass and plastic wastes to produce high-value products1Optimization of nickel-based catalysts for hydrogenolysis of light paraffins using machine learning5Recent developments in recycling of post-consumer polyethylene waste33Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Techno-economic and life cycle analyses of the synthesis of a platinum–strontium titanate catalyst15Upgrading of waste polyolefins with non-noble metal catalysts21Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Recovery of chemicals and energy through thermo-chemical processing of plastic waste33Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation5Plastic pollutants: From wastes to fuels and high-value chemicals8Recent Advances in the Thermo-Catalytic Upcycling of Polyethylene Waste13Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Zinc oxide-mediated C H activation of polypropylene waste for thermochemical valorization1Stable single-site organonickel catalyst preferentially hydrogenolyses branched polyolefin C–C bonds12Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching3Recent Progress in Sustainable Recycling of Waste Acrylonitrile–Butadiene–Styrene (ABS) Plastics16Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene3Polyethylene hydrogenolysis to liquid products over bimetallic catalysts with favorable environmental footprint and economics17Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Data-Driven Discovery of Bimetallic Nanoparticles Catalysts for the Hydrogenolysis of Polyethylene3Mechanistic insights into plastic degradation via catalytic bond breaking: a comprehensive review1Microplastic Pollution in the Environment: A Chemical Engineering Perspective on Sources, Fate, and Mitigation Strategies22Catalytic valorization of polyolefins: from catalysts and processes to reactors0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Advancing Waste Plastic Valorization: Catalytic Production of Aviation Fuel over Zeolite and Ru/CNT-Based Catalysts4Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Application of waste polypropylene pyrolytic oil in CI engines: Performance and emission assessment0NiW alloy catalyst for methane suppression in polyethylene hydrogenolysis to enhance liquid hydrocarbon yields1Single-Atom Nickel Dispersed on Mo 2 TiC 2 T x MXene for Upcycling of Polyolefins via Catalytic Hydropyrolysis for Fuels and Lubricants0Sustainable Aviation Fuel (SAF): A Mini-Review of Advances in Catalytic Pathways Using Lipid-Based Feedstocks and Plastic Waste3Enhanced Production of High-Value BTEX Aromatic Hydrocarbons from the Pyrolysis/Nonthermal Plasma/Catalysis of Waste Plastics0Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Controlling Polyolefin Hydrogenolysis Selectivity by Engineering Single-Site Nickel(II) Hydride Active Catalytic Species0A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Selective hydrogenolysis of waste polyolefins to aviation fuel over a Co‑modified Ni/SiO2 catalyst1Catalytic Hydrogenolysis of Polyethylene-Based Plastics into Fuels Using Ruthenium Catalysts Supported on Micro/Mesoporous Carbons0Thermochemical conversion of metallized plastic packaging waste: Aluminum in waste enhances polymer pre-cracking and steam-cracker precursor formation over zeolite catalysts1In-situ hydrogen generation via water-gas shift reaction over Ni-Fe3O4/USY: A sustainable pathway for efficient polypropylene hydrogenolysis0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Role of molybdenum promotion in Ni/SiO2 catalysts for Polyolefins Hydrogenolysis0

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  1. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

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  2. Recent Advances in Catalytic Chemical Recycling of Polyolefins

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  3. Investigating the impact of TiO2 crystalline phases on catalytic properties of Ru/TiO2 for hydrogenolysis of polyethylene plastic waste

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  4. A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins

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  5. Structure–Property Relationships for Nickel Aluminate Catalysts in Polyethylene Hydrogenolysis with Low Methane Selectivity

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  6. Upcycling of polyethylenes by catalysis

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  7. Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling

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  8. Two Mesoporous Domains Are Better Than One for Catalytic Deconstruction of Polyolefins

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  9. Development of reusable Ni/γ-Al2O3 catalyst for catalytic hydrolysis of waste PET bottles into terephthalic acid

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  10. Clarifying European terminology in plastics recycling

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  11. Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity

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  12. Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis

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  13. Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions

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  14. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

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  15. Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation

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  16. Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts

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  17. Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis

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  18. Catalytic hydrogenolysis of polypropylene and polyethylene mixtures: Effect of temperature on liquid alkane components

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  19. Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts

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  20. Synthesis of sustainable aviation biofuels via catalytic hydropyrolysis of lignin

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  21. Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity

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  22. Catalytic Upcycling of Polyolefins

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  23. The role of size and structure of catalytic active sites in polyolefin hydrogenolysis

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  24. Hydrogenolysis of Polyethylene by Metal–Organic Framework Confined Single-Site Ruthenium Catalysts

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  25. Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions

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  26. Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions

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  27. Synthesis of aviation biofuel precursors from biomass-derived ketones: Substrate adsorption configuration-catalytic activity

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  28. Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins

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  29. Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling

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  30. Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts

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  31. Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques

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  32. Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes

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  33. Hydrogenolysis and hydrocracking of biomass and plastic wastes to produce high-value products

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  35. Recent developments in recycling of post-consumer polyethylene waste

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  36. Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels

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  37. Techno-economic and life cycle analyses of the synthesis of a platinum–strontium titanate catalyst

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  38. Upgrading of waste polyolefins with non-noble metal catalysts

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  39. Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts

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  41. Investigation on polyethylene hydrogenolysis over a nickel catalyst via ReaxFF molecular dynamic simulation

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  45. Zinc oxide-mediated C H activation of polypropylene waste for thermochemical valorization

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  47. Polymer Upcycling by Catalytic Hydrogenolysis: The Role of Polyolefin Short-Chain Branching

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  48. Recent Progress in Sustainable Recycling of Waste Acrylonitrile–Butadiene–Styrene (ABS) Plastics

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  49. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

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  50. Synergy Effects in a Bimetallic Ru ─ Pt Alloy Catalyst for Low‐H 2 ‐Pressure Hydrogenolysis of Low‐Density Polyethylene

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