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RESEARCH PAPER · Nature Communications · 2022

Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalysts

Wei‐Tse Lee, Antoine P. van Muyden, Félix D. Bobbink, Mounir Mensi, Jed R. Carullo, Paul J. Dyson

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Mechanistic classification and benchmarking of polyolefin depolymerization over silica-alumina-based catalystsOriginalDual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst54Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94Evolution of light olefins during the pyrolysis of polyethylene in a two-stage process49Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production90Transport limitations in polyolefin cracking at the single catalyst particle level66Boosting Polyethylene Hydrogenolysis Performance of Ru‐CeO2 Catalysts by Finely Regulating the Ru Sizes66Liquid fuel production from catalytic pyrolysis of municipal plastic waste using synthesized Zeolite from Kaolin0A reusable, impurity-tolerant and noble metal–free catalyst for hydrocracking of waste polyolefins113Conversion of polyethylene waste to short chain hydrocarbons under mild temperature and hydrogen pressure with metal-free and metal-loaded MFI zeolites69Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons171Green/sustainable strategy for the enhanced thermal destruction of abandoned, lost, discarded fishing gears (ALDFGs)8Catalytic cracking of low-density polyethylene dissolved in various solvents: product distribution and coking behavior9Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures43Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions171Upcycling of polyethylenes by catalysis0SMSI-induced charge transfer for selective hydrogenolysis of polyolefins76Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures20Construction of Highly Active and Selective Molecular Imprinting Catalyst for Hydrogenation29Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Controlling the selectivity of the hydrogenolysis of polyamides catalysed by ceria-supported metal nanoparticles26The Other Side of Plastics: Bioplastic-Based Nanoparticles for Drug Delivery Systems in the Brain24Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products60Precise activation of C–C bonds for recycling and upcycling of plastics81Mechanistic understanding of metal–acid synergetic hydroconversion of polyethylene under mild conditions over a Ru/MOR catalyst22Bridging the Gap Between Academia and Chemical Industry through Entrepreneurship: An Account on the Case of Hydrogen-assisted Catalytic Plastic Waste Valorisation0Valorisation of Plastic Waste via Catalytic Hydrocracking: a Technological Survey4Advances in morphology-controlled alumina and its supported Pd catalysts: synthesis and applications116Computational Insights into Catalysis: Evaluating Alternative Metal Potentials in Mgcl2-Supported Ziegler-Natta Catalysts0Opportunities and challenges for plastic depolymerization by biomimetic catalysis36Synergistic catalysis for promoting selective C–C/C–O cleavage in plastic waste: structure–activity relationship and rational design of heterogeneous catalysts for liquid hydrocarbon production18Silica as support and binder in bifunctional catalysts with ultralow Pt loadings for the hydroconversion of n-alkanes3Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters21Shape Selectivity of AEL Channels for Anomalously Facilitating Biojet Fuel Production from Long-Chain n-Alkane Hydrocracking30Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions32Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Supported Platinum Nanoparticles Catalyzed Carbon–Carbon Bond Cleavage of Polyolefins: Role of the Oxide Support Acidity27Tandem catalysis enables chlorine-containing waste as chlorination reagents48Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect24Research Progress in Fuel Oil Production by Catalytic Pyrolysis Technologies of Waste Plastics29PLASTAMINATION: Outcomes on the Central Nervous System and Reproduction26Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity7Pioneering Aromatic Generation from Plastic Waste via Catalytic Thermolysis: A Minireview38Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking24Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Catalytic Upcycling of Polyolefins316Chemical recycling of polyolefin waste: from the perspective of efficient pyrolysis reactors13Pore-Structure Engineering of Hierarchical β Zeolites for the Enhanced Hydrocracking of Waste Plastics to Liquid Fuels51Selective catalytic conversion of model olefin and diolefin compounds of waste plastic pyrolysis oil: Insights for light olefin production and coke minimization25Coupling Conversion of CO2 and High‐Carbon Alkane to CO and Gasoline2Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling43Elucidating the effect of nanocube support morphology on the hydrogenolysis of polypropylene over Ni/CeO 2 catalysts7Enhancing Polypropylene/Polyethylene Blend Performance Through Compatibilization for A Sustainable Future: A Mini Review Focusing on Establishing Bio‐Derived Filler Based Hybrid Compatibilizer System31Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Microwave‐Powered Liquid Metal Degradation of Polyolefins30Bimetallic NiFe/Al 2 O 3 catalyst for efficient hydrogenolysis of polyethylene into aviation fuel range alkanes12Circular plastic economy for sustainable development: current advances and future perspectives49Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Enhancing liquified petroleum gas selectivity through hierarchical porosity in MWW-type MCM-49 zeolite for polyethylene hydrocracking0Harnessing synthetic biology to empower a circular plastics economy1Hydrocracking of polyolefins over ceria-promoted Ni/BEA catalysts23Selective hydrocracking of polyolefin waste into branched liquid fuels over a non-noble metal bifunctional Ni–W/ZrO 2 catalyst4Synergistic effect of acidic sites and mesoporous confinement in Ce-doped Ru/SBA-15 catalysts for efficient hydrogenolysis of low-density polyethylene to liquid fuels7Upgrading of waste polyolefins with non-noble metal catalysts21Solvent-free upcycling of agricultural plastic waste using in situ self-assembly metal nanoparticles co-doped microporous carbocatalyst for advanced transportation fuels12Hydrocracking of polyethylene to high quality liquid fuels over bimetallic catalyst PdAg/HZSM-58Recent advancements in upcycling of polyolefins by hydrocracking: Effect of various heterogeneous catalysts and reaction parameters8Selective production of cycloalkanes through the catalytic hydrodeoxygenation of lignin with CoNi2@BTC catalysts without external hydrogen20Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis2Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Hydrocracking of Polyethylene to Gasoline-Range Hydrocarbons over a Ruthenium-Zeolite Bifunctional Catalyst System with Optimal Synergy of Metal and Acid Sites9Polyolefin Recycling with Binary Cobalt–Nickel Nanosheets6Advances in catalytic transformations of waste plastic resources with zeolites0Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters27Enhancing Waste Plastic Hydrogenolysis on Ru/CeO 2 Through Concurrent Incorporation of Fe Single Atoms and FeO x Nanoclusters4Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels4Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Hydrogenolysis of LDPE over Ni-catalyst promoted by n-hexane solvent7Methods for Carbon Mass Closure in Polyolefin Hydrocracking6A Practical Guide to Heterogeneous Catalysis in Hydrocarbon Transformations10Integrated low-temperature PVC and polyolefin upgrading38Long-lived metal-zeolite catalysts for polyolefin aromatization via synergistic tandem dehydroaromatization and hydrogenolysis12Light-responsive Cu2O–tannic acid nanoparticles enhance the fruit preservation performance of pectin films5Fine regulation of Ru species improved the polyethylene hydrogenolysis performance over Ru/Al 2 O 3 catalyst5Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Production of renewable methyl tert-butyl ether and bioethyl-tertiary-butyl ether from lignocellulosic biomass and its applications as an energy source0Light bulb-inspired high-temperature catalytic depolymerization of polyolefin plastic with high monomer selectivity9A review of recent advances in thermal-catalytic cracking of plastic waste8Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Selective polyethylene hydrocracking to liquid and gaseous hydrocarbons over Co–Ni catalysts supported on H-BEA zeolite10Intrinsically Bifunctional and Tunable Tungsten Carbide Catalysts Enable Efficient PVC-Compatible Polyolefin Hydrocracking8Single-Atom Ni on Tungsten Oxides Drives Hydrogen Spillover for Efficient Plastic Waste Upcycling13Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Converting natural biopolymers to sustainable bioplastics via structure engineering15Highly selective production of gasoline-range hydrocarbons via hydroconversion of polyolefins over Ru/CeO 2 and BEA hybrid catalysts0Plastic Waste Conversion into Monomers Using Microwaves0Synergistic pore-acidity engineering of hierarchical ZSM-5 for hydrogen-free upcycling of Polyethylene to C8–C12 Methylated Aromatics1Tuning ruthenium states for enhanced polyethylene hydroconversion over HZSM-5 catalysts0Upcycling waste polyoxymethylene to value-added chemicals using reusable polymeric acid catalysts at ppm levels2Engineering Microporous Zn-Functionalized Carbon Catalysts for Controllable Chain Cracking and Aromatization in Polyethylene Upcycling1Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Efficient polyolefin upcycling to liquid fuels via Ru–zeolite physical mixtures and pathway control2Hydrocracking Polyolefins to Jet Fuel over a NiW/WO x Catalyst2Low-Temperature Upcycling of Polyethylene into Fuel-Range Hydrocarbons: An Innovative Approach on the Feed-Catalyst Bed Design1Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Recent advancements in catalytic processes for plastic upcycling into fuels: a major step in sustainable waste management and energy production3Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling0Precision bond cleavage in waste plastics: Directed catalytic upcycling1iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Facile synthesis of NiO/C catalyst for microwave-assisted pyrolysis of polypropylene and polyethylene with high selectivity to liquid hydrocarbons and high-value-added products1Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Collaborative Pt–Ni Sites Enable CO-Tolerant Hydrocracking for Upcycling Polyolefin Waste1Machine learning induced tandem catalysis for high-value recovery of polyolefins: pathways, mechanisms and products0Unlocking cost and carbon parity with polyethylene recycling0Elucidating the Spatiotemporal Reaction Mechanism of Polyethylene Aromatization over ZSM-5 Zeolites1Enabling Refinery Integration for Plastic Waste Recycling: A Probabilistic Techno-economic Analysis and Carbon Footprint Assessment of Poly-Crude Production0Impact of Site Identity, Location, and Accessibility on Polyethylene Conversion Rates and Product Selectivities over Metal-Free MFI Zeolites0Confined Isomerization Enables Solar-Thermal Upcycling of Polyolefins into High-Octane Gasoline0Catalytic solvothermal upcycling of mixed polyolefin waste into gasoline-range liquid fuels: Solvent-assisted selectivity and coke kinetics over zeolite-based catalysts0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Hydrodeoxygenation of Mixed Plastic Wastes Towards Aviation Fuels over Ni−Re Alloy Catalyst0From Polyolefin Plastics Back to Olefins: Chemical Recycling and Circular Economy0In-situ hydrogen generation via water-gas shift reaction over Ni-Fe3O4/USY: A sustainable pathway for efficient polypropylene hydrogenolysis0Silicate-cluster-directed formation of mesopores and interfacial Brønsted acid sites in amorphous silica-alumina from zeolite desilication effluents0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Dual-Pathway Polyolefin Upcycling over an Unexpectedly Bifunctional Low-Loading Ru/TiO2-Anatase Catalyst

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  2. Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review

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  3. Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals

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  4. Evolution of light olefins during the pyrolysis of polyethylene in a two-stage process

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  5. Site-Selective Polyolefin Hydrogenolysis on Atomic Ru for Methanation Suppression and Liquid Fuel Production

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  6. Transport limitations in polyolefin cracking at the single catalyst particle level

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  8. Liquid fuel production from catalytic pyrolysis of municipal plastic waste using synthesized Zeolite from Kaolin

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  11. Efficient solvent- and hydrogen-free upcycling of high-density polyethylene into separable cyclic hydrocarbons

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  14. Hydrogen-free catalytic depolymerization of waste polyolefins at mild temperatures

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  15. Photothermal recycling of waste polyolefin plastics into liquid fuels with high selectivity under solvent-free conditions

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  16. Upcycling of polyethylenes by catalysis

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  17. SMSI-induced charge transfer for selective hydrogenolysis of polyolefins

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  18. Activity of Silica-Alumina for the Conversion of Polyethylene into Tunable Aromatics Below Pyrolytic Temperatures

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  19. Construction of Highly Active and Selective Molecular Imprinting Catalyst for Hydrogenation

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  23. Ce-Promoted PtSn-Based Catalyst for Hydrocracking of Polyolefin Plastic Waste into High Yield of Gasoline-Range Products

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  32. Silica as support and binder in bifunctional catalysts with ultralow Pt loadings for the hydroconversion of n-alkanes

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  33. Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters

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  34. Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters

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  35. Shape Selectivity of AEL Channels for Anomalously Facilitating Biojet Fuel Production from Long-Chain n-Alkane Hydrocracking

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  36. Engineering non-noble Ni/WOx-ZrO2 towards boosted fuels production by catalytic upcycling of polyethylene at mild conditions

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  37. Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste

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  39. Tandem catalysis enables chlorine-containing waste as chlorination reagents

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  40. Enhanced hydroconversion of polyethylene via dual-functional catalysis: Exploiting ZSM-22 pore-mouth catalysis and Ru electronic effect

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  42. PLASTAMINATION: Outcomes on the Central Nervous System and Reproduction

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  43. Layered Double Hydroxide Derivatives for Polyolefin Upcycling

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  44. Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels

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  45. Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts

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  46. Influence of Autoclave Liner on Polyethylene Hydrogenolysis Selectivity

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  47. Pioneering Aromatic Generation from Plastic Waste via Catalytic Thermolysis: A Minireview

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  48. Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design

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    Haokun Wang, Shik Chi Edman Tsang

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  49. Advancing Plastic Recycling: A Review on the Synthesis and Applications of Hierarchical Zeolites in Waste Plastic Hydrocracking

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