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RESEARCH PAPER · Advanced Science · 2022

How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics Recycling

Junliang Chen, Jing Wu, Peter Cameron Sherrell, Jun Chen, Huaping Wang, Wei‐xian Zhang, Jianping Yang

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How to Build a Microplastics‐Free Environment: Strategies for Microplastics Degradation and Plastics RecyclingOriginalBiodegradable copolyesters based on a “soft” isohexide building block with tunable viscoelasticity and self-adhesiveness7Investigating the Evolution of the Technologies for Collecting Microplastics20Short-process synthetic strategies of sustainable isohexide-based polyesters towards higher molecular weight and commercial applicability31Upgrade of a Slurry Photocatalytic Membrane Reactor Based on a Vertical Filter and an External Membrane and Testing in the Photodegradation of a Model Pollutant in Water39Feasible Degradation of Polyethylene Terephthalate Fiber‐Based Microplastics in Alkaline Media with Bi 2 O 3 @N‐TiO 2 Z‐Scheme Photocatalytic System87Plastic wastes derived carbon materials for green energy and sustainable environmental applications112Efficient Photocatalytic Degradation of the Persistent PET Fiber-Based Microplastics over Pt Nanoparticles Decorated N-Doped TiO2 Nanoflowers180Fiber Materials for Electrocatalysis Applications86Macromolecular Metabolism Based on Enaminoneamide Achieving Transformation of Polymer Architecture7Removal of microplastics by coagulation treatment in waters and prospect of recycling of separated microplastics: A mini-review51Removal of microplastics and nanoplastics from urban waters: Separation and degradation164Emerging electrochemical techniques for identifying and removing micro/nanoplastics in urban waters132Superhydrophobic PET@ZnO Nanofibrous Membrane Extract from Waste Plastic for Efficient Water-In-Oil Emulsion Separation49Emerging adsorbents for micro/nanoplastics removal from contaminated water: Advances and perspectives103Waste Textile Reutilization Via a Scalable Dyeing Technology: A Strategy to Enhance Dyestuffs Degradation Efficiency78Iron‐Based Nanocatalysts for Electrochemical Nitrate Reduction166Remediation technology towards zero plastic pollution: Recent advance and perspectives30Recycling and Upgrading Utilization of Polymer Plastics †34Conjugated Polymer Nanoparticles as a Universal High-Affinity Probe for the Selective Detection of Microplastics22Microplastics contamination associated with low-value domestic source organic solid waste: A review24Photothermal Catalytic Polyester Upcycling over Cobalt Single‐Site Catalyst129Photo/electro-catalytic degradation of micro- and nano-plastics by nanomaterials and corresponding degradation mechanism44Personal protective equipment (PPE) disposal during COVID-19: An emerging source of microplastic and microfiber pollution in the environment100Mechanically Strong and Tough Poly(urea‐urethane) Thermosets Capable of Being Degraded under Mild Condition12Waste-Derived Catalysts for Water Electrolysis: Circular Economy-Driven Sustainable Green Hydrogen Energy207Aquatic Microplastic Pollution Control Strategies: Sustainable Degradation Techniques, Resource Recovery, and Recommendations for Bangladesh65Molecular mechanisms of microplastics degradation: A review106Innovations in the Development of Promising Adsorbents for the Remediation of Microplastics and Nanoplastics – A Critical Review160Advancements in catalysis for plastic resource utilization21An iron “nano-fishnet” for the rapid removal and surface clean-up of micro/nanoplastics from seawater11Future Research on the Sustainable Utilization of Wastewater as Resources with Emphasis on Plastics0Microplastics Remediation in the Aqueous Environment0Surface topography of nanoplastics modulates their internalization and toxicity in liver cells10Techniques for Removal and Degradation of Microplastics20The Impact of Microplastics on Tissue-specific Gene Expression in the Tropical House Cricket, G. sigillatus0Recycling of Plastic Wastes for the Mass Production of Yolk–Shell-Nanostructured Co3O4@C for Lithium-Ion Batteries27Stretchable, Ultratough, and Intrinsically Self‐Extinguishing Elastomers with Desirable Recyclability167Biotechnological methods to remove microplastics: a review255Biomimetic Bridging for Reconstructing Biomass Components toward Significantly Enhanced Films from the Full Composition of Bamboo25Bandgap engineering approach for designing CuO/Mn3O4/CeO2 heterojunction as a novel photocatalyst for AOP-assisted degradation of Malachite green dye48The potential risks posed by micro-nanoplastics to the safety of disinfected drinking water29Pollution concerns in mariculture water and cultured economical bivalves: Occurrence of microplastics under different aquaculture modes48In vitro wheat protoplast cytotoxicity of polystyrene nanoplastics24Fate and Removal of Microplastics from Industrial Wastewaters54Microplastics in soils during the COVID-19 pandemic: Sources, migration and transformations, and remediation technologies36Global plastic upcycling during and after the COVID-19 pandemic: The status and perspective30Insight into photocatalysis technology as a promising approach to tackle microplastics pollution through degradation and upcycling87Photocatalytic Microplastics “On‐The‐fly” Degradation via Motile Quantum Materials‐Based Microrobots37Contemporary Drift in Emerging Micro(nano)plastics Removal and Upcycling Technologies from Municipal Wastewater Sludge: Strategic Innovations and Prospects43Plastic or plastic-free life: From formation to removal32Advanced oxidation processes for the degradation of microplastics from the environment: A review32The removal characteristics and mechanisms of polystyrene microplastics with various induced photoaging degrees by CuFe2O430Fundamental steps and considerations in the analysis of micro- and nanoplastics in wastewaters, sludges, and comparable matrices1Light‐Powered Self‐Adaptive Mesostructured Microrobots for Simultaneous Microplastics Trapping and Fragmentation via in situ Surface Morphing36Effect of carbon black particle size in chitin sponges on microplastics adsorption65Towards a plastic-less planet. Gender and individual responsibility predict the effect of imagery nudges about marine (micro)plastic pollution on R-behavior intentions6Microplastics in construction and built environment97Photocatalytic Upcycling of Plastic Waste: Mechanism, Integrating Modus, and Selectivity77Degradation of plastic wastes to commercial chemicals and monomers under visible light130Microplastics in the soil environment: Focusing on the sources, its transformation and change in morphology53Discovery and mechanism-guided engineering of BHET hydrolases for improved PET recycling and upcycling111Simultaneous removal of microplastics and doxycycline and preparation of novel hollow carbon nanocakes by pyrolysis15Grasping the supremacy of microplastic in the environment to understand its implications and eradication: a review13Green Techniques for Detecting Microplastics in Marine with Emphasis on FTIR and NIR Spectroscopy—Short Review29Review on design strategies and applications of flexible cellulose‑carbon nanotube functional composites54High Performance Triboelectric Nanogenerators from Compostable Cellulose‐Biodegradable Poly(Butylene Succinate) Composites15Systematic Review of Degradation Processes for Microplastics: Progress and Prospects51An innovative remedy to transform plastic waste and used paper box into high-performance biocomposite4Advanced oxidation processes for removal of organic micropollutants from wastewater22Biological-mechanical pretreated rice straw for constructing foam with mechanically robust and fire-retardant behaviors17Microplastic Pollution: Threats and Impacts on Global Marine Ecosystems98Microplastics sequestered in the soil affect the turnover and stability of soil aggregates: A review63Dual-Doped Nickel Sulfide for Electro-Upgrading Polyethylene Terephthalate into Valuable Chemicals and Hydrogen Fuel130From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Encapsulation of carbon-nanodots into metal-organic frameworks for boosting photocatalytic upcycling of polyvinyl chloride plastic80Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals133Micro- and nano-plastics in food systems: Distribution, combined toxicity with environmental contaminants, and removal strategies23Microplastics as carriers of antibiotic resistance genes and pathogens in municipal solid waste (MSW) landfill leachate and soil: a review34Deamination of Polyols from the Glycolysis of Polyurethane30Photocatalytic degradation of different types of microplastics by TiOx/ZnO tetrapod photocatalysts95Indirect daylight oxidative degradation of polyethylene microplastics by a bio-waste modified TiO2-based material33Ordered mesoporous materials for water pollution treatment: Adsorption and catalysis123Application of advanced oxidation processes for the removal of micro/nanoplastics from water: A review51Environmental Sustainability of Solvent Extraction Method in Recycling Marine Plastic Waste14Concurrent electrocatalytic hydrogen evolution and polyethylene terephthalate plastics reforming by self-supported amorphous cobalt iron phosphide electrode55Layered double hydroxides derived from waste for highly efficient electrocatalytic water splitting: Challenges and implications towards circular economy driven green energy53Removal Mechanisms of Polyethylene, Polypropylene, Polyvinyl Chloride, Polyamide (Nylon), Polystyrene and Polyethylene Terephthalate in Wastewater Treatment Plants by Chemical, Photocatalytic, Biodegradation and Hybrid Processes19Bacteria and Yeasts Isolated from the Environment in Biodegradation of PS and PVC Microplastics: Screening and Treatment Optimization10Environmental aspects of restoring the environment: nanotechnology for removing micro and nanoplastics from water0Chemical recycling of plastic wastes via homogeneous catalysis: A review78Reprocessable and chemically recyclable poly(acylhydrazone–imine) covalent adaptable networks with enhanced mechanical strength and creep resistance17Dual-channel fluorescence dye: Fluorescent color-dependent visual detection of microplastics and selective polyurethane30A novel bio‐based charcoal‐forming agent based on chitosan and phytate@Mg to improve the flame retardancy of poly(lactic acid)6Bioengineering Comamonas testosteroni CNB-1: a robust whole-cell biocatalyst for efficient PET microplastic degradation29Organic Electrode Materials for Dual‐Ion Batteries38Decomposition of metal-organic complexes and metal recovery in wastewater: A systematic review and meta-synthesis14Recent advancement on photocatalytic plastic upcycling90Monomer recycling of polyethylene terephthalate, polycarbonate and polyethers: Scalable processes to achieve high carbon circularity62Bimetallic CoNi-metal–organic framework@molybdenum disulfide core–shell Z-scheme heterojunctions with broad-spectrum response toward optimized photocatalytic performance6Complete Conversion of Waste Pet into Dimethyl Terephthalate and Ethylene Carbonate0Efficient Degradation of Oxidized Polyethylene Containing Ester Bonds by Cutinase or Lipase in Aqueous Phase0High crystalline LDHs with strong adsorption properties effectively remove oil and micro-nano plastics38Nanophotocatalytic conversion of biomass to bioenergy2Occurrence, Fate, and Biodegradation of Microplastics in Marine Environments2Photocatalytic systems: reactions, mechanism, and applications437Plastic Waste Management for Zero Waste to Landfills: Potential, Challenges, and Opportunities13Recent Progress in Electrochemical Methods for Microplastics Detection6Ring-opening polymerization of cyclic esters mediated by base/(thio)urea binary catalysts toward sustainable polyesters21The Effects of the Alkyl Chain Length of Novel Phosphorus-Nitrogen-Containing Lactic Acid-Based Flame-Retardant Plasticizers on Toughness, Flame Retardancy and Crystallization of Poly (Lactic Acid)0The Removal of Microplastics as a Source for Toxic Chemicals in Aquatic Environments: Characteristics, Occurrence and Removal Mechanisms0UNVEILING THE POTENTIAL OF METAGENOMICS FOR ERADICATING MICROPLASTICS FROM DRINKING WATER0Wastewater Treatment Plants and Microplastic Degradation1Upcycling plastic wastes into value-added products via electrocatalysis and photoelectrocatalysis61An insight decipher on photocatalytic degradation of microplastics: Mechanism, limitations, and future outlook134Innovations in chemical degradation technologies for the removal of micro/nano-plastics in water: A comprehensive review20Stereocomplexation-Enhanced Electroactivity of Poly(lactic acid) Nanofibrous Membranes for Long-Term PM Capturing and Remote Respiratory Monitoring51Facile synthesis of MoS2 nanoparticles anchored graphene nanocomposite for enhanced photocatalytic activity under solar irradiation10Effects of charged polystyrene microplastics on the bioavailability of dufulin in tomato plant21Mining strategies for isolating plastic-degrading microorganisms15Ring-Opening Polymerization of Lactones to Prepare Closed-Loop Recyclable Polyesters116Evaluation of Fenton, Photo-Fenton and Fenton-like Processes in Degradation of PE, PP, and PVC Microplastics70Enhanced biodegradation activity toward polyethylene by fusion protein of anchor peptide and Streptomyces sp. strain K30 latex clearing protein13Occurrence, bioaccumulation, fate, and risk assessment of emerging pollutants in aquatic environments: A review106Sustainable Removal of Nanoplastics: Exploiting the Lipolytic Activity of Pseudomonas aeruginosa O6 Isolated from Mariout Wetland, Egypt5Harnessing photosynthetic microorganisms for enhanced bioremediation of microplastics: A comprehensive review48Photoreforming for microplastics recycling: A critical review26Transport of layered and spherical microplastics in aqueous ecosystems: a review18Microplastic pollution in Vietnam's estuarine, coastal and riverine environments: Research advances and future prospects22Heterostructured Photocatalytic Fabric Composed of Ag3PO4 Nanoparticle-Decorated NH2-MIL-88B (Co/Fe) Crystalline Wires for Rhodamine B Adsorption and Degradation15Recent Progresses in Pyrolysis of Plastic Packaging Wastes and Biomass Materials for Conversion of High-Value Carbons: A Review20Degradation of microplastic in water by advanced oxidation processes68Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Unveiling synergy of strain and ligand effects in metallic aerogel for electrocatalytic polyethylene terephthalate upcycling117From sustainable macro debris chemical recycling to microplastic reclamation: Overview, research challenges, and outlook9Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Electrocatalysis for Green(er) Chemistry: Limitations and Opportunities with Traditional and Emerging Characterization Methods for Tangible Societal Impact20Effect of Amino Acid Ionic Liquids on the Interfacial Structure and Degradation Behavior of PLA/PBAT Blends9Magnetic Harvesting and Degradation of Microplastics using Iron Oxide Nanoflowers prepared by a Scaled-up Procedure44Emerging Environmental Contaminats of High Concern: Trends, Potential Sources, Friendly Treatment Technologies and Future Prospects0Formulation and application assessment of lignin-based biodegradable composite mulching film with emphasis on lignin enhancement41A Comparison of new and age-old approaches treating microplastics in the marine environment0Environmental risk substances in soil on seed germination: Chemical species, inhibition performance, and mechanisms22Modified Sodium Alginate for Degradable Supramolecular Plastic with High Mechanical Strength2Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species51Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species8High barrier polyesters based on 2,5-furandicarboxylic acid and disulfide bond: Smart degradation induced by low concentrations of redox reagent7Preparation of green biodegradable lactic acid-based flame-retardant plasticizer for simultaneously enhancing flexibility, flame retardancy, and smoke-suppression of poly(lactic acid)24Simulation of the dynamic processes of microplastic suspension and deposition in a lake sediment–water system10Biochar as adsorbents for environmental microplastics and nanoplastics removal118

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  19. Conjugated Polymer Nanoparticles as a Universal High-Affinity Probe for the Selective Detection of Microplastics

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  43. In vitro wheat protoplast cytotoxicity of polystyrene nanoplastics

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  44. Fate and Removal of Microplastics from Industrial Wastewaters

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  45. Microplastics in soils during the COVID-19 pandemic: Sources, migration and transformations, and remediation technologies

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  46. Global plastic upcycling during and after the COVID-19 pandemic: The status and perspective

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  47. Insight into photocatalysis technology as a promising approach to tackle microplastics pollution through degradation and upcycling

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  48. Photocatalytic Microplastics “On‐The‐fly” Degradation via Motile Quantum Materials‐Based Microrobots

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  49. Contemporary Drift in Emerging Micro(nano)plastics Removal and Upcycling Technologies from Municipal Wastewater Sludge: Strategic Innovations and Prospects

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